A Facile Method for Synthesizing Dendritic Core–Shell Structured Ternary Metallic Aerogels and Their Enhanced Electrochemical Performances
Qiurong Shi
1
,
Chengzhou Zhu
1
,
Yijing Li
2
,
Haibing Xia
2
,
Mark Engelhard
3
,
Shaofang Fu
1
,
Dan Du
1
,
Yan Xu
1
Publication type: Journal Article
Publication date: 2016-10-21
scimago Q1
wos Q1
SJR: 2.065
CiteScore: 12.0
Impact factor: 7.0
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Abstract
Currently, three-dimensional self-supported metallic structures are attractive for their unique properties of high porosity, low density, excellent conductivity, etc., that promote their wide application in fuel cells. Here, for the first time, we report a facile synthesis of Au@Pt3Pd ternary metallic aerogels with a unique dendritic core–shell structure via a one-pot self-assembly gelation strategy. This strategy is simple and saves time without any concentration or destabilizer steps. The as-prepared Au@Pt3Pd ternary metallic aerogels demonstrated enhanced electrochemical performance toward the oxygen reduction reaction compared to that of commercial Pt/C. The unique dendritic core–shell structures, Pt3Pd alloyed shells, and cross-linked network structures are beneficial for the electrochemical oxygen reduction reaction via the electronic effect, geometric effect, and synergistic effect. This strategy of fabrication of metallic hydrogels and aerogels as well as their exceptional properties holds great p...
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Metrics
64
Total citations:
64
Citations from 2024:
5
(7.81%)
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MLA
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GOST
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Shi Q. et al. A Facile Method for Synthesizing Dendritic Core–Shell Structured Ternary Metallic Aerogels and Their Enhanced Electrochemical Performances // Chemistry of Materials. 2016. Vol. 28. No. 21. pp. 7928-7934.
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Shi Q., Zhu C., Li Y., Xia H., Engelhard M., Fu S., Du D., Xu Y. A Facile Method for Synthesizing Dendritic Core–Shell Structured Ternary Metallic Aerogels and Their Enhanced Electrochemical Performances // Chemistry of Materials. 2016. Vol. 28. No. 21. pp. 7928-7934.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.chemmater.6b03549
UR - https://doi.org/10.1021/acs.chemmater.6b03549
TI - A Facile Method for Synthesizing Dendritic Core–Shell Structured Ternary Metallic Aerogels and Their Enhanced Electrochemical Performances
T2 - Chemistry of Materials
AU - Shi, Qiurong
AU - Zhu, Chengzhou
AU - Li, Yijing
AU - Xia, Haibing
AU - Engelhard, Mark
AU - Fu, Shaofang
AU - Du, Dan
AU - Xu, Yan
PY - 2016
DA - 2016/10/21
PB - American Chemical Society (ACS)
SP - 7928-7934
IS - 21
VL - 28
SN - 0897-4756
SN - 1520-5002
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2016_Shi,
author = {Qiurong Shi and Chengzhou Zhu and Yijing Li and Haibing Xia and Mark Engelhard and Shaofang Fu and Dan Du and Yan Xu},
title = {A Facile Method for Synthesizing Dendritic Core–Shell Structured Ternary Metallic Aerogels and Their Enhanced Electrochemical Performances},
journal = {Chemistry of Materials},
year = {2016},
volume = {28},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/acs.chemmater.6b03549},
number = {21},
pages = {7928--7934},
doi = {10.1021/acs.chemmater.6b03549}
}
Cite this
MLA
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Shi, Qiurong, et al. “A Facile Method for Synthesizing Dendritic Core–Shell Structured Ternary Metallic Aerogels and Their Enhanced Electrochemical Performances.” Chemistry of Materials, vol. 28, no. 21, Oct. 2016, pp. 7928-7934. https://doi.org/10.1021/acs.chemmater.6b03549.