ACS Applied Energy Materials, volume 3, issue 7, pages 6422-6433
Synthesis of the g-C3N4/CdS Nanocomposite with a Chemically Bonded Interface for Enhanced Sunlight-Driven CO2 Photoreduction
1
Department of Chemical Engineering, Laval University, 1065 Avenue de la Médecine, Quebec City, Québec G1V 0A6, Canada
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Publication type: Journal Article
Publication date: 2020-06-17
Journal:
ACS Applied Energy Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 6.4
ISSN: 25740962, 25740962
Materials Chemistry
Electrochemistry
Electrical and Electronic Engineering
Energy Engineering and Power Technology
Chemical Engineering (miscellaneous)
Abstract
The
work, herein, reports a simple approach for the synthesis of
the g-C3N4/CdS nanocomposite. The high pressure NH3 and
H2S, which is created by the polycondensation of thiourea,
processes simultaneously the gas-induced lysis to fracture the carbon
nitride framework, and the sulfidation of adsorbed Cd precursor to
form CdS nanoparticles (NPs) with high crystallinity on the surface
of the modified carbon nitride structure. These processes synchronously
alter the fragmentation mechanism of the carbon nitride framework
and shift the crystal grow orientation of the CdS NPs. Importantly,
they result in the creation of the C–S–Cd bridges that
induce an intimate chemically bonded interface between g-C3N4 and CdS NPs. The heterostructure coupled with this
chemically bonded interface favors effective charge separation and
transfer. The as-prepared nanocomposite photocatalyst exhibits an
efficient sunlight-driven photoreduction of CO2 into CO,
which are superior to those of the g-C3N4 material
and CdS NPs alone, in the presence of the metal–organic complex
as a co-catalyst. CO selectivity is greatly enhanced, as compared
to the g-C3N4 material, indicating the critical
role of CdS NPs in the composite to promote the interaction with the
co-catalyst, thus enhancing the CO2 reduction and decreasing
the side reaction of the H2 evolution.
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5
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
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Vu N. N., Kaliaguine S., Do T. Synthesis of the g-C3N4/CdS Nanocomposite with a Chemically Bonded Interface for Enhanced Sunlight-Driven CO2 Photoreduction // ACS Applied Energy Materials. 2020. Vol. 3. No. 7. pp. 6422-6433.
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Vu N. N., Kaliaguine S., Do T. Synthesis of the g-C3N4/CdS Nanocomposite with a Chemically Bonded Interface for Enhanced Sunlight-Driven CO2 Photoreduction // ACS Applied Energy Materials. 2020. Vol. 3. No. 7. pp. 6422-6433.
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TY - JOUR
DO - 10.1021/acsaem.0c00656
UR - https://doi.org/10.1021/acsaem.0c00656
TI - Synthesis of the g-C3N4/CdS Nanocomposite with a Chemically Bonded Interface for Enhanced Sunlight-Driven CO2 Photoreduction
T2 - ACS Applied Energy Materials
AU - Vu, Nhu Nang
AU - Kaliaguine, S.
AU - Do, Trong-On
PY - 2020
DA - 2020/06/17 00:00:00
PB - American Chemical Society (ACS)
SP - 6422-6433
IS - 7
VL - 3
SN - 2574-0962
SN - 2574-0962
ER -
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@article{2020_Vu,
author = {Nhu Nang Vu and S. Kaliaguine and Trong-On Do},
title = {Synthesis of the g-C3N4/CdS Nanocomposite with a Chemically Bonded Interface for Enhanced Sunlight-Driven CO2 Photoreduction},
journal = {ACS Applied Energy Materials},
year = {2020},
volume = {3},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acsaem.0c00656},
number = {7},
pages = {6422--6433},
doi = {10.1021/acsaem.0c00656}
}
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MLA
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Vu, Nhu Nang, et al. “Synthesis of the g-C3N4/CdS Nanocomposite with a Chemically Bonded Interface for Enhanced Sunlight-Driven CO2 Photoreduction.” ACS Applied Energy Materials, vol. 3, no. 7, Jun. 2020, pp. 6422-6433. https://doi.org/10.1021/acsaem.0c00656.