Inorganic Chemistry

, том 61 , издание 12 , страницы 5010-5016

The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids

Тип публикации: Journal Article

Дата публикации: 2022-03-15

American Chemical Society (ACS)

Inorganic Chemistry

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SJR: 0.958

CiteScore: 7.4

Impact factor: 4.7

ISSN: 00201669, 1520510X

DOI: 10.1021/acs.inorgchem.1c03862

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PubMed ID: 35290056

Inorganic Chemistry

Physical and Theoretical Chemistry

Краткое описание

Passivation of perovskite films by ionic liquids (ILs) improves the performance (efficiency and stability) of perovskite solar cells (PSCs). However, the role of ILs in the passivation of perovskite films is not fully understood. Here, we report the reactions of commonly used ILs with the components of perovskites. The reaction of ILs with perovskite precursors (PbI2 and methylammonium iodide or formamidinium iodide) in a 1:1:1 molar ratio affords one-dimensional (1D) salts composed of the IL cation interspersed along infinite 1D polymeric [PbI3]-n chains. If the IL is applied in excess, the resulting crystal is composed of six cations surrounding a discrete [Pb3I12]6- cluster. All the isolated salts were unambiguously characterized by single-crystal X-ray diffraction analysis, which also reveals extensive hydrogen-bonding interactions.

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Zhang S. et al. The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids // Inorganic Chemistry. 2022. Vol. 61. No. 12. pp. 5010-5016.

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Zhang S., Xiao T., Fadaei‐Tirani F., Scopelliti R., Nazeeruddin M., Zhu D., Dyson P. J., Fei Z. The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids // Inorganic Chemistry. 2022. Vol. 61. No. 12. pp. 5010-5016.

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TY - JOUR

DO - 10.1021/acs.inorgchem.1c03862

UR - https://doi.org/10.1021/acs.inorgchem.1c03862

TI - The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids

T2 - Inorganic Chemistry

AU - Zhang, Shunlin

AU - Xiao, Tianyu

AU - Fadaei‐Tirani, Farzaneh

AU - Scopelliti, Rosario

AU - Nazeeruddin, M.

AU - Zhu, Dunru

AU - Dyson, Paul J

AU - Fei, Zhaofu

PY - 2022

DA - 2022/03/15

PB - American Chemical Society (ACS)

SP - 5010-5016

IS - 12

VL - 61

PMID - 35290056

SN - 0020-1669

SN - 1520-510X

ER -

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@article{2022_Zhang,

author = {Shunlin Zhang and Tianyu Xiao and Farzaneh Fadaei‐Tirani and Rosario Scopelliti and M. Nazeeruddin and Dunru Zhu and Paul J Dyson and Zhaofu Fei},

title = {The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids},

journal = {Inorganic Chemistry},

year = {2022},

volume = {61},

publisher = {American Chemical Society (ACS)},

month = {mar},

url = {https://doi.org/10.1021/acs.inorgchem.1c03862},

number = {12},

pages = {5010--5016},

doi = {10.1021/acs.inorgchem.1c03862}

}

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Zhang, Shunlin, et al. “The Chemistry of the Passivation Mechanism of Perovskite Films with Ionic Liquids.” Inorganic Chemistry, vol. 61, no. 12, Mar. 2022, pp. 5010-5016. https://doi.org/10.1021/acs.inorgchem.1c03862.

Издатель

American Chemical Society (ACS)

Журнал

Inorganic Chemistry

scimago Q1

wos Q1

БС1

SJR

0.958

CiteScore

7.4

Impact factor

4.7

ISSN

00201669 (Print)

1520510X (Electronic)