Industrial & Engineering Chemistry Research

, том 58 , издание 31 , страницы 14595-14602

Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil

Shuai Zhao ^{1, 2}

Wanfen Pu ^{1, 2}

Mikhail A. Varfolomeev ^{1, 2}

Chengdong Yuan ^{1, 2}

Alexander A Rodionov ³

Скрыть аффилиации авторов Показать аффилиации авторов: 3 аффилиации

State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation, Southwest Petroleum University, Chengdu 610500, People’s Republic of China |

Department of Physical Chemistry, Kazan Federal University, Kremlevskaya Street 18, Kazan 420008, Russia |

Institute of Physics, Kazan Federal University, Kremlevskaya Street 18, Kazan 420008, Russia |

Тип публикации: Journal Article

Дата публикации: 2019-07-16

American Chemical Society (ACS)

Industrial & Engineering Chemistry Research

scimago Q1

wos Q2

БС1

SJR: 0.828

CiteScore: 6.7

Impact factor: 3.9

ISSN: 08885885, 15205045

DOI: 10.1021/acs.iecr.9b03346

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General Chemistry

General Chemical Engineering

Industrial and Manufacturing Engineering

Краткое описание

During an in situ combustion (ISC) process, low-temperature oxidation (LTO) is of vital significance for the follow-up oxidation reactions and oil recovery. Herein, this work is intended to carry out in-depth investigations regarding LTO of heavy crude oil. Alterations of evolved gas compositions and oil properties caused by LTO were first examined. Then the particular focus was placed on the analyses of electron paramagnetic resonance (EPR) and nuclear magnetic resonance (NMR) of oxidized oil samples. The results indicated that the LTO degree was intensified with the oxidation temperature, during which produced gas compositions and the contents of element, saturates–aromatics–resins–asphaltenes (SARA) fractions, free radicals, and hydrogen groups of oils changed obviously. Furthermore, part of the main LTO reactions are given in this paper. On the basis of these reactions and experimental results obtained, some aspects of LTO mechanisms of the oil are stated, which were highly valuable for ISC field appl...

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Zhao S. et al. Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil // Industrial & Engineering Chemistry Research. 2019. Vol. 58. No. 31. pp. 14595-14602.

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Zhao S., Pu W., Varfolomeev M. A., Yuan C., Rodionov A. A. Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil // Industrial & Engineering Chemistry Research. 2019. Vol. 58. No. 31. pp. 14595-14602.

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TY - JOUR

DO - 10.1021/acs.iecr.9b03346

UR - https://doi.org/10.1021/acs.iecr.9b03346

TI - Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil

T2 - Industrial & Engineering Chemistry Research

AU - Zhao, Shuai

AU - Pu, Wanfen

AU - Varfolomeev, Mikhail A.

AU - Yuan, Chengdong

AU - Rodionov, Alexander A

PY - 2019

DA - 2019/07/16

PB - American Chemical Society (ACS)

SP - 14595-14602

IS - 31

VL - 58

SN - 0888-5885

SN - 1520-5045

ER -

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@article{2019_Zhao,

author = {Shuai Zhao and Wanfen Pu and Mikhail A. Varfolomeev and Chengdong Yuan and Alexander A Rodionov},

title = {Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil},

journal = {Industrial & Engineering Chemistry Research},

year = {2019},

volume = {58},

publisher = {American Chemical Society (ACS)},

month = {jul},

url = {https://doi.org/10.1021/acs.iecr.9b03346},

number = {31},

pages = {14595--14602},

doi = {10.1021/acs.iecr.9b03346}

}

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Zhao, Shuai, et al. “Integrative Investigation of Low-Temperature Oxidation Characteristics and Mechanisms of Heavy Crude Oil.” Industrial & Engineering Chemistry Research, vol. 58, no. 31, Jul. 2019, pp. 14595-14602. https://doi.org/10.1021/acs.iecr.9b03346.