Conversion of Isobutanol to Olefins and Aromatics over HZSM-5-Based Catalysts: Tuning of Product Selectivity
Тип публикации: Journal Article
Дата публикации: 2019-09-20
scimago Q1
wos Q1
БС1
SJR: 1.124
CiteScore: 9.5
Impact factor: 5.3
ISSN: 08870624, 15205029
General Chemical Engineering
Energy Engineering and Power Technology
Fuel Technology
Краткое описание
Isobutanol derived from biomass can serve as a potential renewable candidate for the production of light olefins and aromatics, which are the building blocks to manufacture fuels and chemicals in the petrochemical industry. Dependent upon the product requirements, the product selectivity toward olefins or aromatics can be tuned by adjusting the reaction conditions and the properties of HZSM-5 catalysts. On bare HZSM-5, mild conditions (low temperature, low space time, and low acidity) favored the production of olefins and harsh conditions (high temperature, high space time, and high acidity) were more likely to produce aromatics. Ga was impregnated onto HZSM-5 to enhance the production of aromatics. Unexpectedly, Ga introduction only induced the intertransformation between olefins and aromatics without significantly impacting the selectivity of low-value paraffins. The exchanged Ga sites functioning together with Bronsted acid were identified as active Ga species and strengthened the direct dehydrogenatio...
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Du Z. Y. et al. Conversion of Isobutanol to Olefins and Aromatics over HZSM-5-Based Catalysts: Tuning of Product Selectivity // Energy & Fuels. 2019. Vol. 33. No. 10. pp. 10176-10184.
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Du Z. Y., Zhang B., Chen T. S., Betancur Y., Li W. Conversion of Isobutanol to Olefins and Aromatics over HZSM-5-Based Catalysts: Tuning of Product Selectivity // Energy & Fuels. 2019. Vol. 33. No. 10. pp. 10176-10184.
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TY - JOUR
DO - 10.1021/acs.energyfuels.9b02454
UR - https://doi.org/10.1021/acs.energyfuels.9b02454
TI - Conversion of Isobutanol to Olefins and Aromatics over HZSM-5-Based Catalysts: Tuning of Product Selectivity
T2 - Energy & Fuels
AU - Du, Zhen Yi
AU - Zhang, Bin-Bin
AU - Chen, Ting Sheng
AU - Betancur, Yuli
AU - Li, Wen-ying
PY - 2019
DA - 2019/09/20
PB - American Chemical Society (ACS)
SP - 10176-10184
IS - 10
VL - 33
SN - 0887-0624
SN - 1520-5029
ER -
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@article{2019_Du,
author = {Zhen Yi Du and Bin-Bin Zhang and Ting Sheng Chen and Yuli Betancur and Wen-ying Li},
title = {Conversion of Isobutanol to Olefins and Aromatics over HZSM-5-Based Catalysts: Tuning of Product Selectivity},
journal = {Energy & Fuels},
year = {2019},
volume = {33},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/acs.energyfuels.9b02454},
number = {10},
pages = {10176--10184},
doi = {10.1021/acs.energyfuels.9b02454}
}
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MLA
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Du, Zhen Yi, et al. “Conversion of Isobutanol to Olefins and Aromatics over HZSM-5-Based Catalysts: Tuning of Product Selectivity.” Energy & Fuels, vol. 33, no. 10, Sep. 2019, pp. 10176-10184. https://doi.org/10.1021/acs.energyfuels.9b02454.