Chemistry of Materials, volume 29, issue 4, pages 1769-1778

Dual Substitution Strategy to Enhance Li⁺ Ionic Conductivity in Li₇La₃Zr₂O₁₂ Solid Electrolyte

Lucienne Buannic ¹

Brahim Orayech ¹

Juan Miguel López del Amo ¹

Javier Carrasco ¹

Nebil A. Katcho ¹

Frederic Aguesse ¹

William Wang Manalastas ¹

Wei Zhang ^{1, 2}

John Kilner ^{1, 3}

Anna Llordes ^{1, 2}

Hide authors affiliations Show authors affiliations: 3 affiliations

CIC EnergiGUNE, Parque Tecnológico de Álava, 48, 01510 Miñano, Álava, Spain |

Ikerbasque, The Basque Foundation for Science, 48013 Bilbao, Spain |

Department of Materials, Imperial College, London SW7 2AZ, United Kingdom |

Publication type: Journal Article

Publication date: 2017-02-10

American Chemical Society (ACS)

Journal: Chemistry of Materials

Quartile SCImago

Quartile WOS

Impact factor: 8.6

ISSN: 08974756, 15205002

DOI: 10.1021/acs.chemmater.6b05369

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Materials Chemistry

General Chemistry

General Chemical Engineering

Abstract

Solid state electrolytes could address the current safety concerns of lithium-ion batteries as well as provide higher electrochemical stability and energy density. Among solid electrolyte contenders, garnet-structured Li7La3Zr2O12 appears as a particularly promising material owing to its wide electrochemical stability window; however, its ionic conductivity remains an order of magnitude below that of ubiquitous liquid electrolytes. Here, we present an innovative dual substitution strategy developed to enhance Li-ion mobility in garnet-structured solid electrolytes. A first dopant cation, Ga3+, is introduced on the Li sites to stabilize the fast-conducting cubic phase. Simultaneously, a second cation, Sc3+, is used to partially populate the Zr sites, which consequently increases the concentration of Li ions by charge compensation. This aliovalent dual substitution strategy allows fine-tuning of the number of charge carriers in the cubic Li7La3Zr2O12 according to the resulting stoichiometry, Li7–3x+yGaxLa3Z...

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Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 3, 1.75% Physical Chemistry Chemical Physics 3 publications, 1.75%
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Citations by publishers

	10 20 30 40 50 60
Elsevier	Elsevier, 56, 32.75% Elsevier 56 publications, 32.75%
American Chemical Society (ACS)	American Chemical Society (ACS), 27, 15.79% American Chemical Society (ACS) 27 publications, 15.79%
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IOP Publishing	IOP Publishing, 2, 1.17% IOP Publishing 2 publications, 1.17%
World Scientific	World Scientific, 1, 0.58% World Scientific 1 publication, 0.58%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.58% Frontiers Media S.A. 1 publication, 0.58%
Tsinghua University Press	Tsinghua University Press, 1, 0.58% Tsinghua University Press 1 publication, 0.58%
Chinese Ceramic Society	Chinese Ceramic Society, 1, 0.58% Chinese Ceramic Society 1 publication, 0.58%
Taylor & Francis	Taylor & Francis, 1, 0.58% Taylor & Francis 1 publication, 0.58%
Shanghai Institute of Ceramics	Shanghai Institute of Ceramics, 1, 0.58% Shanghai Institute of Ceramics 1 publication, 0.58%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.58% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.58%
	10 20 30 40 50 60

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Buannic L. et al. Dual Substitution Strategy to Enhance Li+ Ionic Conductivity in Li7La3Zr2O12 Solid Electrolyte // Chemistry of Materials. 2017. Vol. 29. No. 4. pp. 1769-1778.

GOST all authors (up to 50) Copy

Buannic L., Orayech B., López del Amo J. M., Carrasco J., Katcho N. A., Aguesse F., Manalastas W. W., Zhang W., Kilner J., Llordes A. Dual Substitution Strategy to Enhance Li+ Ionic Conductivity in Li7La3Zr2O12 Solid Electrolyte // Chemistry of Materials. 2017. Vol. 29. No. 4. pp. 1769-1778.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acs.chemmater.6b05369

UR - https://doi.org/10.1021/acs.chemmater.6b05369

TI - Dual Substitution Strategy to Enhance Li+ Ionic Conductivity in Li7La3Zr2O12 Solid Electrolyte

T2 - Chemistry of Materials

AU - Buannic, Lucienne

AU - Carrasco, Javier

AU - Aguesse, Frederic

AU - Llordes, Anna

AU - Orayech, Brahim

AU - López del Amo, Juan Miguel

AU - Katcho, Nebil A.

AU - Manalastas, William Wang

AU - Zhang, Wei

AU - Kilner, John

PY - 2017

DA - 2017/02/10 00:00:00

PB - American Chemical Society (ACS)

SP - 1769-1778

IS - 4

VL - 29

SN - 0897-4756

SN - 1520-5002

ER -

BibTex |

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BibTex Copy

@article{2017_Buannic,

author = {Lucienne Buannic and Javier Carrasco and Frederic Aguesse and Anna Llordes and Brahim Orayech and Juan Miguel López del Amo and Nebil A. Katcho and William Wang Manalastas and Wei Zhang and John Kilner},

title = {Dual Substitution Strategy to Enhance Li+ Ionic Conductivity in Li7La3Zr2O12 Solid Electrolyte},

journal = {Chemistry of Materials},

year = {2017},

volume = {29},

publisher = {American Chemical Society (ACS)},

month = {feb},

url = {https://doi.org/10.1021/acs.chemmater.6b05369},

number = {4},

pages = {1769--1778},

doi = {10.1021/acs.chemmater.6b05369}

}

MLA

Cite this

MLA Copy

Buannic, Lucienne, et al. “Dual Substitution Strategy to Enhance Li+ Ionic Conductivity in Li7La3Zr2O12 Solid Electrolyte.” Chemistry of Materials, vol. 29, no. 4, Feb. 2017, pp. 1769-1778. https://doi.org/10.1021/acs.chemmater.6b05369.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Chemistry of Materials

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Quartile WOS

Impact factor

8.6

ISSN

08974756 (Print)
15205002 (Electronic)