Oxidation Behavior and Kinetics of Light, Medium, and Heavy Crude Oils Characterized by Thermogravimetry Coupled with Fourier Transform Infrared Spectroscopy
Тип публикации: Journal Article
Дата публикации: 2018-03-26
scimago Q1
wos Q1
БС1
SJR: 1.124
CiteScore: 9.5
Impact factor: 5.3
ISSN: 08870624, 15205029
General Chemical Engineering
Energy Engineering and Power Technology
Fuel Technology
Краткое описание
The oxidation behavior of three crude oils was characterized by thermogravimetry coupled with Fourier transform infrared spectroscopy (TG–FTIR) to investigate the oxidation mechanism of crude oils. The results indicated that the entire oxidation process can be divided into three main reaction intervals: low-temperature oxidation (LTO) interval (<400 °C), coking process (400–500 °C), and high-temperature oxidation (HTO) interval (500–650 °C). For the LTO interval, oxygen addition reactions to produce hydroperoxides were believed to be dominant at the early stage, while the isomerization and decomposition reactions of hydroperoxides became more significant at the later stage. For light and medium oils, the isomerization and decomposition reactions that release H2O started at about 200 °C and the isomerization and decomposition reactions that release CO2 and CO started at about 300 °C. However, no CO2 and CO were detected in the LTO interval of the heavy oil, which means that the reaction pathways of the hea...
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Yuan C., Emelianov D. A., Varfolomeev M. A. Oxidation Behavior and Kinetics of Light, Medium, and Heavy Crude Oils Characterized by Thermogravimetry Coupled with Fourier Transform Infrared Spectroscopy // Energy & Fuels. 2018. Vol. 32. No. 4. pp. 5571-5580.
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Yuan C., Emelianov D. A., Varfolomeev M. A. Oxidation Behavior and Kinetics of Light, Medium, and Heavy Crude Oils Characterized by Thermogravimetry Coupled with Fourier Transform Infrared Spectroscopy // Energy & Fuels. 2018. Vol. 32. No. 4. pp. 5571-5580.
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TY - JOUR
DO - 10.1021/acs.energyfuels.8b00428
UR - https://doi.org/10.1021/acs.energyfuels.8b00428
TI - Oxidation Behavior and Kinetics of Light, Medium, and Heavy Crude Oils Characterized by Thermogravimetry Coupled with Fourier Transform Infrared Spectroscopy
T2 - Energy & Fuels
AU - Yuan, Chengdong
AU - Emelianov, Dmitrii A
AU - Varfolomeev, Mikhail A.
PY - 2018
DA - 2018/03/26
PB - American Chemical Society (ACS)
SP - 5571-5580
IS - 4
VL - 32
SN - 0887-0624
SN - 1520-5029
ER -
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@article{2018_Yuan,
author = {Chengdong Yuan and Dmitrii A Emelianov and Mikhail A. Varfolomeev},
title = {Oxidation Behavior and Kinetics of Light, Medium, and Heavy Crude Oils Characterized by Thermogravimetry Coupled with Fourier Transform Infrared Spectroscopy},
journal = {Energy & Fuels},
year = {2018},
volume = {32},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/acs.energyfuels.8b00428},
number = {4},
pages = {5571--5580},
doi = {10.1021/acs.energyfuels.8b00428}
}
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Yuan, Chengdong, et al. “Oxidation Behavior and Kinetics of Light, Medium, and Heavy Crude Oils Characterized by Thermogravimetry Coupled with Fourier Transform Infrared Spectroscopy.” Energy & Fuels, vol. 32, no. 4, Mar. 2018, pp. 5571-5580. https://doi.org/10.1021/acs.energyfuels.8b00428.