Ruthenium Olefin Metathesis Catalysts with Six-Membered Chelating Dithioacetal Ligands: Synthesis and Reactivity
Gal Segalovich Gerendash
1
,
Gal Segalovich-Gerendash
1
,
Mark Baranov
1
,
N Gabriel Lemcoff
1, 2
,
Ravindra S Phatake
1, 3
2
Ilse Katz Institute for Nanoscale Science and Technology, Beer-Sheva 8410501, Israel
|
Publication type: Journal Article
Publication date: 2023-04-27
scimago Q2
wos Q1
SJR: 0.676
CiteScore: 5.1
Impact factor: 2.9
ISSN: 02767333, 15206041
Organic Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Ruthenium sulfur-chelated benzylidenes possessing five-membered chelating architectures exhibiting latency and excellent thermal and photochemical activation behavior in various metathesis reactions are well known. On the other hand, six-membered sulfur-Ru-chelates (Ru–S) are much rarer. Herein, we describe a study of the synthesis, characterization, and catalytic properties of four new cis-dichlorido ruthenium dithioacetal-chelated complexes. As expected for sulfur-chelated benzylidenes, the X-ray structures of the complexes disclosed cis-dichloro configurations for all the complexes. The catalytic profiles of these complexes were systematically studied for benchmark RCM and ROMP reactions and provided findings on latency and activation based on chelating dithioacetal groups.
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11
Total citations:
11
Citations from 2024:
9
(81.82%)
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GOST
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Segalovich Gerendash G. et al. Ruthenium Olefin Metathesis Catalysts with Six-Membered Chelating Dithioacetal Ligands: Synthesis and Reactivity // Organometallics. 2023. Vol. 42. No. 9. pp. 825-831.
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Segalovich Gerendash G., Segalovich-Gerendash G., Baranov M., Lemcoff N. G., Phatake R. S. Ruthenium Olefin Metathesis Catalysts with Six-Membered Chelating Dithioacetal Ligands: Synthesis and Reactivity // Organometallics. 2023. Vol. 42. No. 9. pp. 825-831.
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RIS
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TY - JOUR
DO - 10.1021/acs.organomet.3c00093
UR - https://pubs.acs.org/doi/10.1021/acs.organomet.3c00093
TI - Ruthenium Olefin Metathesis Catalysts with Six-Membered Chelating Dithioacetal Ligands: Synthesis and Reactivity
T2 - Organometallics
AU - Segalovich Gerendash, Gal
AU - Segalovich-Gerendash, Gal
AU - Baranov, Mark
AU - Lemcoff, N Gabriel
AU - Phatake, Ravindra S
PY - 2023
DA - 2023/04/27
PB - American Chemical Society (ACS)
SP - 825-831
IS - 9
VL - 42
SN - 0276-7333
SN - 1520-6041
ER -
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BibTex (up to 50 authors)
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@article{2023_Segalovich Gerendash,
author = {Gal Segalovich Gerendash and Gal Segalovich-Gerendash and Mark Baranov and N Gabriel Lemcoff and Ravindra S Phatake},
title = {Ruthenium Olefin Metathesis Catalysts with Six-Membered Chelating Dithioacetal Ligands: Synthesis and Reactivity},
journal = {Organometallics},
year = {2023},
volume = {42},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://pubs.acs.org/doi/10.1021/acs.organomet.3c00093},
number = {9},
pages = {825--831},
doi = {10.1021/acs.organomet.3c00093}
}
Cite this
MLA
Copy
Segalovich Gerendash, Gal, et al. “Ruthenium Olefin Metathesis Catalysts with Six-Membered Chelating Dithioacetal Ligands: Synthesis and Reactivity.” Organometallics, vol. 42, no. 9, Apr. 2023, pp. 825-831. https://pubs.acs.org/doi/10.1021/acs.organomet.3c00093.
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