Heterocyclic Nitrilimines and Their Use in the Synthesis of Complex High-Nitrogen Materials
Jesse J. Sabatini
1, 2, 3
,
Sarah E Davis Finch
4
,
Ashank Sethia
5
,
Edward B. Byrd
6
,
Matthias Zeller
7
,
Davin G Piercey
1, 2, 4
3
Department of Chemistry & Life Science, U.S. Military Academy, West Point, New York 10996, United States
|
Publication type: Journal Article
Publication date: 2021-05-10
scimago Q1
wos Q1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
33970605
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
We show the ability of a nitrilimine prepared from 3-amino-5-nitro-1,2,4-triazole to undergo various cyclization and rearrangement reactions, giving a beautiful diversity of nitrogen-rich heterocyclic products. This chemistry includes the first cyclization of a nitrilimine with a diazonium species, giving a tetrazole, a previously unknown transformation, as well as leading to the creation of several new energetic materials with backbones not available by traditional techniques. New materials prepared were characterized both chemically (multinuclear NMR, IR, mass spectrometry, and elemental analysis) and energetically, with sensitivities and performances reported.
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21
Total citations:
21
Citations from 2025:
6
(28.57%)
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GOST
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Sabatini J. J. et al. Heterocyclic Nitrilimines and Their Use in the Synthesis of Complex High-Nitrogen Materials // Inorganic Chemistry. 2021. Vol. 60. No. 11. pp. 7607-7611.
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Sabatini J. J., Davis Finch S. E., Sethia A., Byrd E. B., Zeller M., Piercey D. G. Heterocyclic Nitrilimines and Their Use in the Synthesis of Complex High-Nitrogen Materials // Inorganic Chemistry. 2021. Vol. 60. No. 11. pp. 7607-7611.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.inorgchem.1c00469
UR - https://doi.org/10.1021/acs.inorgchem.1c00469
TI - Heterocyclic Nitrilimines and Their Use in the Synthesis of Complex High-Nitrogen Materials
T2 - Inorganic Chemistry
AU - Sabatini, Jesse J.
AU - Davis Finch, Sarah E
AU - Sethia, Ashank
AU - Byrd, Edward B.
AU - Zeller, Matthias
AU - Piercey, Davin G
PY - 2021
DA - 2021/05/10
PB - American Chemical Society (ACS)
SP - 7607-7611
IS - 11
VL - 60
PMID - 33970605
SN - 0020-1669
SN - 1520-510X
ER -
Cite this
BibTex (up to 50 authors)
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@article{2021_Sabatini,
author = {Jesse J. Sabatini and Sarah E Davis Finch and Ashank Sethia and Edward B. Byrd and Matthias Zeller and Davin G Piercey},
title = {Heterocyclic Nitrilimines and Their Use in the Synthesis of Complex High-Nitrogen Materials},
journal = {Inorganic Chemistry},
year = {2021},
volume = {60},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/acs.inorgchem.1c00469},
number = {11},
pages = {7607--7611},
doi = {10.1021/acs.inorgchem.1c00469}
}
Cite this
MLA
Copy
Sabatini, Jesse J., et al. “Heterocyclic Nitrilimines and Their Use in the Synthesis of Complex High-Nitrogen Materials.” Inorganic Chemistry, vol. 60, no. 11, May. 2021, pp. 7607-7611. https://doi.org/10.1021/acs.inorgchem.1c00469.