Core/Shell Ruthenium–Halloysite Nanocatalysts for Hydrogenation of Phenol
Aleksandr Glotov
1
,
Yaroslav Chudakov
1
,
Anna Stavitskaya
2
,
Evgenii A. Ivanov
2
,
Evgenii Ivanov
1
,
Pavel Gushchin
1
,
Anna Zolotukhina
3
,
Anton Maximov
3
,
E.A Karakhanov
3
,
Eduard Karakhanov
4
,
Y. Lvov
1, 5
1
2
Publication type: Journal Article
Publication date: 2017-11-17
scimago Q1
wos Q2
SJR: 0.828
CiteScore: 6.7
Impact factor: 3.9
ISSN: 08885885, 15205045
General Chemistry
General Chemical Engineering
Industrial and Manufacturing Engineering
Abstract
Halloysite tubular nanoclay was applied as a template for synthesis of ruthenium core–shell composite catalysts for the first time; 50 nm diameter ceramic tubular systems with metal seeded interiors were produced. The procedure for the metal deposition and prior halloysite modification had a significant influence on properties of the catalyst and, as a consequence, on its activity in hydrogenation of phenol. Cyclohexanol was the main reaction product, but its yield depended on the substrate conversion and nanoarchitectural composition of the catalysts used. The maximum catalytic activity (turnover frequency, TOF) achieved was 17 282 h–1 in terms of hydrogen uptake per surface Ru atoms. The substrate selectivity of halloysite-based catalysts was also demonstrated at the comparative hydrogenation of phenol and various cresols.
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Total citations:
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GOST
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Vinokurov V. et al. Core/Shell Ruthenium–Halloysite Nanocatalysts for Hydrogenation of Phenol // Industrial & Engineering Chemistry Research. 2017. Vol. 56. No. 47. pp. 14043-14052.
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Vinokurov V., Glotov A., Chudakov Y., Stavitskaya A., Ivanov E. A., Ivanov E., Gushchin P. V., Gushchin P., Zolotukhina A., Maximov A., Karakhanov E., Karakhanov E., Lvov Y. Core/Shell Ruthenium–Halloysite Nanocatalysts for Hydrogenation of Phenol // Industrial & Engineering Chemistry Research. 2017. Vol. 56. No. 47. pp. 14043-14052.
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TY - JOUR
DO - 10.1021/acs.iecr.7b03282
UR - https://pubs.acs.org/doi/10.1021/acs.iecr.7b03282
TI - Core/Shell Ruthenium–Halloysite Nanocatalysts for Hydrogenation of Phenol
T2 - Industrial & Engineering Chemistry Research
AU - Vinokurov, Vladimir
AU - Glotov, Aleksandr
AU - Chudakov, Yaroslav
AU - Stavitskaya, Anna
AU - Ivanov, Evgenii A.
AU - Ivanov, Evgenii
AU - Gushchin, Pavel V.
AU - Gushchin, Pavel
AU - Zolotukhina, Anna
AU - Maximov, Anton
AU - Karakhanov, E.A
AU - Karakhanov, Eduard
AU - Lvov, Y.
PY - 2017
DA - 2017/11/17
PB - American Chemical Society (ACS)
SP - 14043-14052
IS - 47
VL - 56
SN - 0888-5885
SN - 1520-5045
ER -
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BibTex (up to 50 authors)
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@article{2017_Vinokurov,
author = {Vladimir Vinokurov and Aleksandr Glotov and Yaroslav Chudakov and Anna Stavitskaya and Evgenii A. Ivanov and Evgenii Ivanov and Pavel V. Gushchin and Pavel Gushchin and Anna Zolotukhina and Anton Maximov and E.A Karakhanov and Eduard Karakhanov and Y. Lvov},
title = {Core/Shell Ruthenium–Halloysite Nanocatalysts for Hydrogenation of Phenol},
journal = {Industrial & Engineering Chemistry Research},
year = {2017},
volume = {56},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://pubs.acs.org/doi/10.1021/acs.iecr.7b03282},
number = {47},
pages = {14043--14052},
doi = {10.1021/acs.iecr.7b03282}
}
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MLA
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Vinokurov, Vladimir, et al. “Core/Shell Ruthenium–Halloysite Nanocatalysts for Hydrogenation of Phenol.” Industrial & Engineering Chemistry Research, vol. 56, no. 47, Nov. 2017, pp. 14043-14052. https://pubs.acs.org/doi/10.1021/acs.iecr.7b03282.