For Whom a Puddle Is the Sea? Adsorption of Organic Guests on Hydrated MCM-41 Silica
Publication type: Journal Article
Publication date: 2020-09-08
scimago Q1
wos Q2
SJR: 0.763
CiteScore: 6.0
Impact factor: 3.9
ISSN: 07437463, 15205827
PubMed ID:
32900200
Spectroscopy
Electrochemistry
Condensed Matter Physics
General Materials Science
Surfaces and Interfaces
Abstract
Thermal and hydration effects on the mobility of compact and branched organic molecules and a bulky pharmaceutical substance loaded in submonolayer amounts onto mesoporous silica have been elucidated using 1H and 31P solid-state NMR. In all cases, the ambient hydration has a stronger effect than an increase in temperature to 370 K for water-free silica. The effect of hydration depends on the guest and ranges from complete solvation to a silica-water-guest sandwich structure to a silica-guest/silica-water pattern. The mobility of the guests under different conditions has been described. The specific structure of the MCM-41 surface allows one to study very slow surface diffusion, a diffusivity of about 10-15-10-16 m2/s. The data reported are relevant to any nonfunctionalized silica, while the method used is applicable to any phosphor-containing guest on any host.
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Total citations:
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Citations from 2024:
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GOST
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Shenderovich I. G. For Whom a Puddle Is the Sea? Adsorption of Organic Guests on Hydrated MCM-41 Silica // Langmuir. 2020. Vol. 36. No. 38. pp. 11383-11392.
GOST all authors (up to 50)
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Shenderovich I. G. For Whom a Puddle Is the Sea? Adsorption of Organic Guests on Hydrated MCM-41 Silica // Langmuir. 2020. Vol. 36. No. 38. pp. 11383-11392.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.langmuir.0c02327
UR - https://doi.org/10.1021/acs.langmuir.0c02327
TI - For Whom a Puddle Is the Sea? Adsorption of Organic Guests on Hydrated MCM-41 Silica
T2 - Langmuir
AU - Shenderovich, Ilya G.
PY - 2020
DA - 2020/09/08
PB - American Chemical Society (ACS)
SP - 11383-11392
IS - 38
VL - 36
PMID - 32900200
SN - 0743-7463
SN - 1520-5827
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2020_Shenderovich,
author = {Ilya G. Shenderovich},
title = {For Whom a Puddle Is the Sea? Adsorption of Organic Guests on Hydrated MCM-41 Silica},
journal = {Langmuir},
year = {2020},
volume = {36},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/acs.langmuir.0c02327},
number = {38},
pages = {11383--11392},
doi = {10.1021/acs.langmuir.0c02327}
}
Cite this
MLA
Copy
Shenderovich, Ilya G.. “For Whom a Puddle Is the Sea? Adsorption of Organic Guests on Hydrated MCM-41 Silica.” Langmuir, vol. 36, no. 38, Sep. 2020, pp. 11383-11392. https://doi.org/10.1021/acs.langmuir.0c02327.
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