Swelling of Thin Graphene Oxide Films Studied by in Situ Neutron Reflectivity
Publication type: Journal Article
Publication date: 2018-05-24
scimago Q1
wos Q3
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
Permeation of multilayered graphene oxide (GO) membranes by polar solvents is known to correlate with their swelling properties and amount of sorbed solvent. However, quantitative estimation of sorption using standard (e.g., gravimetric) methods is technically challenging for few nanometers thick GO membranes/films exposed to solvent vapors. Neutron reflectivity (NR) was used here to evaluate the amount of solvents intercalated into the film which consists of only ∼31.5 layers of GO. Analysis of NR data recorded from the GO film exposed to vapors of polar solvents provides information about change of film thickness due to swelling, amount of intercalated solvent, and selectivity in sorption of solvents from binary mixtures. A quantitative study of GO film sorption was performed for D2O, d-methanol, ethanol, dimethyl sulfoxide (DMSO), acetonitrile, dimethylformamide (DMF), and acetone. Using isotopic contrast, we estimated selectivity in sorption of ethanol/d-methanol mixtures by the GO film. Estimation of...
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24
Total citations:
24
Citations from 2024:
5
(20.84%)
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GOST
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Klechikov A. et al. Swelling of Thin Graphene Oxide Films Studied by in Situ Neutron Reflectivity // Journal of Physical Chemistry C. 2018. Vol. 122. No. 24. pp. 13106-13116.
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Klechikov A., Sun J., Vorobiev A., Talyzin A. Swelling of Thin Graphene Oxide Films Studied by in Situ Neutron Reflectivity // Journal of Physical Chemistry C. 2018. Vol. 122. No. 24. pp. 13106-13116.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.jpcc.8b01616
UR - https://doi.org/10.1021/acs.jpcc.8b01616
TI - Swelling of Thin Graphene Oxide Films Studied by in Situ Neutron Reflectivity
T2 - Journal of Physical Chemistry C
AU - Klechikov, Alexey
AU - Sun, Jinhua
AU - Vorobiev, Alexei
AU - Talyzin, A.V.
PY - 2018
DA - 2018/05/24
PB - American Chemical Society (ACS)
SP - 13106-13116
IS - 24
VL - 122
SN - 1932-7447
SN - 1932-7455
ER -
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BibTex (up to 50 authors)
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@article{2018_Klechikov,
author = {Alexey Klechikov and Jinhua Sun and Alexei Vorobiev and A.V. Talyzin},
title = {Swelling of Thin Graphene Oxide Films Studied by in Situ Neutron Reflectivity},
journal = {Journal of Physical Chemistry C},
year = {2018},
volume = {122},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/acs.jpcc.8b01616},
number = {24},
pages = {13106--13116},
doi = {10.1021/acs.jpcc.8b01616}
}
Cite this
MLA
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Klechikov, Alexey, et al. “Swelling of Thin Graphene Oxide Films Studied by in Situ Neutron Reflectivity.” Journal of Physical Chemistry C, vol. 122, no. 24, May. 2018, pp. 13106-13116. https://doi.org/10.1021/acs.jpcc.8b01616.
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