Industrial & Engineering Chemistry Research, volume 58, issue 20, pages 8612-8624
Indirect Z-Scheme Assembly of 2D ZnV2O6/RGO/g-C3N4 Nanosheets with RGO/pCN as Solid-State Electron Mediators toward Visible-Light-Enhanced CO2 Reduction
Publication type: Journal Article
Publication date: 2019-04-12
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 4.2
ISSN: 08885885, 15205045
General Chemistry
General Chemical Engineering
Industrial and Manufacturing Engineering
Abstract
Indirect Z-scheme assembly of graphene-bridged 2D ZnV2O6/pCN nanosheets composite has been fabricated by one-step solvothermal process and tested for photoinduced CO2 conversion under visible-light irradiations. The highest CH3OH production of 3488 μmol g-cat–1 was obtained over ZnV2O6/RGO/g-C3N4 composite, 1.02 and 1.25 times higher comparing to ZnV2O6/RGO and ZnV2O6/g-C3N4 samples, respectively. This enhanced efficiency can be ascribed to well-designed ternary heterojunction with hierarchical structure and efficient charges separation by RGO. More importantly, CH3OH yield was further improved by introducing RGO/pCN as an electron sink, which led to a 1.07 times higher yield than using only RGO. This reveals that ternary 2D ZnV2O6/RGO/pCN nanostructure has higher visible-light absorption, improved charge separation, and enhanced photocatalytic efficiency due to RGO/pCN as multiple mediators. The stability of composite catalyst also prevailed for 32 h for continuous CH3OH production. Therefore, structured...
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Citations by publishers
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1 publication, 1.3%
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IOS Press
1 publication, 1.3%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Bafaqeer A. et al. Indirect Z-Scheme Assembly of 2D ZnV2O6/RGO/g-C3N4 Nanosheets with RGO/pCN as Solid-State Electron Mediators toward Visible-Light-Enhanced CO2 Reduction // Industrial & Engineering Chemistry Research. 2019. Vol. 58. No. 20. pp. 8612-8624.
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Bafaqeer A., Tahir M., Ali Khan A., Amin N. S. Indirect Z-Scheme Assembly of 2D ZnV2O6/RGO/g-C3N4 Nanosheets with RGO/pCN as Solid-State Electron Mediators toward Visible-Light-Enhanced CO2 Reduction // Industrial & Engineering Chemistry Research. 2019. Vol. 58. No. 20. pp. 8612-8624.
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TY - JOUR
DO - 10.1021/acs.iecr.8b06053
UR - https://doi.org/10.1021/acs.iecr.8b06053
TI - Indirect Z-Scheme Assembly of 2D ZnV2O6/RGO/g-C3N4 Nanosheets with RGO/pCN as Solid-State Electron Mediators toward Visible-Light-Enhanced CO2 Reduction
T2 - Industrial & Engineering Chemistry Research
AU - Bafaqeer, Abdullah
AU - Tahir, Muhammad
AU - Ali Khan, Azmat
AU - Amin, NorAishah Saidina
PY - 2019
DA - 2019/04/12 00:00:00
PB - American Chemical Society (ACS)
SP - 8612-8624
IS - 20
VL - 58
SN - 0888-5885
SN - 1520-5045
ER -
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@article{2019_Bafaqeer,
author = {Abdullah Bafaqeer and Muhammad Tahir and Azmat Ali Khan and NorAishah Saidina Amin},
title = {Indirect Z-Scheme Assembly of 2D ZnV2O6/RGO/g-C3N4 Nanosheets with RGO/pCN as Solid-State Electron Mediators toward Visible-Light-Enhanced CO2 Reduction},
journal = {Industrial & Engineering Chemistry Research},
year = {2019},
volume = {58},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/acs.iecr.8b06053},
number = {20},
pages = {8612--8624},
doi = {10.1021/acs.iecr.8b06053}
}
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Bafaqeer, Abdullah, et al. “Indirect Z-Scheme Assembly of 2D ZnV2O6/RGO/g-C3N4 Nanosheets with RGO/pCN as Solid-State Electron Mediators toward Visible-Light-Enhanced CO2 Reduction.” Industrial & Engineering Chemistry Research, vol. 58, no. 20, Apr. 2019, pp. 8612-8624. https://doi.org/10.1021/acs.iecr.8b06053.