Mechanochromic Luminescence and Liquid Crystallinity of Molecular Copper Clusters
Brendan Huitorel
1
,
Quentin Benito
1
,
Alexandre Fargues
2
,
Alain Garcia
2
,
Thierry Gacoin
1
,
Jean-Pierre Boilot
1
,
1
Laboratoire
de Physique de la Matière Condensée (PMC), Ecole Polytechnique-CNRS, 91128 Palaiseau Cedex, France
|
2
Institut de Chimie de la Matière Condensée de Bordeaux (ICMCB)-CNRS, 87 Avenue du Docteur A. Schweitzer, 33608 Pessac Cedex, France
|
Тип публикации: Journal Article
Дата публикации: 2016-11-07
scimago Q1
wos Q1
БС1
SJR: 2.065
CiteScore: 12.0
Impact factor: 7.0
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Краткое описание
Molecular copper iodide clusters with the [Cu4I4] cubane core have been functionalized by phosphine ligands carrying protomesogenic gallate-based derivatives bearing either long alkyl chains (C8, C12, and C16) or cyanobiphenyl (CBP) fragments. The mesomorphic properties of the functionalized clusters were studied by combining differential scanning calorimetry (DSC), polarized optical microscopy (POM), and small-angle X-ray scattering (SAXS) experiments. Whereas clusters functionalized solely with long alkyl chains present amorphous or crystalline states, the cluster carrying CBP fragments displays liquid crystal properties with the formation of a smectic A mesophase from room temperature up to 100 °C. Temperature-dependent photoluminescence measurements show that the CBP derivative displays an unusual luminescence thermochromism which is possibly due to a resonance energy transfer mechanism between the emissive [Cu4I4] inorganic and CBP moieties. The emission properties of this original cluster are also s...
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Huitorel B. et al. Mechanochromic Luminescence and Liquid Crystallinity of Molecular Copper Clusters // Chemistry of Materials. 2016. Vol. 28. No. 22. pp. 8190-8200.
ГОСТ со всеми авторами (до 50)
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Huitorel B., Benito Q., Fargues A., Garcia A., Gacoin T., Boilot J., Perruchas S., Camerel F. Mechanochromic Luminescence and Liquid Crystallinity of Molecular Copper Clusters // Chemistry of Materials. 2016. Vol. 28. No. 22. pp. 8190-8200.
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TY - JOUR
DO - 10.1021/acs.chemmater.6b03002
UR - https://doi.org/10.1021/acs.chemmater.6b03002
TI - Mechanochromic Luminescence and Liquid Crystallinity of Molecular Copper Clusters
T2 - Chemistry of Materials
AU - Huitorel, Brendan
AU - Benito, Quentin
AU - Fargues, Alexandre
AU - Garcia, Alain
AU - Gacoin, Thierry
AU - Boilot, Jean-Pierre
AU - Perruchas, Sandrine
AU - Camerel, Franck
PY - 2016
DA - 2016/11/07
PB - American Chemical Society (ACS)
SP - 8190-8200
IS - 22
VL - 28
SN - 0897-4756
SN - 1520-5002
ER -
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@article{2016_Huitorel,
author = {Brendan Huitorel and Quentin Benito and Alexandre Fargues and Alain Garcia and Thierry Gacoin and Jean-Pierre Boilot and Sandrine Perruchas and Franck Camerel},
title = {Mechanochromic Luminescence and Liquid Crystallinity of Molecular Copper Clusters},
journal = {Chemistry of Materials},
year = {2016},
volume = {28},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/acs.chemmater.6b03002},
number = {22},
pages = {8190--8200},
doi = {10.1021/acs.chemmater.6b03002}
}
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MLA
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Huitorel, Brendan, et al. “Mechanochromic Luminescence and Liquid Crystallinity of Molecular Copper Clusters.” Chemistry of Materials, vol. 28, no. 22, Nov. 2016, pp. 8190-8200. https://doi.org/10.1021/acs.chemmater.6b03002.