Sb3+ Doping-Induced Triplet Self-Trapped Excitons Emission in Lead-Free Cs2SnCl6 Nanocrystals.
Тип публикации: Journal Article
Дата публикации: 2019-11-15
scimago Q1
wos Q1
white level БС1
SJR: 1.394
CiteScore: 8.7
Impact factor: 4.6
ISSN: 19487185
PubMed ID:
31726830
Physical and Theoretical Chemistry
General Materials Science
Краткое описание
Doped halide perovskite nanocrystals (NCs) have opened new opportunities for the emerging optical and optoelectronic applications. Here, we describe a hot-injection synthesis of all-inorganic lead-free Cs2SnCl6 and Sb3+ doped Cs2SnCl6 NCs. Cs2SnCl6 NCs present a blue emission peak at 438 nm, whereas a new broad-band emission peak appears at 615 nm for the Sb3+ doped NCs. A comparative structural and spectral characterizations of Sb3+ doped Cs2SnCl6 NCs with micrometer-sized undoped and Sb3+ doped crystals show that the formation of broadband orange emission is originted from triplet self-trapped excitons, attributed to the 3Pn - 1S0 transitions ( n = 0, 1, 2). Our results in Sb3+ doped Cs2SnCl6 materials provides insights into the machanisms of doping-induced emission centers, and it extends the existing knowledge of optical properties of doped halide NCs for further studies.
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Jing Y. et al. Sb3+ Doping-Induced Triplet Self-Trapped Excitons Emission in Lead-Free Cs2SnCl6 Nanocrystals. // Journal of Physical Chemistry Letters. 2019. Vol. 10. No. 23. pp. 7439-7444.
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Jing Y., Liu Y., Zhao J., Xia Z. Sb3+ Doping-Induced Triplet Self-Trapped Excitons Emission in Lead-Free Cs2SnCl6 Nanocrystals. // Journal of Physical Chemistry Letters. 2019. Vol. 10. No. 23. pp. 7439-7444.
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TY - JOUR
DO - 10.1021/acs.jpclett.9b03035
UR - https://doi.org/10.1021/acs.jpclett.9b03035
TI - Sb3+ Doping-Induced Triplet Self-Trapped Excitons Emission in Lead-Free Cs2SnCl6 Nanocrystals.
T2 - Journal of Physical Chemistry Letters
AU - Jing, Yuyu
AU - Liu, Ying
AU - Zhao, Jing
AU - Xia, Zhiguo
PY - 2019
DA - 2019/11/15
PB - American Chemical Society (ACS)
SP - 7439-7444
IS - 23
VL - 10
PMID - 31726830
SN - 1948-7185
ER -
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@article{2019_Jing,
author = {Yuyu Jing and Ying Liu and Jing Zhao and Zhiguo Xia},
title = {Sb3+ Doping-Induced Triplet Self-Trapped Excitons Emission in Lead-Free Cs2SnCl6 Nanocrystals.},
journal = {Journal of Physical Chemistry Letters},
year = {2019},
volume = {10},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/acs.jpclett.9b03035},
number = {23},
pages = {7439--7444},
doi = {10.1021/acs.jpclett.9b03035}
}
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MLA
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Jing, Yuyu, et al. “Sb3+ Doping-Induced Triplet Self-Trapped Excitons Emission in Lead-Free Cs2SnCl6 Nanocrystals..” Journal of Physical Chemistry Letters, vol. 10, no. 23, Nov. 2019, pp. 7439-7444. https://doi.org/10.1021/acs.jpclett.9b03035.
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