volume 11 issue 15 pages 6456-6462

Gas-phase Synthesis and Characterisation of the Methyl-2,2-dicyanoacetate Anion Using Photoelectron Imaging and Dipole-bound State Autodetachment.

Publication typeJournal Article
Publication date2020-07-20
scimago Q1
wos Q1
SJR1.394
CiteScore8.7
Impact factor4.6
ISSN19487185
Physical and Theoretical Chemistry
General Materials Science
Abstract
The methyl-2,2-dicyanoacetate anion is synthesised in an electrospray ionisation source through a gas-phase reaction involving tetracyanoethylene and methanol. Photoelectron imaging is used to determine the isomeric form of the product. The photoelectron spectra and angular distributions are only consistent with a single isomer. Additionally, mode-specific vibrational autodetachment is observed. This can be correlated with the emission from a photoexcited dipole-bound state by considering the IR spectrum of the neutral molecule, adding further confirmation of the isomeric form and providing a binding energy of the dipole-bound state. Our experiments show how conventional photoelectron imaging can be used to determine detailed information about gas-phase reaction products.
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Anstöter C. S., Verlet J. R. Gas-phase Synthesis and Characterisation of the Methyl-2,2-dicyanoacetate Anion Using Photoelectron Imaging and Dipole-bound State Autodetachment. // Journal of Physical Chemistry Letters. 2020. Vol. 11. No. 15. pp. 6456-6462.
GOST all authors (up to 50) Copy
Anstöter C. S., Verlet J. R. Gas-phase Synthesis and Characterisation of the Methyl-2,2-dicyanoacetate Anion Using Photoelectron Imaging and Dipole-bound State Autodetachment. // Journal of Physical Chemistry Letters. 2020. Vol. 11. No. 15. pp. 6456-6462.
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TY - JOUR
DO - 10.1021/acs.jpclett.0c02036
UR - https://doi.org/10.1021/acs.jpclett.0c02036
TI - Gas-phase Synthesis and Characterisation of the Methyl-2,2-dicyanoacetate Anion Using Photoelectron Imaging and Dipole-bound State Autodetachment.
T2 - Journal of Physical Chemistry Letters
AU - Anstöter, Cate S.
AU - Verlet, Jan R. R.
PY - 2020
DA - 2020/07/20
PB - American Chemical Society (ACS)
SP - 6456-6462
IS - 15
VL - 11
PMID - 32687376
SN - 1948-7185
ER -
BibTex |
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BibTex (up to 50 authors) Copy
@article{2020_Anstöter,
author = {Cate S. Anstöter and Jan R. R. Verlet},
title = {Gas-phase Synthesis and Characterisation of the Methyl-2,2-dicyanoacetate Anion Using Photoelectron Imaging and Dipole-bound State Autodetachment.},
journal = {Journal of Physical Chemistry Letters},
year = {2020},
volume = {11},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/acs.jpclett.0c02036},
number = {15},
pages = {6456--6462},
doi = {10.1021/acs.jpclett.0c02036}
}
MLA
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Anstöter, Cate S., and Jan R. R. Verlet. “Gas-phase Synthesis and Characterisation of the Methyl-2,2-dicyanoacetate Anion Using Photoelectron Imaging and Dipole-bound State Autodetachment..” Journal of Physical Chemistry Letters, vol. 11, no. 15, Jul. 2020, pp. 6456-6462. https://doi.org/10.1021/acs.jpclett.0c02036.