Co-Solvent Effect in the Processing of the Perovskite:Fullerene Blend Films for Electron Transport Layer-Free Solar Cells
Jorge Pascual
1, 2
,
Ivet Kosta
2
,
E. Palacios-Lidon
3
,
Andrey Chuvilin
4, 5
,
Giulia Grancini
6
,
M. Nazeeruddin
6
,
Hans J Grande
2, 7
,
Juan Luis Delgado
1, 5
,
1
IK4-CIDETEC, Parque Tecnológico de San Sebastián, Paseo Miramón 196, Donostia-San Sebastián 20009, Spain
|
2
Publication type: Journal Article
Publication date: 2018-01-30
scimago Q1
wos Q3
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
An understanding of the improvements achieved in the use of cosolvents for methylammonium lead triiodide (MAPbI3):C70 blend films (MAPbI3:C70) processing is presented. A comparative study using aromatic (i.e., o-xylene and o-dichlorobenzene) and aliphatic (i.e., methylcyclohexane and chlorocyclohexane) cosolvents proves the nature of the cosolvent interacting with fullerene to be determining for achieving enhanced devices. UV–vis spectra of the different C70 solutions suggest a major impact of the solute–aromatic solvent interactions on the optoelectronic properties. The effect of aromatic and aliphatic solvents in the electronic structure of C70 crystals, obtained from the different solutions, is indeed demonstrated by electron energy loss spectroscopy. Morphological studies show elimination of pinholes (field emission scanning electron microscopy) and different nanometric features related to fullerene (atomic force microscopy) in MAPbI3:C70 blend films processed using aromatic cosolvents. A severe quenc...
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Total citations:
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Citations from 2024:
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(9%)
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GOST
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Pascual J. et al. Co-Solvent Effect in the Processing of the Perovskite:Fullerene Blend Films for Electron Transport Layer-Free Solar Cells // Journal of Physical Chemistry C. 2018. Vol. 122. No. 5. pp. 2512-2520.
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Pascual J., Kosta I., Palacios-Lidon E., Chuvilin A., Grancini G., Nazeeruddin M., Grande H. J., Delgado J. L., Tena-Zaera R. Co-Solvent Effect in the Processing of the Perovskite:Fullerene Blend Films for Electron Transport Layer-Free Solar Cells // Journal of Physical Chemistry C. 2018. Vol. 122. No. 5. pp. 2512-2520.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.jpcc.7b11141
UR - https://doi.org/10.1021/acs.jpcc.7b11141
TI - Co-Solvent Effect in the Processing of the Perovskite:Fullerene Blend Films for Electron Transport Layer-Free Solar Cells
T2 - Journal of Physical Chemistry C
AU - Pascual, Jorge
AU - Kosta, Ivet
AU - Palacios-Lidon, E.
AU - Chuvilin, Andrey
AU - Grancini, Giulia
AU - Nazeeruddin, M.
AU - Grande, Hans J
AU - Delgado, Juan Luis
AU - Tena-Zaera, Ramon
PY - 2018
DA - 2018/01/30
PB - American Chemical Society (ACS)
SP - 2512-2520
IS - 5
VL - 122
SN - 1932-7447
SN - 1932-7455
ER -
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BibTex (up to 50 authors)
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@article{2018_Pascual,
author = {Jorge Pascual and Ivet Kosta and E. Palacios-Lidon and Andrey Chuvilin and Giulia Grancini and M. Nazeeruddin and Hans J Grande and Juan Luis Delgado and Ramon Tena-Zaera},
title = {Co-Solvent Effect in the Processing of the Perovskite:Fullerene Blend Films for Electron Transport Layer-Free Solar Cells},
journal = {Journal of Physical Chemistry C},
year = {2018},
volume = {122},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acs.jpcc.7b11141},
number = {5},
pages = {2512--2520},
doi = {10.1021/acs.jpcc.7b11141}
}
Cite this
MLA
Copy
Pascual, Jorge, et al. “Co-Solvent Effect in the Processing of the Perovskite:Fullerene Blend Films for Electron Transport Layer-Free Solar Cells.” Journal of Physical Chemistry C, vol. 122, no. 5, Jan. 2018, pp. 2512-2520. https://doi.org/10.1021/acs.jpcc.7b11141.