Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix
Тип публикации: Journal Article
Дата публикации: 2017-12-21
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SJR: 0.634
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ISSN: 10895639, 15205215
PubMed ID:
29206459
Physical and Theoretical Chemistry
Краткое описание
We report on the complex of a noble-gas hydride HXeOH with carbon monoxide. This species is prepared via the annealing-induced H + Xe + OH···CO reaction in a xenon matrix, the OH···CO complexes being produced by VUV photolysis of the H2O···CO complexes. The H-Xe stretching mode of the HXeOH···CO complex absorbs at 1590.3 cm-1 and it is blue-shifted by 12.7 cm-1 from the H-Xe stretching band of HXeOH monomer. The observed blue shift indicates the stabilization of the H-Xe bond upon complexation, which is characteristic of complexes of noble-gas hydrides. The HXeOH···CO species is the first complex of a noble-gas hydride with carbon monoxide and the second observed complex of HXeOH. On the basis of the MP2/aug-cc-pVTZ-PP calculations, the experimental complex is assigned to the structure, where the carbon atom of CO interacts with the oxygen atom of HXeOH.
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Ryazantsev S. V. et al. Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix // Journal of Physical Chemistry A. 2017. Vol. 122. No. 1. pp. 159-166.
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Ryazantsev S. V., Lundell J., Feldman V. I., Khriachtchev L. Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix // Journal of Physical Chemistry A. 2017. Vol. 122. No. 1. pp. 159-166.
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TY - JOUR
DO - 10.1021/acs.jpca.7b10293
UR - https://pubs.acs.org/doi/10.1021/acs.jpca.7b10293
TI - Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix
T2 - Journal of Physical Chemistry A
AU - Ryazantsev, Sergey V
AU - Lundell, Jan
AU - Feldman, Vladimir I.
AU - Khriachtchev, Leonid
PY - 2017
DA - 2017/12/21
PB - American Chemical Society (ACS)
SP - 159-166
IS - 1
VL - 122
PMID - 29206459
SN - 1089-5639
SN - 1520-5215
ER -
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@article{2017_Ryazantsev,
author = {Sergey V Ryazantsev and Jan Lundell and Vladimir I. Feldman and Leonid Khriachtchev},
title = {Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix},
journal = {Journal of Physical Chemistry A},
year = {2017},
volume = {122},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://pubs.acs.org/doi/10.1021/acs.jpca.7b10293},
number = {1},
pages = {159--166},
doi = {10.1021/acs.jpca.7b10293}
}
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Ryazantsev, Sergey V., et al. “Photochemistry of the H2O/CO System Revisited: The HXeOH···CO Complex in a Xenon Matrix.” Journal of Physical Chemistry A, vol. 122, no. 1, Dec. 2017, pp. 159-166. https://pubs.acs.org/doi/10.1021/acs.jpca.7b10293.
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