Controlled Synthesis of Lead-Free and Stable Perovskite Derivative Cs2SnI6 Nanocrystals via a Facile Hot-Injection Process
Тип публикации: Journal Article
Дата публикации: 2016-11-07
SCImago Q1
Tоп 10% SCImago
WOS Q1
БС1
SJR: 1.796
CiteScore: 12
Impact factor: 7
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Краткое описание
Colloidal nanocrystals of lead halide perovskites have recently received great attention due to their remarkable performance in optoelectronic applications (e.g., light-emitting devices, flexible electronics, and photodetectors). However, the use of lead remains of great concern due to its toxicity and bioaccumulation in the ecosystem; herein we report a strategy to address this issue by using tetravalent tin (Sn4+) instead of divalent lead (Pb2+) to synthesize stable Cs2SnI6 perovskite nanocrystals. The shapes of as-synthesized Cs2SnI6 nanocrystals are tuned from spherical quantum dots, nanorods, nanowires, and nanobelts to nanoplatelets via a facile hot-injection process using inexpensive and nontoxic commercial precursors. Spherical aberration corrected scanning transmission electron microscopy (Cs-corrected STEM) and simulation studies revealed a well-defined face-centered-cubic (fcc) perovskite derivative structure of Cs2SnI6 nanocrystals. The solution-processed Cs2SnI6 nanocrystal-based field effect...
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Wang A. et al. Controlled Synthesis of Lead-Free and Stable Perovskite Derivative Cs2SnI6 Nanocrystals via a Facile Hot-Injection Process // Chemistry of Materials. 2016. Vol. 28. No. 22. pp. 8132-8140.
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Wang A., Yan X., Zhang M., Sun S., Yang M., Shen W., Pan X., Wang P., Deng Z. Controlled Synthesis of Lead-Free and Stable Perovskite Derivative Cs2SnI6 Nanocrystals via a Facile Hot-Injection Process // Chemistry of Materials. 2016. Vol. 28. No. 22. pp. 8132-8140.
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TY - JOUR
DO - 10.1021/acs.chemmater.6b01329
UR - https://doi.org/10.1021/acs.chemmater.6b01329
TI - Controlled Synthesis of Lead-Free and Stable Perovskite Derivative Cs2SnI6 Nanocrystals via a Facile Hot-Injection Process
T2 - Chemistry of Materials
AU - Wang, Aifei
AU - Yan, Xingxu
AU - Zhang, Mian
AU - Sun, Shibin
AU - Yang, Ming
AU - Shen, Wei
AU - Pan, Xiaoqing
AU - Wang, Peng
AU - Deng, Zhengtao
PY - 2016
DA - 2016/11/07
PB - American Chemical Society (ACS)
SP - 8132-8140
IS - 22
VL - 28
SN - 0897-4756
SN - 1520-5002
ER -
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@article{2016_Wang,
author = {Aifei Wang and Xingxu Yan and Mian Zhang and Shibin Sun and Ming Yang and Wei Shen and Xiaoqing Pan and Peng Wang and Zhengtao Deng},
title = {Controlled Synthesis of Lead-Free and Stable Perovskite Derivative Cs2SnI6 Nanocrystals via a Facile Hot-Injection Process},
journal = {Chemistry of Materials},
year = {2016},
volume = {28},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/acs.chemmater.6b01329},
number = {22},
pages = {8132--8140},
doi = {10.1021/acs.chemmater.6b01329}
}
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MLA
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Wang, Aifei, et al. “Controlled Synthesis of Lead-Free and Stable Perovskite Derivative Cs2SnI6 Nanocrystals via a Facile Hot-Injection Process.” Chemistry of Materials, vol. 28, no. 22, Nov. 2016, pp. 8132-8140. https://doi.org/10.1021/acs.chemmater.6b01329.
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