Chemistry of Materials, volume 31, issue 3, pages 759-773
Lanthanide Complexes with 2-(Tosylamino)-benzylidene-N-(aryloyl)hydrazones: Universal Luminescent Materials
Kovalenko Anton
1, 2
,
Rublev Pavel O
1
,
Tcelykh L
1
,
Lepnev Leonid S.
4
,
Burlov A.S
5
,
Vashchenko A A
4
,
Marciniak Lukasz
6
,
Magerramov Abel M
7
,
Shikhaliyev Namig G.
7
,
2
Centre de Biophysique Moléculaire—UPR 4301, Center National De La Recherche Scientifique, Rue Charles Sadron, Orléans 45071, France
|
6
Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P Nr 1410, 50-950 Wrocław 2, Poland
|
8
SIA Evoled, 1a-24 Puskina iela, LV-1050 Riga, Latvia
|
Publication type: Journal Article
Publication date: 2019-01-04
Journal:
Chemistry of Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 8.6
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Abstract
Lanthanide complexes Ln(L1)(HL1) (Ln = Lu, Yb, Er, Gd, Eu, Sm) and Ln(L2)(HL2) (Ln = Lu, Yb, Gd, Eu) with 2-(tosylamino)-benzylidene-N-(aryloyl)hydrazones (H2L1, aryloyl = 2-hydroxybenzoyl; H2L2, aryloyl = isonicotinoyl) were obtained with the aim to explore them as new luminescent materials. They were found to form monomeric species independently on the aryloyl group, and their crystal structures were determined from single-crystal X-ray data (Yb(L2)(HL2)·0.5(C2H5OH)), as well as from powder X-ray data by Rietveld refinement (Eu(L1)(HL1)). Ytterbium complexes exhibited intense luminescence, which allowed using them in host-free organic light-emitting diodes, which demonstrated remarkable efficiency of near infrared electroluminescence (50 μW/W) at low voltage (5 V). The special mechanism of europium luminescence quenching allowed using europium complexes as luminescent thermometers, which demonstrated very high sensitivity up to 12%/K. The theory of luminescence thermometry based on a three-level system ...
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Kovalenko A. et al. Lanthanide Complexes with 2-(Tosylamino)-benzylidene-N-(aryloyl)hydrazones: Universal Luminescent Materials // Chemistry of Materials. 2019. Vol. 31. No. 3. pp. 759-773.
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Kovalenko A., Rublev P. O., Tcelykh L., Goloveshkin A. S., Lepnev L. S., Burlov A., Vashchenko A. A., Marciniak L., Magerramov A. M., Shikhaliyev N. G., Vatsadze S. Z., Utochnikova V. Lanthanide Complexes with 2-(Tosylamino)-benzylidene-N-(aryloyl)hydrazones: Universal Luminescent Materials // Chemistry of Materials. 2019. Vol. 31. No. 3. pp. 759-773.
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TY - JOUR
DO - 10.1021/acs.chemmater.8b03675
UR - https://doi.org/10.1021%2Facs.chemmater.8b03675
TI - Lanthanide Complexes with 2-(Tosylamino)-benzylidene-N-(aryloyl)hydrazones: Universal Luminescent Materials
T2 - Chemistry of Materials
AU - Rublev, Pavel O
AU - Lepnev, Leonid S.
AU - Shikhaliyev, Namig G.
AU - Magerramov, Abel M
AU - Kovalenko, Anton
AU - Marciniak, Lukasz
AU - Vatsadze, Sergey Z.
AU - Utochnikova, Valentina
AU - Tcelykh, L
AU - Goloveshkin, Alexander S.
AU - Burlov, A.S
AU - Vashchenko, A A
PY - 2019
DA - 2019/01/04 00:00:00
PB - American Chemical Society (ACS)
SP - 759-773
IS - 3
VL - 31
SN - 0897-4756
SN - 1520-5002
ER -
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@article{2019_Kovalenko,
author = {Pavel O Rublev and Leonid S. Lepnev and Namig G. Shikhaliyev and Abel M Magerramov and Anton Kovalenko and Lukasz Marciniak and Sergey Z. Vatsadze and Valentina Utochnikova and L Tcelykh and Alexander S. Goloveshkin and A.S Burlov and A A Vashchenko},
title = {Lanthanide Complexes with 2-(Tosylamino)-benzylidene-N-(aryloyl)hydrazones: Universal Luminescent Materials},
journal = {Chemistry of Materials},
year = {2019},
volume = {31},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021%2Facs.chemmater.8b03675},
number = {3},
pages = {759--773},
doi = {10.1021/acs.chemmater.8b03675}
}
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Kovalenko, Anton, et al. “Lanthanide Complexes with 2-(Tosylamino)-benzylidene-N-(aryloyl)hydrazones: Universal Luminescent Materials.” Chemistry of Materials, vol. 31, no. 3, Jan. 2019, pp. 759-773. https://doi.org/10.1021%2Facs.chemmater.8b03675.