Tuning of Emission by Eu3+ Concentration in a Pyrophosphate: the Effect of Local Symmetry
Тип публикации: Journal Article
Дата публикации: 2019-12-27
scimago Q1
wos Q1
БС1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
31880440
Inorganic Chemistry
Physical and Theoretical Chemistry
Краткое описание
The local symmetry of a Eu3+ ion has a crucial effect on its luminescence properties. In this work, we show that the red/orange ratio in the emission of Eu3+-doped MgIn2P4O14 phosphors is tunable by adjusting the Eu3+ concentrations, due to the change in the local symmetry of metal ions. The substitution of Eu3+ for In3+ lowers the distortion in the lattice of monoclinic MgIn2P4O14, and an increase in Eu3+ doping concentration causes the metal ion sites to shift closer to an inverse center, leading to a reversal of the relative emission intensity of a magnetic dipole transition to an electric dipole transition. Meanwhile, the higher asymmetry of metal ion sites occupied by Eu3+ in MgIn2P4O14 makes the luminescence less thermally stable than that in Mg3In4P6O24.
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Zhang J. et al. Tuning of Emission by Eu3+ Concentration in a Pyrophosphate: the Effect of Local Symmetry // Inorganic Chemistry. 2019. Vol. 59. No. 4. pp. 2241-2247.
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Zhang J., Liu J., Wang W., Ma L., Wang X., Jin Z. Tuning of Emission by Eu3+ Concentration in a Pyrophosphate: the Effect of Local Symmetry // Inorganic Chemistry. 2019. Vol. 59. No. 4. pp. 2241-2247.
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TY - JOUR
DO - 10.1021/acs.inorgchem.9b02949
UR - https://doi.org/10.1021/acs.inorgchem.9b02949
TI - Tuning of Emission by Eu3+ Concentration in a Pyrophosphate: the Effect of Local Symmetry
T2 - Inorganic Chemistry
AU - Zhang, Jing
AU - Liu, Jinkang
AU - Wang, Wenjun
AU - Ma, Li
AU - Wang, Xiao-jun
AU - Jin, Zhanpeng
PY - 2019
DA - 2019/12/27
PB - American Chemical Society (ACS)
SP - 2241-2247
IS - 4
VL - 59
PMID - 31880440
SN - 0020-1669
SN - 1520-510X
ER -
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@article{2019_Zhang,
author = {Jing Zhang and Jinkang Liu and Wenjun Wang and Li Ma and Xiao-jun Wang and Zhanpeng Jin},
title = {Tuning of Emission by Eu3+ Concentration in a Pyrophosphate: the Effect of Local Symmetry},
journal = {Inorganic Chemistry},
year = {2019},
volume = {59},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/acs.inorgchem.9b02949},
number = {4},
pages = {2241--2247},
doi = {10.1021/acs.inorgchem.9b02949}
}
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Zhang, Jing, et al. “Tuning of Emission by Eu3+ Concentration in a Pyrophosphate: the Effect of Local Symmetry.” Inorganic Chemistry, vol. 59, no. 4, Dec. 2019, pp. 2241-2247. https://doi.org/10.1021/acs.inorgchem.9b02949.
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