Journal of Organic Chemistry

, volume 88 , issue 13 , pages 9518-9522

Electrochemical Oxidative C–H Amination through a Ritter-Type Reaction

Yiwen Xu ¹

Qiang Li ¹

Runyou Ye ¹

Buyi Xu ²

Xiangge Zhou ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

College of Chemistry, Sichuan University, Wangjiang Road 29, Chengdu, Sichuan 610064, China |

National Anti-Drug Laboratory Sichuan Regional Center, 36 Yunling Road, Chengdu, Sichuan 610200, P.R. China |

Publication type: Journal Article

Publication date: 2023-06-01

American Chemical Society (ACS)

Journal of Organic Chemistry

scimago Q2

wos Q1

SJR: 0.737

CiteScore: 6.1

Impact factor: 3.6

ISSN: 00223263, 15206904

DOI: 10.1021/acs.joc.3c00609

Copy DOI

PubMed ID: 37262003

Organic Chemistry

Abstract

A straightforward strategy for direct benzylic C–H bond amination via an electrochemical Ritter-type reaction is developed. The reaction demonstrates simpler and milder reaction conditions over the existing methods without extra mediator. Moderate to excellent yields up to 94% of the desired amide products were obtained with a broad substrate scope. The removal of the Ac group by a simple step can afford NH-free benzylic amines, providing a suitable approach for the late-stage functionalization of bioactive molecules.

Found

3 citations

Budnikova Yulia

DSc in Chemistry, professor

258 publications, 4 500 citations, 54 reviews

h-index: 34

A.E. Arbuzov Institute of Organic and Physical Chemistry of the Kazan Scientific Center of the Russian Academy of Sciences

Kazan Scientific Center of the Russian Academy of Sciences

Research interests

C-H functionalization

Catalysis

Charge transfer

Chemistry of organoelement compounds

2 citations

Babaeva Olga

PhD in Chemistry

56 publications, 438 citations

h-index: 12

A.E. Arbuzov Institute of Organic and Physical Chemistry of the Kazan Scientific Center of the Russian Academy of Sciences

Research interests

Organic Chemistry

Physical Chemistry

2 citations

Bashirova Ekaterina

5 publications, 13 citations

h-index: 2

A.E. Arbuzov Institute of Organic and Physical Chemistry of the Kazan Scientific Center of the Russian Academy of Sciences

Kazan Scientific Center of the Russian Academy of Sciences

1 citation

Babaev Vasily

PhD in Chemistry, associate professor

81 publications, 931 citations

h-index: 17

A.E. Arbuzov Institute of Organic and Physical Chemistry of the Kazan Scientific Center of the Russian Academy of Sciences

Research interests

Mass Spectrometry

1 citation

Medvedev Michael

PhD in Physics and Mathematics, associate professor

85 publications, 2 068 citations, 7 reviews

h-index: 19

N.D. Zelinsky Institute of Organic Chemistry of the Russian Academy of Sciences

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Cite this

GOST |

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GOST Copy

Xu Y. et al. Electrochemical Oxidative C–H Amination through a Ritter-Type Reaction // Journal of Organic Chemistry. 2023. Vol. 88. No. 13. pp. 9518-9522.

GOST all authors (up to 50) Copy

Xu Y., Li Q., Ye R., Xu B., Zhou X. Electrochemical Oxidative C–H Amination through a Ritter-Type Reaction // Journal of Organic Chemistry. 2023. Vol. 88. No. 13. pp. 9518-9522.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acs.joc.3c00609

UR - https://pubs.acs.org/doi/10.1021/acs.joc.3c00609

TI - Electrochemical Oxidative C–H Amination through a Ritter-Type Reaction

T2 - Journal of Organic Chemistry

AU - Xu, Yiwen

AU - Li, Qiang

AU - Ye, Runyou

AU - Xu, Buyi

AU - Zhou, Xiangge

PY - 2023

DA - 2023/06/01

PB - American Chemical Society (ACS)

SP - 9518-9522

IS - 13

VL - 88

PMID - 37262003

SN - 0022-3263

SN - 1520-6904

ER -

BibTex |

Cite this

BibTex (up to 50 authors) Copy

@article{2023_Xu,

author = {Yiwen Xu and Qiang Li and Runyou Ye and Buyi Xu and Xiangge Zhou},

title = {Electrochemical Oxidative C–H Amination through a Ritter-Type Reaction},

journal = {Journal of Organic Chemistry},

year = {2023},

volume = {88},

publisher = {American Chemical Society (ACS)},

month = {jun},

url = {https://pubs.acs.org/doi/10.1021/acs.joc.3c00609},

number = {13},

pages = {9518--9522},

doi = {10.1021/acs.joc.3c00609}

}

MLA

Cite this

MLA Copy

Xu, Yiwen, et al. “Electrochemical Oxidative C–H Amination through a Ritter-Type Reaction.” Journal of Organic Chemistry, vol. 88, no. 13, Jun. 2023, pp. 9518-9522. https://pubs.acs.org/doi/10.1021/acs.joc.3c00609.

Publisher

American Chemical Society (ACS)

Journal

Journal of Organic Chemistry

scimago Q2

wos Q1

SJR

0.737

CiteScore

6.1

Impact factor

3.6

ISSN

00223263 (Print)

15206904 (Electronic)

Profiles

Xiangge Zhou