Dibromo-BODIPY as an Organic Photocatalyst for Radical–Ionic Sequences
Тип публикации: Journal Article
Дата публикации: 2021-11-02
SCImago Q2
WOS Q1
БС1
SJR: 0.604
CiteScore: 6.1
Impact factor: 3.6
ISSN: 00223263, 15206904
PubMed ID:
34726403
Organic Chemistry
Краткое описание
A new dibrominated 4,4-difluoro-4-bora-3a,4a-diaza-s-indacene (BODIPY) is reported as a new metal-free photocatalyst. This BODIPY showed similar optoelectronic, electrochemical, and performance properties to those of Ru(bpy)3Cl2, one of the most common photocatalysts in a known radical-ionic transformation, such as the formation of 1,4-dicarbonyl compounds. Moreover, additional sequences in which the generated oxonium ion is trapped by an internal nucleophile were developed using this BODIPY photocatalyst. These new sequences allowed the straightforward preparation of γ-alkoxylactones, monoprotected 1,4-ketoaldehydes, and dihydrofurans. This new catalyst, the methodology, and the forged functional groups could be important tools in organic synthesis.
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García Santos W. H. et al. Dibromo-BODIPY as an Organic Photocatalyst for Radical–Ionic Sequences // Journal of Organic Chemistry. 2021. Vol. 86. No. 23. pp. 16315-16326.
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García Santos W. H., Ordóñez Hernández J., Farfán Paredes M., Castro-Cruz H. M., Macías-Ruvalcaba N. A., García-Ortega H., Cordero-Vargas A. Dibromo-BODIPY as an Organic Photocatalyst for Radical–Ionic Sequences // Journal of Organic Chemistry. 2021. Vol. 86. No. 23. pp. 16315-16326.
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TY - JOUR
DO - 10.1021/acs.joc.1c01598
UR - https://doi.org/10.1021/acs.joc.1c01598
TI - Dibromo-BODIPY as an Organic Photocatalyst for Radical–Ionic Sequences
T2 - Journal of Organic Chemistry
AU - García Santos, William H
AU - Ordóñez Hernández, Javier
AU - Farfán Paredes, Mónica
AU - Castro-Cruz, Hiram M.
AU - Macías-Ruvalcaba, Norma A.
AU - García-Ortega, Héctor
AU - Cordero-Vargas, Alejandro
PY - 2021
DA - 2021/11/02
PB - American Chemical Society (ACS)
SP - 16315-16326
IS - 23
VL - 86
PMID - 34726403
SN - 0022-3263
SN - 1520-6904
ER -
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@article{2021_García Santos,
author = {William H García Santos and Javier Ordóñez Hernández and Mónica Farfán Paredes and Hiram M. Castro-Cruz and Norma A. Macías-Ruvalcaba and Héctor García-Ortega and Alejandro Cordero-Vargas},
title = {Dibromo-BODIPY as an Organic Photocatalyst for Radical–Ionic Sequences},
journal = {Journal of Organic Chemistry},
year = {2021},
volume = {86},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/acs.joc.1c01598},
number = {23},
pages = {16315--16326},
doi = {10.1021/acs.joc.1c01598}
}
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García Santos, William H., et al. “Dibromo-BODIPY as an Organic Photocatalyst for Radical–Ionic Sequences.” Journal of Organic Chemistry, vol. 86, no. 23, Nov. 2021, pp. 16315-16326. https://doi.org/10.1021/acs.joc.1c01598.
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