Oxygen Reduction Reaction on Classically Immiscible Bimetallics: A Case Study of RhAu
Publication type: Journal Article
Publication date: 2018-01-25
scimago Q1
wos Q3
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
The catalytic properties of bulk-immiscible alloys are less explored than their bulk-miscible counterparts due to inherent difficulties in their synthesis and stabilization. The development of alternative synthetic methods can, however, provide routes toward bulk-immiscible nanoparticles with metastable randomly alloyed structures. In this study, we combine computational screening and a microwave-based synthesis method to target bulk-immiscible alloys that show enhanced reactivity over pure metals for the oxygen reduction reaction (ORR). A number of systems are identified theoretically as promising ORR catalysts. The theoretical predictions are experimentally verified for the RhAu system, for which a specific surface ensemble is identified as being highly active in the ORR.
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Metrics
122
Total citations:
122
Citations from 2024:
6
(4%)
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MLA
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GOST
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Li H. et al. Oxygen Reduction Reaction on Classically Immiscible Bimetallics: A Case Study of RhAu // Journal of Physical Chemistry C. 2018. Vol. 122. No. 5. pp. 2712-2716.
GOST all authors (up to 50)
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Bonifacio C. S., Yang J. C. Oxygen Reduction Reaction on Classically Immiscible Bimetallics: A Case Study of RhAu // Journal of Physical Chemistry C. 2018. Vol. 122. No. 5. pp. 2712-2716.
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RIS
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TY - JOUR
DO - 10.1021/acs.jpcc.7b10974
UR - https://doi.org/10.1021/acs.jpcc.7b10974
TI - Oxygen Reduction Reaction on Classically Immiscible Bimetallics: A Case Study of RhAu
T2 - Journal of Physical Chemistry C
AU - Bonifacio, Cecile S
AU - Yang, Judith C
PY - 2018
DA - 2018/01/25
PB - American Chemical Society (ACS)
SP - 2712-2716
IS - 5
VL - 122
SN - 1932-7447
SN - 1932-7455
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Li,
author = {Cecile S Bonifacio and Judith C Yang},
title = {Oxygen Reduction Reaction on Classically Immiscible Bimetallics: A Case Study of RhAu},
journal = {Journal of Physical Chemistry C},
year = {2018},
volume = {122},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acs.jpcc.7b10974},
number = {5},
pages = {2712--2716},
doi = {10.1021/acs.jpcc.7b10974}
}
Cite this
MLA
Copy
Li, Hao, et al. “Oxygen Reduction Reaction on Classically Immiscible Bimetallics: A Case Study of RhAu.” Journal of Physical Chemistry C, vol. 122, no. 5, Jan. 2018, pp. 2712-2716. https://doi.org/10.1021/acs.jpcc.7b10974.