Mass Transport through Defects in Graphene Layers
A. A. Eliseev
1, 2
,
Andrei A Eliseev
3, 4
,
A S Kumskov
5, 6, 7
,
N S Falaleev
3
,
V G Zhigalina
5, 6, 7
,
Artem A Eliseev
1, 2, 3, 4
,
Artem Mitrofanov
1, 2, 3, 4
,
Dmitry Petukhov
1, 2
,
D I Petukhov
3, 4
,
A. L. Vasiliev
5, 6
,
N.A. Kiselev
5
7
Scientific-Research Center for Studying Surface and Vacuum Properties, Moscow, 119421 Russia
|
Publication type: Journal Article
Publication date: 2017-10-16
scimago Q1
wos Q3
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
The paper reports an experimental study of ZnTe and CuI transport through graphene wall of SWNTs by high resolution transmission electron microscopy. It is shown that encapsulated material evacuates the tube through the defects in the nanotube walls, while in-tube diffusion appears high enough to provide matter intake from the nanotube volume. Diffusion kinetics was studied by “atoms count” resulting in ZnTe and CuI diffusivities of 7.67 × 10–21 and 1.99 × 10–20 m2/s through single defects in SWNT wall. Semiempirical and DFT modeling of potential energy profiles for different types of defects was utilized to propose minimal structural disturbances in a graphene layer to make possible cross-plane transport of matter. The comparison of experimentally observed diffusivities with calculated activation barrier heights was carried out taking into account an effective temperature of substance under electron beam. Neither of the defects including framework disturbance with 5–7 defects or sp3-bound carbon atomic p...
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6
Total citations:
6
Citations from 2024:
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GOST
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Eliseev A. A. et al. Mass Transport through Defects in Graphene Layers // Journal of Physical Chemistry C. 2017. Vol. 121. No. 42. pp. 23669-23675.
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Eliseev A. A., Eliseev A. A., Kumskov A. S., Falaleev N. S., Falaleev N. S., Zhigalina V. G., Eliseev A. A., Mitrofanov A., Petukhov D., Petukhov D. I., Vasiliev A. L., Kiselev N. Mass Transport through Defects in Graphene Layers // Journal of Physical Chemistry C. 2017. Vol. 121. No. 42. pp. 23669-23675.
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TY - JOUR
DO - 10.1021/acs.jpcc.7b06100
UR - https://pubs.acs.org/doi/10.1021/acs.jpcc.7b06100
TI - Mass Transport through Defects in Graphene Layers
T2 - Journal of Physical Chemistry C
AU - Eliseev, A. A.
AU - Eliseev, Andrei A
AU - Kumskov, A S
AU - Falaleev, Nikolay S
AU - Falaleev, N S
AU - Zhigalina, V G
AU - Eliseev, Artem A
AU - Mitrofanov, Artem
AU - Petukhov, Dmitry
AU - Petukhov, D I
AU - Vasiliev, A. L.
AU - Kiselev, N.A.
PY - 2017
DA - 2017/10/16
PB - American Chemical Society (ACS)
SP - 23669-23675
IS - 42
VL - 121
SN - 1932-7447
SN - 1932-7455
ER -
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BibTex (up to 50 authors)
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@article{2017_Eliseev,
author = {A. A. Eliseev and Andrei A Eliseev and A S Kumskov and Nikolay S Falaleev and N S Falaleev and V G Zhigalina and Artem A Eliseev and Artem Mitrofanov and Dmitry Petukhov and D I Petukhov and A. L. Vasiliev and N.A. Kiselev},
title = {Mass Transport through Defects in Graphene Layers},
journal = {Journal of Physical Chemistry C},
year = {2017},
volume = {121},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://pubs.acs.org/doi/10.1021/acs.jpcc.7b06100},
number = {42},
pages = {23669--23675},
doi = {10.1021/acs.jpcc.7b06100}
}
Cite this
MLA
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Eliseev, A. A., et al. “Mass Transport through Defects in Graphene Layers.” Journal of Physical Chemistry C, vol. 121, no. 42, Oct. 2017, pp. 23669-23675. https://pubs.acs.org/doi/10.1021/acs.jpcc.7b06100.
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