Inorganic Chemistry

, том 56 , издание 19 , страницы 11845-11853

Insight into the Electrochemical Sodium Insertion of Vanadium Superstoichiometric NASICON Phosphate

Тип публикации: Journal Article

Дата публикации: 2017-09-13

American Chemical Society (ACS)

Inorganic Chemistry

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SJR: 0.958

CiteScore: 7.4

Impact factor: 4.7

ISSN: 00201669, 1520510X

DOI: 10.1021/acs.inorgchem.7b01846

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PubMed ID: 28902502

Inorganic Chemistry

Physical and Theoretical Chemistry

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A slight deviation of the stoichiometry has been introduced in Na3-3xV2+x(PO4)3 (0 ≤ x ≤ 0.1) samples to determine the effect on the structural and electrochemical behavior as a positive electrode in sodium-ion batteries. X-ray diffraction and XPS results provide evidence for the flexibility of the NASICON framework to allow a limited vanadium superstoichiometry. In particular, the Na2.94V2.02(PO4)3 formula reveals the best electrochemical performance at the highest rate (40C) and capacity retention upon long cycling. It is attributed to the excellent kinetic response and interphase chemical stability upon cycling. The electrochemical performance of this vanadium superstoichiometric sample in a full sodium-ion cell is also described.

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Aragón M. J. et al. Insight into the Electrochemical Sodium Insertion of Vanadium Superstoichiometric NASICON Phosphate // Inorganic Chemistry. 2017. Vol. 56. No. 19. pp. 11845-11853.

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Aragón M. J., Lavela P., Alcántara R., Tirado J. L. Insight into the Electrochemical Sodium Insertion of Vanadium Superstoichiometric NASICON Phosphate // Inorganic Chemistry. 2017. Vol. 56. No. 19. pp. 11845-11853.

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TY - JOUR

DO - 10.1021/acs.inorgchem.7b01846

UR - https://doi.org/10.1021/acs.inorgchem.7b01846

TI - Insight into the Electrochemical Sodium Insertion of Vanadium Superstoichiometric NASICON Phosphate

T2 - Inorganic Chemistry

AU - Aragón, María José

AU - Lavela, P.

AU - Alcántara, Ricardo

AU - Tirado, José L.

PY - 2017

DA - 2017/09/13

PB - American Chemical Society (ACS)

SP - 11845-11853

IS - 19

VL - 56

PMID - 28902502

SN - 0020-1669

SN - 1520-510X

ER -

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@article{2017_Aragón,

author = {María José Aragón and P. Lavela and Ricardo Alcántara and José L. Tirado},

title = {Insight into the Electrochemical Sodium Insertion of Vanadium Superstoichiometric NASICON Phosphate},

journal = {Inorganic Chemistry},

year = {2017},

volume = {56},

publisher = {American Chemical Society (ACS)},

month = {sep},

url = {https://doi.org/10.1021/acs.inorgchem.7b01846},

number = {19},

pages = {11845--11853},

doi = {10.1021/acs.inorgchem.7b01846}

}

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Aragón, María José, et al. “Insight into the Electrochemical Sodium Insertion of Vanadium Superstoichiometric NASICON Phosphate.” Inorganic Chemistry, vol. 56, no. 19, Sep. 2017, pp. 11845-11853. https://doi.org/10.1021/acs.inorgchem.7b01846.