The Role of Synthesis Parameters on Crystallization and Grain Size in Hybrid Halide Perovskite Solar Cells
Jianyou Chen
1
,
Jinkui Song
1
,
Feihong Huang
1
,
Z. Li Haoran
1
,
Shuangshuang Liu
1
,
Mingkui Wang
1
,
Yan Shen
1
Тип публикации: Journal Article
Дата публикации: 2017-08-04
scimago Q1
wos Q3
БС1
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Краткое описание
Antisolvent method has been widely applied to fabricate hybrid halide perovskite solar cells. However, the quality of perovskite film is unable to effectively control for the excessively fast crystallization. In this work, we investigated the effect of precursor concentration and spinning speed as well as additive CH3NH3Cl on quality perovskite film and thus the performance solar cells. The growth of crystal toward the orientation parallel to the direction of facet (002)/(004) slows down as the concentration and spinning speed increases. The lattice constants points out the expansion of crystal size in the direction along the c-axis of around 0.04 A due to the size difference between I and Cl ions. A vertical growth mechanism was proposed to elaborate the crystallite growth of CH3NH3PbI3(Cl) perovskite film. Consequently, the perovskite solar cell efficiency impressively increases from ∼12% to ∼16% along enlarging the crystal size. Various advanced characterization techniques including ultrafast spectrosc...
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Chen J. et al. The Role of Synthesis Parameters on Crystallization and Grain Size in Hybrid Halide Perovskite Solar Cells // Journal of Physical Chemistry C. 2017. Vol. 121. No. 32. pp. 17053-17061.
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Chen J., Song J., Huang F., Li Haoran Z., Liu S., Wang M., Shen Y. The Role of Synthesis Parameters on Crystallization and Grain Size in Hybrid Halide Perovskite Solar Cells // Journal of Physical Chemistry C. 2017. Vol. 121. No. 32. pp. 17053-17061.
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TY - JOUR
DO - 10.1021/acs.jpcc.7b03279
UR - https://doi.org/10.1021/acs.jpcc.7b03279
TI - The Role of Synthesis Parameters on Crystallization and Grain Size in Hybrid Halide Perovskite Solar Cells
T2 - Journal of Physical Chemistry C
AU - Chen, Jianyou
AU - Song, Jinkui
AU - Huang, Feihong
AU - Li Haoran, Z.
AU - Liu, Shuangshuang
AU - Wang, Mingkui
AU - Shen, Yan
PY - 2017
DA - 2017/08/04
PB - American Chemical Society (ACS)
SP - 17053-17061
IS - 32
VL - 121
SN - 1932-7447
SN - 1932-7455
ER -
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@article{2017_Chen,
author = {Jianyou Chen and Jinkui Song and Feihong Huang and Z. Li Haoran and Shuangshuang Liu and Mingkui Wang and Yan Shen},
title = {The Role of Synthesis Parameters on Crystallization and Grain Size in Hybrid Halide Perovskite Solar Cells},
journal = {Journal of Physical Chemistry C},
year = {2017},
volume = {121},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.jpcc.7b03279},
number = {32},
pages = {17053--17061},
doi = {10.1021/acs.jpcc.7b03279}
}
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Chen, Jianyou, et al. “The Role of Synthesis Parameters on Crystallization and Grain Size in Hybrid Halide Perovskite Solar Cells.” Journal of Physical Chemistry C, vol. 121, no. 32, Aug. 2017, pp. 17053-17061. https://doi.org/10.1021/acs.jpcc.7b03279.