Interplay of Intra- and Intermolecular Interactions in Solid Iodine at Low Temperatures: Experimental and Theoretic Spectroscopy Study
Irina D. Yushina
1
,
B.A. Kolesov
2, 3
Тип публикации: Journal Article
Дата публикации: 2019-05-07
scimago Q2
wos Q2
БС2
SJR: 0.634
CiteScore: 4.8
Impact factor: 2.8
ISSN: 10895639, 15205215
PubMed ID:
31063373
Physical and Theoretical Chemistry
Краткое описание
This work is devoted to the discussion of structural changes in crystalline iodine under low temperature studied from experimental and theoretic points of view. Experimental Raman spectra in the temperature range 5-300 K demonstrated unusual behavior of stretching vibration at ∼180 cm-1 with temperature. The data allowed obtaining of ω( T) functions for both external translational and internal stretching modes of I2. It was found that ω( T) trends significantly differ in comparison to typical van der Waals crystal α-S8. The observed anomalies are explained from a theoretic point of view because of the strengthening of intralayer halogen bonding between I2 molecules.
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Yushina I. D., Kolesov B. Interplay of Intra- and Intermolecular Interactions in Solid Iodine at Low Temperatures: Experimental and Theoretic Spectroscopy Study // Journal of Physical Chemistry A. 2019. Vol. 123. No. 21. pp. 4575-4580.
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Yushina I. D., Kolesov B. Interplay of Intra- and Intermolecular Interactions in Solid Iodine at Low Temperatures: Experimental and Theoretic Spectroscopy Study // Journal of Physical Chemistry A. 2019. Vol. 123. No. 21. pp. 4575-4580.
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TY - JOUR
DO - 10.1021/acs.jpca.9b01167
UR - https://pubs.acs.org/doi/10.1021/acs.jpca.9b01167
TI - Interplay of Intra- and Intermolecular Interactions in Solid Iodine at Low Temperatures: Experimental and Theoretic Spectroscopy Study
T2 - Journal of Physical Chemistry A
AU - Yushina, Irina D.
AU - Kolesov, B.A.
PY - 2019
DA - 2019/05/07
PB - American Chemical Society (ACS)
SP - 4575-4580
IS - 21
VL - 123
PMID - 31063373
SN - 1089-5639
SN - 1520-5215
ER -
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@article{2019_Yushina,
author = {Irina D. Yushina and B.A. Kolesov},
title = {Interplay of Intra- and Intermolecular Interactions in Solid Iodine at Low Temperatures: Experimental and Theoretic Spectroscopy Study},
journal = {Journal of Physical Chemistry A},
year = {2019},
volume = {123},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://pubs.acs.org/doi/10.1021/acs.jpca.9b01167},
number = {21},
pages = {4575--4580},
doi = {10.1021/acs.jpca.9b01167}
}
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Yushina, Irina D., et al. “Interplay of Intra- and Intermolecular Interactions in Solid Iodine at Low Temperatures: Experimental and Theoretic Spectroscopy Study.” Journal of Physical Chemistry A, vol. 123, no. 21, May. 2019, pp. 4575-4580. https://pubs.acs.org/doi/10.1021/acs.jpca.9b01167.
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