Chemical Reviews, volume 120, issue 10, pages 4257-4300

Garnet-Type Solid-State Electrolytes: Materials, Interfaces, and Batteries

Chengwei Wang ¹

Kun Fu ^{1, 2}

Sanoop Palakkathodi Kammampata ³

Dennis W. McOwen ^{1, 4}

Alfred Junio Samson ³

Lei Zhang ^{1, 4}

Gregory T. Hitz ^{1, 4}

Adelaide M Nolan ¹

Eric D. Wachsman ^{1, 4}

Yifei Mo ¹

Venkataraman Thangadurai ³

Liangbing Hu ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742, United States |

Department of Mechanical Engineering, University of Delaware, Newark, Delaware 19716, United States |

Department of Chemistry, University of Calgary, 2500 University Drive Northwest, Calgary T2N 1N4, Canada |

⁴

Maryland Energy Innovation Institute, University of Maryland, College Park, Maryland 20742, United States |

Publication type: Journal Article

Publication date: 2020-04-09

American Chemical Society (ACS)

Journal: Chemical Reviews

Quartile SCImago

Quartile WOS

Impact factor: 62.1

ISSN: 00092665, 15206890

DOI: 10.1021/acs.chemrev.9b00427

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General Chemistry

Abstract

Solid-state batteries with desirable advantages, including high-energy density, wide temperature tolerance, and fewer safety-concerns, have been considered as a promising energy storage technology to replace organic liquid electrolyte-dominated Li-ion batteries. Solid-state electrolytes (SSEs) as the most critical component in solid-state batteries largely lead the future battery development. Among different types of solid-state electrolytes, garnet-type Li7La3Zr2O12 (LLZO) solid-state electrolytes have particularly high ionic conductivity (10-3 to 10-4 S/cm) and good chemical stability against Li metal, offering a great opportunity for solid-state Li-metal batteries. Since the discovery of garnet-type LLZO in 2007, there has been an increasing interest in the development of garnet-type solid-state electrolytes and all solid-state batteries. Garnet-type electrolyte has been considered one of the most promising and important solid-state electrolytes for batteries with potential benefits in energy density, electrochemical stability, high temperature stability, and safety. In this Review, we will survey recent development of garnet-type LLZO electrolytes with discussions of experimental studies and theoretical results in parallel, LLZO electrolyte synthesis strategies and modifications, stability of garnet solid electrolytes/electrodes, emerging nanostructure designs, degradation mechanisms and mitigations, and battery architectures and integrations. We will also provide a target-oriented research overview of garnet-type LLZO electrolyte and its application in various types of solid-state battery concepts (e.g., Li-ion, Li-S, and Li-air), and we will show opportunities and perspectives as guides for future development of solid electrolytes and solid-state batteries.

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Citations by journals

	5 10 15 20 25 30 35 40 45 50
ACS applied materials & interfaces	ACS applied materials & interfaces, 46, 6.35% ACS applied materials & interfaces 46 publications, 6.35%
Advanced Functional Materials	Advanced Functional Materials, 32, 4.42% Advanced Functional Materials 32 publications, 4.42%
Energy Storage Materials	Energy Storage Materials, 30, 4.14% Energy Storage Materials 30 publications, 4.14%
Journal of Power Sources	Journal of Power Sources, 25, 3.45% Journal of Power Sources 25 publications, 3.45%
Advanced Energy Materials	Advanced Energy Materials, 24, 3.31% Advanced Energy Materials 24 publications, 3.31%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 24, 3.31% Journal of Materials Chemistry A 24 publications, 3.31%
Chemical Engineering Journal	Chemical Engineering Journal, 23, 3.18% Chemical Engineering Journal 23 publications, 3.18%
Small	Small, 21, 2.9% Small 21 publications, 2.9%
ACS Applied Energy Materials	ACS Applied Energy Materials, 18, 2.49% ACS Applied Energy Materials 18 publications, 2.49%
ACS Energy Letters	ACS Energy Letters, 15, 2.07% ACS Energy Letters 15 publications, 2.07%
Advanced Materials	Advanced Materials, 15, 2.07% Advanced Materials 15 publications, 2.07%
Journal of Energy Storage	Journal of Energy Storage, 14, 1.93% Journal of Energy Storage 14 publications, 1.93%
Ceramics International	Ceramics International, 13, 1.8% Ceramics International 13 publications, 1.8%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 11, 1.52% Journal of Alloys and Compounds 11 publications, 1.52%
Batteries	Batteries, 10, 1.38% Batteries 10 publications, 1.38%
Ionics	Ionics, 10, 1.38% Ionics 10 publications, 1.38%
Journal of Energy Chemistry	Journal of Energy Chemistry, 10, 1.38% Journal of Energy Chemistry 10 publications, 1.38%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 9, 1.24% Journal of Physical Chemistry C 9 publications, 1.24%
Energy and Environmental Science	Energy and Environmental Science, 9, 1.24% Energy and Environmental Science 9 publications, 1.24%
Journal of the European Ceramic Society	Journal of the European Ceramic Society, 8, 1.1% Journal of the European Ceramic Society 8 publications, 1.1%
Advanced Science	Advanced Science, 7, 0.97% Advanced Science 7 publications, 0.97%
Solid State Ionics	Solid State Ionics, 7, 0.97% Solid State Ionics 7 publications, 0.97%
Nano Energy	Nano Energy, 7, 0.97% Nano Energy 7 publications, 0.97%
Electrochimica Acta	Electrochimica Acta, 7, 0.97% Electrochimica Acta 7 publications, 0.97%
Nano Letters	Nano Letters, 7, 0.97% Nano Letters 7 publications, 0.97%
Batteries & Supercaps	Batteries & Supercaps, 6, 0.83% Batteries & Supercaps 6 publications, 0.83%
Nature Communications	Nature Communications, 6, 0.83% Nature Communications 6 publications, 0.83%
Materials Today Energy	Materials Today Energy, 6, 0.83% Materials Today Energy 6 publications, 0.83%
Small Methods	Small Methods, 6, 0.83% Small Methods 6 publications, 0.83%
	5 10 15 20 25 30 35 40 45 50

Citations by publishers

	50 100 150 200 250
Elsevier	Elsevier, 231, 31.91% Elsevier 231 publications, 31.91%
Wiley	Wiley, 169, 23.34% Wiley 169 publications, 23.34%
American Chemical Society (ACS)	American Chemical Society (ACS), 127, 17.54% American Chemical Society (ACS) 127 publications, 17.54%
Springer Nature	Springer Nature, 56, 7.73% Springer Nature 56 publications, 7.73%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 51, 7.04% Royal Society of Chemistry (RSC) 51 publications, 7.04%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 32, 4.42% Multidisciplinary Digital Publishing Institute (MDPI) 32 publications, 4.42%
The Electrochemical Society	The Electrochemical Society, 5, 0.69% The Electrochemical Society 5 publications, 0.69%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 4, 0.55% American Institute of Physics (AIP) 4 publications, 0.55%
IOP Publishing	IOP Publishing, 4, 0.55% IOP Publishing 4 publications, 0.55%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 4, 0.55% American Association for the Advancement of Science (AAAS) 4 publications, 0.55%
Chinese Physical Society	Chinese Physical Society, 4, 0.55% Chinese Physical Society 4 publications, 0.55%
Frontiers Media S.A.	Frontiers Media S.A., 3, 0.41% Frontiers Media S.A. 3 publications, 0.41%
Cambridge University Press	Cambridge University Press, 3, 0.41% Cambridge University Press 3 publications, 0.41%
Oxford University Press	Oxford University Press, 3, 0.41% Oxford University Press 3 publications, 0.41%
International Union of Crystallography (IUCr)	International Union of Crystallography (IUCr), 2, 0.28% International Union of Crystallography (IUCr) 2 publications, 0.28%
World Scientific	World Scientific, 2, 0.28% World Scientific 2 publications, 0.28%
Tsinghua University Press	Tsinghua University Press, 2, 0.28% Tsinghua University Press 2 publications, 0.28%
Taylor & Francis	Taylor & Francis, 2, 0.28% Taylor & Francis 2 publications, 0.28%
Annual Reviews	Annual Reviews, 2, 0.28% Annual Reviews 2 publications, 0.28%
Pleiades Publishing	Pleiades Publishing, 2, 0.28% Pleiades Publishing 2 publications, 0.28%
Hindawi Limited	Hindawi Limited, 2, 0.28% Hindawi Limited 2 publications, 0.28%
ASME	ASME, 1, 0.14% ASME 1 publication, 0.14%
American Vacuum Society	American Vacuum Society, 1, 0.14% American Vacuum Society 1 publication, 0.14%
Canadian Science Publishing	Canadian Science Publishing, 1, 0.14% Canadian Science Publishing 1 publication, 0.14%
Higher Education Press	Higher Education Press, 1, 0.14% Higher Education Press 1 publication, 0.14%
University of Science and Technology Beijing	University of Science and Technology Beijing, 1, 0.14% University of Science and Technology Beijing 1 publication, 0.14%
American Physical Society (APS)	American Physical Society (APS), 1, 0.14% American Physical Society (APS) 1 publication, 0.14%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.14% Nonferrous Metals Society of China 1 publication, 0.14%
SAE International	SAE International, 1, 0.14% SAE International 1 publication, 0.14%
	50 100 150 200 250

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Wang C. et al. Garnet-Type Solid-State Electrolytes: Materials, Interfaces, and Batteries // Chemical Reviews. 2020. Vol. 120. No. 10. pp. 4257-4300.

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Wang C., Fu K., Kammampata S. P., McOwen D. W., Samson A. J., Zhang L., Hitz G. T., Nolan A. M., Wachsman E. D., Mo Y., Thangadurai V., Hu L. Garnet-Type Solid-State Electrolytes: Materials, Interfaces, and Batteries // Chemical Reviews. 2020. Vol. 120. No. 10. pp. 4257-4300.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acs.chemrev.9b00427

UR - https://doi.org/10.1021/acs.chemrev.9b00427

TI - Garnet-Type Solid-State Electrolytes: Materials, Interfaces, and Batteries

T2 - Chemical Reviews

AU - Kammampata, Sanoop Palakkathodi

AU - Samson, Alfred Junio

AU - Hitz, Gregory T.

AU - Fu, Kun

AU - Wachsman, Eric D.

AU - Mo, Yifei

AU - Thangadurai, Venkataraman

AU - Hu, Liangbing

AU - Wang, Chengwei

AU - McOwen, Dennis W.

AU - Zhang, Lei

AU - Nolan, Adelaide M

PY - 2020

DA - 2020/04/09 00:00:00

PB - American Chemical Society (ACS)

SP - 4257-4300

IS - 10

VL - 120

SN - 0009-2665

SN - 1520-6890

ER -

BibTex |

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BibTex Copy

@article{2020_Wang,

author = {Sanoop Palakkathodi Kammampata and Alfred Junio Samson and Gregory T. Hitz and Kun Fu and Eric D. Wachsman and Yifei Mo and Venkataraman Thangadurai and Liangbing Hu and Chengwei Wang and Dennis W. McOwen and Lei Zhang and Adelaide M Nolan},

title = {Garnet-Type Solid-State Electrolytes: Materials, Interfaces, and Batteries},

journal = {Chemical Reviews},

year = {2020},

volume = {120},

publisher = {American Chemical Society (ACS)},

month = {apr},

url = {https://doi.org/10.1021/acs.chemrev.9b00427},

number = {10},

pages = {4257--4300},

doi = {10.1021/acs.chemrev.9b00427}

}

MLA

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MLA Copy

Wang, Chengwei, et al. “Garnet-Type Solid-State Electrolytes: Materials, Interfaces, and Batteries.” Chemical Reviews, vol. 120, no. 10, Apr. 2020, pp. 4257-4300. https://doi.org/10.1021/acs.chemrev.9b00427.

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Publisher

American Chemical Society (ACS)

Journal

Chemical Reviews

Quartile SCImago

Quartile WOS

Impact factor

62.1

ISSN

00092665 (Print)
15206890 (Electronic)

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