The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids
Publication type: Journal Article
Publication date: 2022-03-15
scimago Q1
wos Q1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
35290056
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Passivation of perovskite films by ionic liquids (ILs) improves the performance (efficiency and stability) of perovskite solar cells (PSCs). However, the role of ILs in the passivation of perovskite films is not fully understood. Here, we report the reactions of commonly used ILs with the components of perovskites. The reaction of ILs with perovskite precursors (PbI2 and methylammonium iodide or formamidinium iodide) in a 1:1:1 molar ratio affords one-dimensional (1D) salts composed of the IL cation interspersed along infinite 1D polymeric [PbI3]-n chains. If the IL is applied in excess, the resulting crystal is composed of six cations surrounding a discrete [Pb3I12]6- cluster. All the isolated salts were unambiguously characterized by single-crystal X-ray diffraction analysis, which also reveals extensive hydrogen-bonding interactions.
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21
Total citations:
21
Citations from 2024:
11
(52%)
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GOST
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Zhang S. et al. The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids // Inorganic Chemistry. 2022. Vol. 61. No. 12. pp. 5010-5016.
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Zhang S., Xiao T., Fadaei‐Tirani F., Scopelliti R., Nazeeruddin M., Zhu D., Dyson P. J., Fei Z. The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids // Inorganic Chemistry. 2022. Vol. 61. No. 12. pp. 5010-5016.
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RIS
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TY - JOUR
DO - 10.1021/acs.inorgchem.1c03862
UR - https://doi.org/10.1021/acs.inorgchem.1c03862
TI - The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids
T2 - Inorganic Chemistry
AU - Zhang, Shunlin
AU - Xiao, Tianyu
AU - Fadaei‐Tirani, Farzaneh
AU - Scopelliti, Rosario
AU - Nazeeruddin, M.
AU - Zhu, Dunru
AU - Dyson, Paul J
AU - Fei, Zhaofu
PY - 2022
DA - 2022/03/15
PB - American Chemical Society (ACS)
SP - 5010-5016
IS - 12
VL - 61
PMID - 35290056
SN - 0020-1669
SN - 1520-510X
ER -
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BibTex (up to 50 authors)
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@article{2022_Zhang,
author = {Shunlin Zhang and Tianyu Xiao and Farzaneh Fadaei‐Tirani and Rosario Scopelliti and M. Nazeeruddin and Dunru Zhu and Paul J Dyson and Zhaofu Fei},
title = {The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids},
journal = {Inorganic Chemistry},
year = {2022},
volume = {61},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/acs.inorgchem.1c03862},
number = {12},
pages = {5010--5016},
doi = {10.1021/acs.inorgchem.1c03862}
}
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MLA
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Zhang, Shunlin, et al. “The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids.” Inorganic Chemistry, vol. 61, no. 12, Mar. 2022, pp. 5010-5016. https://doi.org/10.1021/acs.inorgchem.1c03862.