Macromolecular Brushes by Combination of Ring-Opening and Ring-Opening Metathesis Polymerization. Synthesis, Self-Assembly, Thermodynamics, and Dynamics
Christiana Nikovia
1
,
Lazaros Theodoridis
2
,
Stelios Alexandris
2
,
Panayiotis Bilalis
3
,
N. Hadjichristidis
3
,
George Floudas
2
,
M Pitsikalis
1
Publication type: Journal Article
Publication date: 2018-10-31
scimago Q1
wos Q1
SJR: 1.352
CiteScore: 9.0
Impact factor: 5.2
ISSN: 00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Abstract
Statistical and block copolymerization of poly(l-lactide) (PLLA) and poly(e-caprolactone) (PCL) macromonomers having an end norbornenyl group was performed via ring-opening metathesis polymerization (ROMP) to produce the corresponding statistical and block brush copolymers consisting of PLLA and PCL side chains on a polynorbornene (PNBE) backbone. The molecular characteristics of the macromolecular brushes were determined by 1H NMR spectroscopy and size exclusion chromatography equipped with various detectors. These complex topologies allow addressing important questions on the physics of semicrystalline polymers. These include the role of (i) a doubly grafted PCL or PLLA chain on a NBE moiety (in the macromonomers) and the role of (ii) brush architecture on the crystallization behavior and dynamics of block and statistical copolymers. Significant differences were found between the macromonomers and the corresponding brush copolymers at the crystalline lamellar and spherulitic superstructure levels. In th...
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Total citations:
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Citations from 2024:
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(11.54%)
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GOST
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Nikovia C. et al. Macromolecular Brushes by Combination of Ring-Opening and Ring-Opening Metathesis Polymerization. Synthesis, Self-Assembly, Thermodynamics, and Dynamics // Macromolecules. 2018. Vol. 51. No. 21. pp. 8940-8955.
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Nikovia C., Theodoridis L., Alexandris S., Bilalis P., Hadjichristidis N., Floudas G., Pitsikalis M. Macromolecular Brushes by Combination of Ring-Opening and Ring-Opening Metathesis Polymerization. Synthesis, Self-Assembly, Thermodynamics, and Dynamics // Macromolecules. 2018. Vol. 51. No. 21. pp. 8940-8955.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.macromol.8b01905
UR - https://doi.org/10.1021/acs.macromol.8b01905
TI - Macromolecular Brushes by Combination of Ring-Opening and Ring-Opening Metathesis Polymerization. Synthesis, Self-Assembly, Thermodynamics, and Dynamics
T2 - Macromolecules
AU - Nikovia, Christiana
AU - Theodoridis, Lazaros
AU - Alexandris, Stelios
AU - Bilalis, Panayiotis
AU - Hadjichristidis, N.
AU - Floudas, George
AU - Pitsikalis, M
PY - 2018
DA - 2018/10/31
PB - American Chemical Society (ACS)
SP - 8940-8955
IS - 21
VL - 51
SN - 0024-9297
SN - 1520-5835
ER -
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BibTex (up to 50 authors)
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@article{2018_Nikovia,
author = {Christiana Nikovia and Lazaros Theodoridis and Stelios Alexandris and Panayiotis Bilalis and N. Hadjichristidis and George Floudas and M Pitsikalis},
title = {Macromolecular Brushes by Combination of Ring-Opening and Ring-Opening Metathesis Polymerization. Synthesis, Self-Assembly, Thermodynamics, and Dynamics},
journal = {Macromolecules},
year = {2018},
volume = {51},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/acs.macromol.8b01905},
number = {21},
pages = {8940--8955},
doi = {10.1021/acs.macromol.8b01905}
}
Cite this
MLA
Copy
Nikovia, Christiana, et al. “Macromolecular Brushes by Combination of Ring-Opening and Ring-Opening Metathesis Polymerization. Synthesis, Self-Assembly, Thermodynamics, and Dynamics.” Macromolecules, vol. 51, no. 21, Oct. 2018, pp. 8940-8955. https://doi.org/10.1021/acs.macromol.8b01905.