American Chemical Society (ACS)
Inorganic Chemistry
,  том 58 ,  издание 17 ,  страницы 11546-11552

Alkali-Glass Behavior in Honeycomb-Type Layered Li3–xNaxNi2SbO6 Solid Solution

Coélio Vallée 1
, 
Matthieu Saubanère 1, 2
, 
Paula Sanz Camacho 2, 3
, 
Yohan Biecher 2, 3
, 
Bernard Fraisse 1
, 
E. Suard 4
, 
Gwenaelle Rousse 2, 5, 6
, 
Dany Carlier 2, 3
, 
Romain Berthelot 1, 2
1
 
2
 
Re′seau sur le Stockage E′lectrochimique de l’Énergie (RS2E), CNRS, 80039 Amiens, France | 
3
 
4
 
5
 
6
 
Тип публикации: Journal Article
Дата публикации: 2019-08-22
American Chemical Society (ACS)
scimago Q1
wos Q1
БС1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
Inorganic Chemistry
Physical and Theoretical Chemistry
Краткое описание
Layered oxide compositions Li3-xNaxNi2SbO6 have been prepared by solid-state synthesis. A complete solid solution is evidenced and characterized by X-ray and neutron diffraction as well as 7Li and 23Na solid-state nuclear magnetic resonance spectroscopy. The transition-metal layer is characterized by the classic honeycomb Ni2+/Sb5+ ordering, whereas a more uncommon randomly mixed occupancy of lithium and sodium is evidenced within the alkali interslab space. In situ X-ray diffraction and density functional theory calculations show that this alkali disordered feature is entropically driven. Fast cooling then appears as a synthesis root to confine bidimensional alkali glass within crystalline layered oxides.
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Vallée C. et al. Alkali-Glass Behavior in Honeycomb-Type Layered Li3–xNaxNi2SbO6 Solid Solution // Inorganic Chemistry. 2019. Vol. 58. No. 17. pp. 11546-11552.
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Vallée C., Saubanère M., Sanz Camacho P., Biecher Y., Fraisse B., Suard E., Rousse G., Carlier D., Berthelot R. Alkali-Glass Behavior in Honeycomb-Type Layered Li3–xNaxNi2SbO6 Solid Solution // Inorganic Chemistry. 2019. Vol. 58. No. 17. pp. 11546-11552.
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TY - JOUR
DO - 10.1021/acs.inorgchem.9b01385
UR - https://doi.org/10.1021/acs.inorgchem.9b01385
TI - Alkali-Glass Behavior in Honeycomb-Type Layered Li3–xNaxNi2SbO6 Solid Solution
T2 - Inorganic Chemistry
AU - Vallée, Coélio
AU - Saubanère, Matthieu
AU - Sanz Camacho, Paula
AU - Biecher, Yohan
AU - Fraisse, Bernard
AU - Suard, E.
AU - Rousse, Gwenaelle
AU - Carlier, Dany
AU - Berthelot, Romain
PY - 2019
DA - 2019/08/22
PB - American Chemical Society (ACS)
SP - 11546-11552
IS - 17
VL - 58
PMID - 31436964
SN - 0020-1669
SN - 1520-510X
ER -
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@article{2019_Vallée,
author = {Coélio Vallée and Matthieu Saubanère and Paula Sanz Camacho and Yohan Biecher and Bernard Fraisse and E. Suard and Gwenaelle Rousse and Dany Carlier and Romain Berthelot},
title = {Alkali-Glass Behavior in Honeycomb-Type Layered Li3–xNaxNi2SbO6 Solid Solution},
journal = {Inorganic Chemistry},
year = {2019},
volume = {58},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.inorgchem.9b01385},
number = {17},
pages = {11546--11552},
doi = {10.1021/acs.inorgchem.9b01385}
}
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Vallée, Coélio, et al. “Alkali-Glass Behavior in Honeycomb-Type Layered Li3–xNaxNi2SbO6 Solid Solution.” Inorganic Chemistry, vol. 58, no. 17, Aug. 2019, pp. 11546-11552. https://doi.org/10.1021/acs.inorgchem.9b01385.