Journal of Physical Chemistry C, volume 119, issue 51, pages 28679-28684

Half Metallic Ferromagnetism in Eu-Doped CdS Nanoparticles

Rui Zhao 1, 2
Pan Wang 1
Tianye Yang 1
Zhifang Li 1
Bingxin Xiao 1
Mingzhe Zhang 1
Publication typeJournal Article
Publication date2015-12-15
scimago Q1
SJR0.957
CiteScore6.5
Impact factor3.3
ISSN19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
Hexagonal wurtzite structured Eu3+-doped CdS nanoparticles (CdS:Eu NPs) were synthesized via a gas–liquid phase chemical deposition method. It is found that as-prepared CdS:Eu NPs exhibit distinct and stronger room-temperature ferromagnetism (RTFM). The ferromagnetism as observed from the zero-field-cooling and field-cooling curves of CdS:Eu NPs has been further confirmed by our first-principles calculations based on the density functional theory. Because of a coupling between the 4f-related spin polarized states and the carriers, the half metallic ferromagnetic CdS:Eu NPs could be a desired material for the use in spintronics. The origin of ferromagnetism in CdS:Eu NPs is attributed primarily to the Eu atoms and partially to the Cd vacancies as well.
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