Macromolecules

, volume 50 , issue 19 , pages 7559-7566

Fused Perylene Diimide-Based Polymeric Acceptors for Efficient All-Polymer Solar Cells

Ming Liu ^{1, 2}

Jing Yang ³

Caili Lang ¹

Yong Zhang ¹

Erjun Zhou ³

Zhitian Liu ²

Fengyun Guo ¹

Liancheng Zhao ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

School of Materials Science and Engineering, Harbin Institute of Technology, Harbin 150001, China |

School of Materials Science and Engineering, Wuhan Institute of Technology, Wuhan 430073, China |

CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China |

Publication type: Journal Article

Publication date: 2017-09-29

American Chemical Society (ACS)

Macromolecules

scimago Q1

wos Q1

SJR: 1.352

CiteScore: 9.0

Impact factor: 5.2

ISSN: 00249297, 15205835

DOI: 10.1021/acs.macromol.7b01539

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Materials Chemistry

Organic Chemistry

Inorganic Chemistry

Polymers and Plastics

Abstract

Two polymeric electron acceptors (PFPDI-2T and PFPDI-2FT) based on the fused perylene diimide (PDI) and bithiophene or difluorobithiophene units were synthesized via the Stille polymerization. Both polymers exhibit the strong absorption between 350 and 650 nm, which have the good absorption compensation with the low band gap conjugated polymer in polymer solar cells (PSCs). PFPDI-2T and PFPDI-2FT have the LUMO energy levels of around −4.12 to −4.15 eV, which are comparable with other PDI-based polymers and fullerene derivatives. All-polymer solar cells (all-PSCs) based on PFPDI-2T or PFPDI-2FT as the polymeric electron acceptor were fabricated with PTB7-Th as the polymeric electron donor. Power conversion efficiency of as high as 6.39% based on PFPDI-2T/PTB7-Th was achieved under the standard illumination of simulated sunlight (AM 1.5, 100 mW cm–2), which is significant higher than that of the all-PSC based on the nonfused PDI counterpart. The results demonstrate that the direct fusion of PDI unit is an e...

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GOST |

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GOST Copy

Liu M. et al. Fused Perylene Diimide-Based Polymeric Acceptors for Efficient All-Polymer Solar Cells // Macromolecules. 2017. Vol. 50. No. 19. pp. 7559-7566.

GOST all authors (up to 50) Copy

Liu M., Yang J., Lang C., Zhang Y., Zhou E., Liu Z., Guo F., Zhao L. Fused Perylene Diimide-Based Polymeric Acceptors for Efficient All-Polymer Solar Cells // Macromolecules. 2017. Vol. 50. No. 19. pp. 7559-7566.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acs.macromol.7b01539

UR - https://doi.org/10.1021/acs.macromol.7b01539

TI - Fused Perylene Diimide-Based Polymeric Acceptors for Efficient All-Polymer Solar Cells

T2 - Macromolecules

AU - Liu, Ming

AU - Yang, Jing

AU - Lang, Caili

AU - Zhang, Yong

AU - Zhou, Erjun

AU - Liu, Zhitian

AU - Guo, Fengyun

AU - Zhao, Liancheng

PY - 2017

DA - 2017/09/29

PB - American Chemical Society (ACS)

SP - 7559-7566

IS - 19

VL - 50

SN - 0024-9297

SN - 1520-5835

ER -

BibTex |

Cite this

BibTex (up to 50 authors) Copy

@article{2017_Liu,

author = {Ming Liu and Jing Yang and Caili Lang and Yong Zhang and Erjun Zhou and Zhitian Liu and Fengyun Guo and Liancheng Zhao},

title = {Fused Perylene Diimide-Based Polymeric Acceptors for Efficient All-Polymer Solar Cells},

journal = {Macromolecules},

year = {2017},

volume = {50},

publisher = {American Chemical Society (ACS)},

month = {sep},

url = {https://doi.org/10.1021/acs.macromol.7b01539},

number = {19},

pages = {7559--7566},

doi = {10.1021/acs.macromol.7b01539}

}

MLA

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MLA Copy

Liu, Ming, et al. “Fused Perylene Diimide-Based Polymeric Acceptors for Efficient All-Polymer Solar Cells.” Macromolecules, vol. 50, no. 19, Sep. 2017, pp. 7559-7566. https://doi.org/10.1021/acs.macromol.7b01539.

Publisher

American Chemical Society (ACS)

Journal

Macromolecules

scimago Q1

wos Q1

SJR

1.352

CiteScore

9.0

Impact factor

5.2

ISSN

00249297 (Print)

15205835 (Electronic)

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