Industrial & Engineering Chemistry Research

, volume 58 , issue 31 , pages 14595-14602

Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil

Shuai Zhao ^{1, 2}

Wanfen Pu ^{1, 2}

Mikhail A. Varfolomeev ^{1, 2}

Chengdong Yuan ^{1, 2}

Alexander A Rodionov ³

Hide authors affiliations Show authors affiliations: 3 affiliations

State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation, Southwest Petroleum University, Chengdu 610500, People’s Republic of China |

Department of Physical Chemistry, Kazan Federal University, Kremlevskaya Street 18, Kazan 420008, Russia |

Institute of Physics, Kazan Federal University, Kremlevskaya Street 18, Kazan 420008, Russia |

Publication type: Journal Article

Publication date: 2019-07-16

American Chemical Society (ACS)

Industrial & Engineering Chemistry Research

scimago Q1

wos Q2

SJR: 0.828

CiteScore: 6.7

Impact factor: 3.9

ISSN: 08885885, 15205045

DOI: 10.1021/acs.iecr.9b03346

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General Chemistry

General Chemical Engineering

Industrial and Manufacturing Engineering

Abstract

During an in situ combustion (ISC) process, low-temperature oxidation (LTO) is of vital significance for the follow-up oxidation reactions and oil recovery. Herein, this work is intended to carry out in-depth investigations regarding LTO of heavy crude oil. Alterations of evolved gas compositions and oil properties caused by LTO were first examined. Then the particular focus was placed on the analyses of electron paramagnetic resonance (EPR) and nuclear magnetic resonance (NMR) of oxidized oil samples. The results indicated that the LTO degree was intensified with the oxidation temperature, during which produced gas compositions and the contents of element, saturates–aromatics–resins–asphaltenes (SARA) fractions, free radicals, and hydrogen groups of oils changed obviously. Furthermore, part of the main LTO reactions are given in this paper. On the basis of these reactions and experimental results obtained, some aspects of LTO mechanisms of the oil are stated, which were highly valuable for ISC field appl...

Found

2 citations

Emelianov Dmitrii

🤝

65 publications, 1 200 citations

h-index: 21

Kazan Federal University

1 citation

Cheremisin Alexey

🥼 🤝

PhD in Engineering, lecturer

159 publications, 2 044 citations

h-index: 26

Skolkovo Institute of Science and Technology

Surgut State University

Research interests

Digital core

Flows in porous media

Machine learning

Methods of increasing oil recovery

Microfluidics

Numerical simulation

Physics of continuous media

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Cite this

GOST |

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GOST Copy

Zhao S. et al. Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil // Industrial & Engineering Chemistry Research. 2019. Vol. 58. No. 31. pp. 14595-14602.

GOST all authors (up to 50) Copy

Zhao S., Pu W., Varfolomeev M. A., Yuan C., Rodionov A. A. Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil // Industrial & Engineering Chemistry Research. 2019. Vol. 58. No. 31. pp. 14595-14602.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acs.iecr.9b03346

UR - https://doi.org/10.1021/acs.iecr.9b03346

TI - Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil

T2 - Industrial & Engineering Chemistry Research

AU - Zhao, Shuai

AU - Pu, Wanfen

AU - Varfolomeev, Mikhail A.

AU - Yuan, Chengdong

AU - Rodionov, Alexander A

PY - 2019

DA - 2019/07/16

PB - American Chemical Society (ACS)

SP - 14595-14602

IS - 31

VL - 58

SN - 0888-5885

SN - 1520-5045

ER -

BibTex |

Cite this

BibTex (up to 50 authors) Copy

@article{2019_Zhao,

author = {Shuai Zhao and Wanfen Pu and Mikhail A. Varfolomeev and Chengdong Yuan and Alexander A Rodionov},

title = {Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil},

journal = {Industrial & Engineering Chemistry Research},

year = {2019},

volume = {58},

publisher = {American Chemical Society (ACS)},

month = {jul},

url = {https://doi.org/10.1021/acs.iecr.9b03346},

number = {31},

pages = {14595--14602},

doi = {10.1021/acs.iecr.9b03346}

}

MLA

Cite this

MLA Copy

Zhao, Shuai, et al. “Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil.” Industrial & Engineering Chemistry Research, vol. 58, no. 31, Jul. 2019, pp. 14595-14602. https://doi.org/10.1021/acs.iecr.9b03346.

Publisher

American Chemical Society (ACS)

Journal

Industrial & Engineering Chemistry Research

scimago Q1

wos Q2

SJR

0.828

CiteScore

6.7

Impact factor

3.9

ISSN

08885885 (Print)

15205045 (Electronic)

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