Crystal Growth and Design, volume 17, issue 1, pages 214-220
Peroxosolvates: Formation criteria, H2O2 hydrogen bonding, and isomorphism with the corresponding hydrates
Publication type: Journal Article
Publication date: 2016-12-02
Journal:
Crystal Growth and Design
Quartile SCImago
Q2
Quartile WOS
Q1
Impact factor: 3.8
ISSN: 15287483, 15287505
General Chemistry
Condensed Matter Physics
General Materials Science
Abstract
The Cambridge Structural Database has been used to investigate the detailed environment of H2O2 molecules and hydrogen-bond patterns within “true” peroxosolvates in which the H2O2 molecules do not interact directly with the metal atoms. A study of 65 crystal structures and over 260 hydrogen bonds reveals that H2O2 always forms two H-bonds as proton donors and up to four H-bonds as a proton acceptor, but the latter can be absent altogether. The necessary features of peroxosolvate coformers are clarified. (1) Coformers should not participate in redox reactions with H2O2 and should not catalyze its decomposition. (2) Coformers should be Bronsted bases or exhibit amphoteric properties. The efficiency of the proposed criteria for peroxosolvate formation is illustrated by the synthesis and characterization of several new crystals. Conditions preventing the H2O2/H2O isomorphous substitution are essential for peroxosolvate stability: (1) Every H2O2 in the peroxosolvate has to participate in five or six hydrogen b...
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Chernyshov I. et al. Peroxosolvates: Formation criteria, H2O2 hydrogen bonding, and isomorphism with the corresponding hydrates // Crystal Growth and Design. 2016. Vol. 17. No. 1. pp. 214-220.
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Chernyshov I., Vener M. V., Prikhodchenko P. V., Medvedev A. G., Lev O., Churakov A. V. Peroxosolvates: Formation criteria, H2O2 hydrogen bonding, and isomorphism with the corresponding hydrates // Crystal Growth and Design. 2016. Vol. 17. No. 1. pp. 214-220.
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TY - JOUR
DO - 10.1021/acs.cgd.6b01449
UR - https://doi.org/10.1021%2Facs.cgd.6b01449
TI - Peroxosolvates: Formation criteria, H2O2 hydrogen bonding, and isomorphism with the corresponding hydrates
T2 - Crystal Growth and Design
AU - Vener, Mikhail V.
AU - Medvedev, Alexander G.
AU - Lev, Ovadia
AU - Chernyshov, Ivan
AU - Prikhodchenko, Petr V.
AU - Churakov, Andrei V.
PY - 2016
DA - 2016/12/02 00:00:00
PB - American Chemical Society (ACS)
SP - 214-220
IS - 1
VL - 17
SN - 1528-7483
SN - 1528-7505
ER -
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@article{2016_Chernyshov
author = {Mikhail V. Vener and Alexander G. Medvedev and Ovadia Lev and Ivan Chernyshov and Petr V. Prikhodchenko and Andrei V. Churakov},
title = {Peroxosolvates: Formation criteria, H2O2 hydrogen bonding, and isomorphism with the corresponding hydrates},
journal = {Crystal Growth and Design},
year = {2016},
volume = {17},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021%2Facs.cgd.6b01449},
number = {1},
pages = {214--220},
doi = {10.1021/acs.cgd.6b01449}
}
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MLA
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Chernyshov, Ivan, et al. “Peroxosolvates: Formation criteria, H2O2 hydrogen bonding, and isomorphism with the corresponding hydrates.” Crystal Growth and Design, vol. 17, no. 1, Dec. 2016, pp. 214-220. https://doi.org/10.1021%2Facs.cgd.6b01449.