Unravelling the Material Composition Effects on the Gamma Ray Stability of Lead Halide Perovskite Solar Cells: MAPbI3 Breaks the Records
Lyubov A Frolova
2
,
I. S. ZHIDKOV
3
,
Lavrenty G Gutsev
2, 4
,
E. Z. Kurmaev
3, 5
,
Ernst Z Kurmaev
3, 5
,
S. M. Aldoshin
2
,
Sergey M. Aldoshin
2
,
Pavel A. Troshin
1, 2
4
Publication type: Journal Article
Publication date: 2020-03-17
scimago Q1
wos Q1
SJR: 1.394
CiteScore: 8.7
Impact factor: 4.6
ISSN: 19487185
PubMed ID:
32178515
Physical and Theoretical Chemistry
General Materials Science
Abstract
In this work, we report a comparative study of the gamma ray stability of perovskite solar cells based on a series of perovskite absorbers including MAPbI3 (MA = methylammonium), MAPbBr3, Cs0.15FA0.85PbI3 (FA = formamidinim), Cs0.1MA0.15FA0.75PbI3, CsPbI3, and CsPbBr3. We reveal that the composition of the perovskite material strongly affects the radiation stability of the solar cells. In particular, solar cells based on the MAPbI3 were found to be the most resistant to gamma rays since this perovskite undergoes rapid self-healing due to the special gas-phase chemistry analyzed with ab initio calculations. The fact that the solar cells based on MAPbI3 can withstand 1000 kRad gamma ray dose without any noticeable degradation of the photovoltaic properties) is particularly exciting and shifts the paradigm of research in this field towards designing more dynamic rather than intrinsically robust (e.g. inorganic) materials.
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Total citations:
56
Citations from 2024:
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(46.43%)
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Boldyreva A. G. et al. Unravelling the Material Composition Effects on the Gamma Ray Stability of Lead Halide Perovskite Solar Cells: MAPbI3 Breaks the Records // Journal of Physical Chemistry Letters. 2020. Vol. 11. No. 7. pp. 2630-2636.
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Boldyreva A. G., Frolova L. A., ZHIDKOV I. S., Gutsev L. G., Kurmaev E. Z., Kurmaev E. Z., Ramachandran B. R., Petrov V. G., Stevenson K. J., Aldoshin S. M., Aldoshin S. M., Troshin P. A. Unravelling the Material Composition Effects on the Gamma Ray Stability of Lead Halide Perovskite Solar Cells: MAPbI3 Breaks the Records // Journal of Physical Chemistry Letters. 2020. Vol. 11. No. 7. pp. 2630-2636.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.jpclett.0c00581
UR - https://pubs.acs.org/doi/10.1021/acs.jpclett.0c00581
TI - Unravelling the Material Composition Effects on the Gamma Ray Stability of Lead Halide Perovskite Solar Cells: MAPbI3 Breaks the Records
T2 - Journal of Physical Chemistry Letters
AU - Boldyreva, Aleksandra G
AU - Frolova, Lyubov A
AU - ZHIDKOV, I. S.
AU - Gutsev, Lavrenty G
AU - Kurmaev, E. Z.
AU - Kurmaev, Ernst Z
AU - Ramachandran, B. Ramu
AU - Petrov, Vladimir G
AU - Stevenson, Keith J
AU - Aldoshin, S. M.
AU - Aldoshin, Sergey M.
AU - Troshin, Pavel A.
PY - 2020
DA - 2020/03/17
PB - American Chemical Society (ACS)
SP - 2630-2636
IS - 7
VL - 11
PMID - 32178515
SN - 1948-7185
ER -
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BibTex (up to 50 authors)
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@article{2020_Boldyreva,
author = {Aleksandra G Boldyreva and Lyubov A Frolova and I. S. ZHIDKOV and Lavrenty G Gutsev and E. Z. Kurmaev and Ernst Z Kurmaev and B. Ramu Ramachandran and Vladimir G Petrov and Keith J Stevenson and S. M. Aldoshin and Sergey M. Aldoshin and Pavel A. Troshin},
title = {Unravelling the Material Composition Effects on the Gamma Ray Stability of Lead Halide Perovskite Solar Cells: MAPbI3 Breaks the Records},
journal = {Journal of Physical Chemistry Letters},
year = {2020},
volume = {11},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://pubs.acs.org/doi/10.1021/acs.jpclett.0c00581},
number = {7},
pages = {2630--2636},
doi = {10.1021/acs.jpclett.0c00581}
}
Cite this
MLA
Copy
Boldyreva, Aleksandra G., et al. “Unravelling the Material Composition Effects on the Gamma Ray Stability of Lead Halide Perovskite Solar Cells: MAPbI3 Breaks the Records.” Journal of Physical Chemistry Letters, vol. 11, no. 7, Mar. 2020, pp. 2630-2636. https://pubs.acs.org/doi/10.1021/acs.jpclett.0c00581.