Inorganic Chemistry, volume 60, issue 3, pages 1755-1766
Constructed Z-Scheme g-C3N4/Ag3VO4/rGO Photocatalysts with Multi-interfacial Electron-Transfer Paths for High Photoreduction of CO2
Ming Gao
1
,
Linlin Sun
1, 2
,
Changchang Ma
1
,
Xiaolin Li
1
,
Haopeng Jiang
1
,
DONG SHEN
1
,
王慧琴 Wang Huiqin
3
,
Pengwei Huo
1
Publication type: Journal Article
Publication date: 2021-01-19
Journal:
Inorganic Chemistry
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 4.6
ISSN: 00201669, 1520510X
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Z-scheme g-C3N4/Ag3VO4/reduced graphene oxide (rGO) photocatalysts with multi-interfacial electron-transfer paths enhancing CO2 photoreduction under UV-vis light irradiation were successfully prepared by a hydrothermal process. Transmission electron microscope images displayed that the prepared photocatalysts have a unique 2D-0D-2D ternary sandwich structure. Photoelectrochemical characterizations including TPR, electrochemical impedance spectroscopy, photoluminescence, and linear sweep voltammetry explained that the multi-interfacial structure effectively improved the separation and transmission capabilities of photogenerated carriers. Electron spin resonance spectroscopy and band position analysis proved that the electron-transfer mode of g-C3N4/Ag3VO4 meets the Z-scheme mechanism. The introduction of rGO provided more electron-transfer paths for the photocatalysts and enhanced the stability of Ag-based semiconductors. In addition, the π-π conjugation effect between g-C3N4 and rGO further improved the generation and separation efficiency of photogenerated electron-hole pairs. Then, the multiple channels (Ag3VO4 → CN, Ag3VO4 → rGO → CN, and rGO → CN) due to the 2D-0D-2D structure greatly improving the photocatalytic CO2 reduction ability have been discussed in detail.
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Gao M. et al. Constructed Z-Scheme g-C3N4/Ag3VO4/rGO Photocatalysts with Multi-interfacial Electron-Transfer Paths for High Photoreduction of CO2 // Inorganic Chemistry. 2021. Vol. 60. No. 3. pp. 1755-1766.
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Gao M., Sun L., Ma C., Li X., Jiang H., SHEN D., Wang Huiqin 王., Huo P. Constructed Z-Scheme g-C3N4/Ag3VO4/rGO Photocatalysts with Multi-interfacial Electron-Transfer Paths for High Photoreduction of CO2 // Inorganic Chemistry. 2021. Vol. 60. No. 3. pp. 1755-1766.
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TY - JOUR
DO - 10.1021/acs.inorgchem.0c03233
UR - https://doi.org/10.1021/acs.inorgchem.0c03233
TI - Constructed Z-Scheme g-C3N4/Ag3VO4/rGO Photocatalysts with Multi-interfacial Electron-Transfer Paths for High Photoreduction of CO2
T2 - Inorganic Chemistry
AU - Sun, Linlin
AU - Jiang, Haopeng
AU - SHEN, DONG
AU - Gao, Ming
AU - Huo, Pengwei
AU - Ma, Changchang
AU - Li, Xiaolin
AU - Wang Huiqin, 王慧琴
PY - 2021
DA - 2021/01/19 00:00:00
PB - American Chemical Society (ACS)
SP - 1755-1766
IS - 3
VL - 60
SN - 0020-1669
SN - 1520-510X
ER -
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@article{2021_Gao,
author = {Linlin Sun and Haopeng Jiang and DONG SHEN and Ming Gao and Pengwei Huo and Changchang Ma and Xiaolin Li and 王慧琴 Wang Huiqin},
title = {Constructed Z-Scheme g-C3N4/Ag3VO4/rGO Photocatalysts with Multi-interfacial Electron-Transfer Paths for High Photoreduction of CO2},
journal = {Inorganic Chemistry},
year = {2021},
volume = {60},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acs.inorgchem.0c03233},
number = {3},
pages = {1755--1766},
doi = {10.1021/acs.inorgchem.0c03233}
}
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MLA
Copy
Gao, Ming, et al. “Constructed Z-Scheme g-C3N4/Ag3VO4/rGO Photocatalysts with Multi-interfacial Electron-Transfer Paths for High Photoreduction of CO2.” Inorganic Chemistry, vol. 60, no. 3, Jan. 2021, pp. 1755-1766. https://doi.org/10.1021/acs.inorgchem.0c03233.