New Type of Nanocrystalline Luminescent Thermometers Based on Ti3+/Ti4+ and Ti4+/Ln3+ (Ln3+ = Nd3+, Eu3+, Dy3+) Luminescence Intensity Ratio
Publication type: Journal Article
Publication date: 2018-06-12
scimago Q1
wos Q3
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
The spectroscopic properties of YAG:Ti and YAG:Ti,Ln nanocrystalline powders were examined as part of the search for new functional materials devoted to luminescent thermometry. Various temperature-dependent processes occurring in the studied systems were analyzed and the mechanism of absorption and emission of trivalent and tetravalent titanium ions was proposed. The first luminescent thermometer based on the Ti4+/Ti3+ luminescence intensity ratio with maximum sensitivity of 0.71% C–1 is shown. It was shown that the codoping with lanthanide ions enhances the relative sensitivity of YAG:Ti,Ln nanocrystalline luminescent thermometers because of the Ti4+ → Ln3+ energy transfer. The maximal relative sensitivities in the physiological range (2.26% C–1 at 50 °C) were found for YAG:Ti,Nd3+ nanocrystals and the value increases with temperature reaching 3.70% C–1 at 200 °C.
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Drabik J., Cichy B., Marciniak L. New Type of Nanocrystalline Luminescent Thermometers Based on Ti3+/Ti4+ and Ti4+/Ln3+ (Ln3+ = Nd3+, Eu3+, Dy3+) Luminescence Intensity Ratio // Journal of Physical Chemistry C. 2018. Vol. 122. No. 26. pp. 14928-14936.
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Drabik J., Cichy B., Marciniak L. New Type of Nanocrystalline Luminescent Thermometers Based on Ti3+/Ti4+ and Ti4+/Ln3+ (Ln3+ = Nd3+, Eu3+, Dy3+) Luminescence Intensity Ratio // Journal of Physical Chemistry C. 2018. Vol. 122. No. 26. pp. 14928-14936.
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TY - JOUR
DO - 10.1021/acs.jpcc.8b02328
UR - https://doi.org/10.1021/acs.jpcc.8b02328
TI - New Type of Nanocrystalline Luminescent Thermometers Based on Ti3+/Ti4+ and Ti4+/Ln3+ (Ln3+ = Nd3+, Eu3+, Dy3+) Luminescence Intensity Ratio
T2 - Journal of Physical Chemistry C
AU - Drabik, J
AU - Cichy, Bartłomiej
AU - Marciniak, Lukasz
PY - 2018
DA - 2018/06/12
PB - American Chemical Society (ACS)
SP - 14928-14936
IS - 26
VL - 122
SN - 1932-7447
SN - 1932-7455
ER -
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@article{2018_Drabik,
author = {J Drabik and Bartłomiej Cichy and Lukasz Marciniak},
title = {New Type of Nanocrystalline Luminescent Thermometers Based on Ti3+/Ti4+ and Ti4+/Ln3+ (Ln3+ = Nd3+, Eu3+, Dy3+) Luminescence Intensity Ratio},
journal = {Journal of Physical Chemistry C},
year = {2018},
volume = {122},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acs.jpcc.8b02328},
number = {26},
pages = {14928--14936},
doi = {10.1021/acs.jpcc.8b02328}
}
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Drabik, J., et al. “New Type of Nanocrystalline Luminescent Thermometers Based on Ti3+/Ti4+ and Ti4+/Ln3+ (Ln3+ = Nd3+, Eu3+, Dy3+) Luminescence Intensity Ratio.” Journal of Physical Chemistry C, vol. 122, no. 26, Jun. 2018, pp. 14928-14936. https://doi.org/10.1021/acs.jpcc.8b02328.
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