Insight on the Sequential Vapor Infiltration Mechanisms of Trimethylaluminum with Poly(methyl methacrylate), Poly(vinylpyrrolidone), and Poly(acrylic acid)
Тип публикации: Journal Article
Дата публикации: 2019-06-14
scimago Q1
wos Q3
БС1
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Краткое описание
The sequential vapor infiltration (SVI) method, based on atomic layer deposition chemistry, allows the creation of a polymer–inorganic hybrid material through the diffusion of metal–organic vapor reagents into a polymer substrate. This study investigates the reactivity of the ester, amide, and carboxylic acid functional groups of poly(methyl methacrylate) (PMMA), poly(vinylpyrrolidone) (PVP), and poly(acrylic acid) (PAA), respectively, in the presence of trimethylaluminum (TMA) vapor. This work explores the possible reaction mechanisms of these functional groups through in situ Fourier transform infrared spectroscopy and ab initio quantum chemical analysis. At temperatures of ≤100 °C, TMA physisorbs to the carbonyl groups of PMMA. As the temperature is increased, TMA forms a covalent bond with PMMA. TMA physisorbs to PVP and then partially desorbs in the presence of water for all studied temperatures of ≤150 °C. PAA readily reacts with TMA to form a covalent bond with the carbonyl group at 60 °C. This inc...
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Hill G. T. et al. Insight on the Sequential Vapor Infiltration Mechanisms of Trimethylaluminum with Poly(methyl methacrylate), Poly(vinylpyrrolidone), and Poly(acrylic acid) // Journal of Physical Chemistry C. 2019. Vol. 123. No. 26. pp. 16146-16152.
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Hill G. T., Lee D. T., Williams P. S., Needham C. D., Dandley E. C., Oldham C., Parsons G. Insight on the Sequential Vapor Infiltration Mechanisms of Trimethylaluminum with Poly(methyl methacrylate), Poly(vinylpyrrolidone), and Poly(acrylic acid) // Journal of Physical Chemistry C. 2019. Vol. 123. No. 26. pp. 16146-16152.
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TY - JOUR
DO - 10.1021/acs.jpcc.9b02153
UR - https://doi.org/10.1021/acs.jpcc.9b02153
TI - Insight on the Sequential Vapor Infiltration Mechanisms of Trimethylaluminum with Poly(methyl methacrylate), Poly(vinylpyrrolidone), and Poly(acrylic acid)
T2 - Journal of Physical Chemistry C
AU - Hill, Grant T
AU - Lee, Dennis T
AU - Williams, Philip S
AU - Needham, Craig D
AU - Dandley, Erinn C
AU - Oldham, Christopher
AU - Parsons, Gregory
PY - 2019
DA - 2019/06/14
PB - American Chemical Society (ACS)
SP - 16146-16152
IS - 26
VL - 123
SN - 1932-7447
SN - 1932-7455
ER -
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@article{2019_Hill,
author = {Grant T Hill and Dennis T Lee and Philip S Williams and Craig D Needham and Erinn C Dandley and Christopher Oldham and Gregory Parsons},
title = {Insight on the Sequential Vapor Infiltration Mechanisms of Trimethylaluminum with Poly(methyl methacrylate), Poly(vinylpyrrolidone), and Poly(acrylic acid)},
journal = {Journal of Physical Chemistry C},
year = {2019},
volume = {123},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acs.jpcc.9b02153},
number = {26},
pages = {16146--16152},
doi = {10.1021/acs.jpcc.9b02153}
}
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Hill, Grant T., et al. “Insight on the Sequential Vapor Infiltration Mechanisms of Trimethylaluminum with Poly(methyl methacrylate), Poly(vinylpyrrolidone), and Poly(acrylic acid).” Journal of Physical Chemistry C, vol. 123, no. 26, Jun. 2019, pp. 16146-16152. https://doi.org/10.1021/acs.jpcc.9b02153.