volume 68 issue 5 pages 1954-1957

Dual Nucleophilic Catalysis with DABCO for the N-Methylation of Indoles

Wen-Chung Shieh 1
Steven Dell 1
Andrew Bach 1
Oljan Repič 1
Thomas J. Blacklock 1
1
 
Chemical and Analytical Development, Novartis Institute for Biomedical Research, East Hanover, New Jersey 07936
Publication typeJournal Article
Publication date2003-02-07
scimago Q2
wos Q1
SJR0.737
CiteScore6.1
Impact factor3.6
ISSN00223263, 15206904
PubMed ID:  12608816
Organic Chemistry
Abstract
DABCO is an extremely active catalyst for the methylation of indoles in conjunction with dimethyl carbonate (DMC). This green chemistry is highly effective and produces N-methylindoles in nearly quantitative yields. The reaction sequence consists of competing alkylation and acylation pathways and involves 1,4-diazabicyclo[2.2.2]octane (DABCO) dually as a nucleophilic catalyst, ultimately resulting in a single product: the N-methylated indole.
Found 
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GOST |
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GOST Copy
Shieh W. et al. Dual Nucleophilic Catalysis with DABCO for the N-Methylation of Indoles // Journal of Organic Chemistry. 2003. Vol. 68. No. 5. pp. 1954-1957.
GOST all authors (up to 50) Copy
Shieh W., Dell S., Bach A., Repič O., Blacklock T. J. Dual Nucleophilic Catalysis with DABCO for the N-Methylation of Indoles // Journal of Organic Chemistry. 2003. Vol. 68. No. 5. pp. 1954-1957.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1021/jo0266644
UR - https://doi.org/10.1021/jo0266644
TI - Dual Nucleophilic Catalysis with DABCO for the N-Methylation of Indoles
T2 - Journal of Organic Chemistry
AU - Shieh, Wen-Chung
AU - Dell, Steven
AU - Bach, Andrew
AU - Repič, Oljan
AU - Blacklock, Thomas J.
PY - 2003
DA - 2003/02/07
PB - American Chemical Society (ACS)
SP - 1954-1957
IS - 5
VL - 68
PMID - 12608816
SN - 0022-3263
SN - 1520-6904
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2003_Shieh,
author = {Wen-Chung Shieh and Steven Dell and Andrew Bach and Oljan Repič and Thomas J. Blacklock},
title = {Dual Nucleophilic Catalysis with DABCO for the N-Methylation of Indoles},
journal = {Journal of Organic Chemistry},
year = {2003},
volume = {68},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/jo0266644},
number = {5},
pages = {1954--1957},
doi = {10.1021/jo0266644}
}
MLA
Cite this
MLA Copy
Shieh, Wen-Chung, et al. “Dual Nucleophilic Catalysis with DABCO for the N-Methylation of Indoles.” Journal of Organic Chemistry, vol. 68, no. 5, Feb. 2003, pp. 1954-1957. https://doi.org/10.1021/jo0266644.