Chemistry of Materials, volume 28, issue 17, pages 6409-6416
Tuning Optical Activity of IV–VI Colloidal Quantum Dots in the Short-Wave Infrared (SWIR) Spectral Regime
Publication type: Journal Article
Publication date: 2016-08-23
Journal:
Chemistry of Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 8.6
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Abstract
The achievement of tunable optical properties across a wide spectral range, along with an efficient surface passivation of lead chalcogenide (PbSe) colloidal quantum dots (CQDs), has significant importance for scientific research and for technological applications. This paper describes two comprehensive pathways to tune optical activities of PbSe CQDs in the near-infrared (NIR, 0.75–1.4 μm) and the short-wave infrared (SWIR, 1.4–3 μm) ranges. A one-pot procedure enabled the growth of relatively large PbSe CQDs (with average sizes up to 14 nm) exploiting programmable temperature control during the growth process. These CQDs showed optical activity up to 3.2 μm. In addition, PbSe/PbS core/shell CQDs prepared by an orderly injection rate led to an energy red-shift of the absorption edge with the increase of the shell thickness, whereas a postannealing treatment further extended the band-edge energy toward the SWIR regime. A better chemical stability of the CQDs with respect to that of PbSe core CQDs was atta...
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SHAPIRO A. et al. Tuning Optical Activity of IV–VI Colloidal Quantum Dots in the Short-Wave Infrared (SWIR) Spectral Regime // Chemistry of Materials. 2016. Vol. 28. No. 17. pp. 6409-6416.
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SHAPIRO A., Jang Y., Rubin Brusilovski A., Budniak A. K., Horani F., Sashchiuk A., Lifshitz E. Tuning Optical Activity of IV–VI Colloidal Quantum Dots in the Short-Wave Infrared (SWIR) Spectral Regime // Chemistry of Materials. 2016. Vol. 28. No. 17. pp. 6409-6416.
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TY - JOUR
DO - 10.1021/acs.chemmater.6b02917
UR - https://doi.org/10.1021/acs.chemmater.6b02917
TI - Tuning Optical Activity of IV–VI Colloidal Quantum Dots in the Short-Wave Infrared (SWIR) Spectral Regime
T2 - Chemistry of Materials
AU - SHAPIRO, ARTHUR
AU - Jang, Youngjin
AU - Rubin Brusilovski, Anna
AU - Sashchiuk, Aldona
AU - Budniak, Adam K
AU - Horani, Faris
AU - Lifshitz, Efrat
PY - 2016
DA - 2016/08/23 00:00:00
PB - American Chemical Society (ACS)
SP - 6409-6416
IS - 17
VL - 28
SN - 0897-4756
SN - 1520-5002
ER -
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@article{2016_SHAPIRO,
author = {ARTHUR SHAPIRO and Youngjin Jang and Anna Rubin Brusilovski and Aldona Sashchiuk and Adam K Budniak and Faris Horani and Efrat Lifshitz},
title = {Tuning Optical Activity of IV–VI Colloidal Quantum Dots in the Short-Wave Infrared (SWIR) Spectral Regime},
journal = {Chemistry of Materials},
year = {2016},
volume = {28},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.chemmater.6b02917},
number = {17},
pages = {6409--6416},
doi = {10.1021/acs.chemmater.6b02917}
}
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SHAPIRO, ARTHUR, et al. “Tuning Optical Activity of IV–VI Colloidal Quantum Dots in the Short-Wave Infrared (SWIR) Spectral Regime.” Chemistry of Materials, vol. 28, no. 17, Aug. 2016, pp. 6409-6416. https://doi.org/10.1021/acs.chemmater.6b02917.