Edge-Rich Black Phosphorus for Photocatalytic Nitrogen Fixation
Publication type: Journal Article
Publication date: 2020-01-17
scimago Q1
wos Q1
SJR: 1.394
CiteScore: 8.7
Impact factor: 4.6
ISSN: 19487185
PubMed ID:
31952439
Physical and Theoretical Chemistry
General Materials Science
Abstract
Development of efficient catalysts for ammonia production under ambient conditions is a challenge. In this work, edge-rich black phosphorus nanoflakes (eBP NFs) are synthesized for highly efficient photocatalytic nitrogen fixation. The eBP NFs synthesized by a chemical etching exfoliation method have a uniform size and about 90 nm wide and the flake-like structure is enshrouded with crystal-domain edges. Without using any cocatalysts, the eBP NFs catalyze nitrogen fixation at a rate of 2.37 mmol·h-1·g-1 under visible-light irradiation. The photocatalytic process is analyzed by photoelectrochemical and transient absorption measurements, which disclose electron transfer from eBP NFs to N2 for subsequent hydrogenation. Besides the facile and scalable synthesis method, eBP NFs with a high photocatalytic nitrogen fixation efficiency have great potential in ammonia production.
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Metrics
74
Total citations:
74
Citations from 2025:
12
(16.22%)
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GOST
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Bian S. et al. Edge-Rich Black Phosphorus for Photocatalytic Nitrogen Fixation // Journal of Physical Chemistry Letters. 2020. Vol. 11. No. 3. pp. 1052-1058.
GOST all authors (up to 50)
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Bian S., Wen M., Wang J., Yang N., Chu P. K., Yu X. Edge-Rich Black Phosphorus for Photocatalytic Nitrogen Fixation // Journal of Physical Chemistry Letters. 2020. Vol. 11. No. 3. pp. 1052-1058.
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RIS
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TY - JOUR
DO - 10.1021/acs.jpclett.9b03507
UR - https://doi.org/10.1021/acs.jpclett.9b03507
TI - Edge-Rich Black Phosphorus for Photocatalytic Nitrogen Fixation
T2 - Journal of Physical Chemistry Letters
AU - Bian, Shi
AU - Wen, Min
AU - Wang, Jiahong
AU - Yang, Na
AU - Chu, Paul K.
AU - Yu, Xue-Feng
PY - 2020
DA - 2020/01/17
PB - American Chemical Society (ACS)
SP - 1052-1058
IS - 3
VL - 11
PMID - 31952439
SN - 1948-7185
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2020_Bian,
author = {Shi Bian and Min Wen and Jiahong Wang and Na Yang and Paul K. Chu and Xue-Feng Yu},
title = {Edge-Rich Black Phosphorus for Photocatalytic Nitrogen Fixation},
journal = {Journal of Physical Chemistry Letters},
year = {2020},
volume = {11},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acs.jpclett.9b03507},
number = {3},
pages = {1052--1058},
doi = {10.1021/acs.jpclett.9b03507}
}
Cite this
MLA
Copy
Bian, Shi, et al. “Edge-Rich Black Phosphorus for Photocatalytic Nitrogen Fixation.” Journal of Physical Chemistry Letters, vol. 11, no. 3, Jan. 2020, pp. 1052-1058. https://doi.org/10.1021/acs.jpclett.9b03507.