Side Chain Effects on the Optoelectronic Properties and Self-Assembly Behaviors of Terthiophene–Thieno[3,4-c]pyrrole-4,6-dione Based Conjugated Polymers
Publication type: Journal Article
Publication date: 2018-09-26
scimago Q1
wos Q1
SJR: 1.352
CiteScore: 9.0
Impact factor: 5.2
ISSN: 00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Abstract
The donor–acceptor conjugated polymers (CPs) of terthiophene–thieno[3,4-c]pyrrole-4,6-dione (3T-TPD) are widely used to fabricate low-cost flexible electronics. We present a comprehensive study of the side chain effect on the optical properties, electrochemical properties, thermal properties, and self-assembly behavior of 3T-TPD CPs, including side chain location (outward vs inward), type (tetraethylene glycol (TEG) vs dodecyl), and length (octyl vs hexyl vs butyl). For the side chain location effect, the polymers with outward side chains show better coplanarity of backbone than the polymers with inward side chains, leading to form lamellae structure. However, interestingly, the inward series polymers exhibit novel hexagonal structure. Through replacing dodecyl chains with TEG chains and changing the side chain length, ultrahigh ordered lamellae and hexagonal structure can be obtained. Furthermore, two models are purposed to explain the formation mechanism of lamellae and hexagonal structure. This study c...
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Total citations:
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Citations from 2024:
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Chen C. et al. Side Chain Effects on the Optoelectronic Properties and Self-Assembly Behaviors of Terthiophene–Thieno[3,4-c]pyrrole-4,6-dione Based Conjugated Polymers // Macromolecules. 2018. Vol. 51. No. 19. pp. 7828-7835.
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Chen C., Yang P., Wang S., Tung S. P., Su W. Side Chain Effects on the Optoelectronic Properties and Self-Assembly Behaviors of Terthiophene–Thieno[3,4-c]pyrrole-4,6-dione Based Conjugated Polymers // Macromolecules. 2018. Vol. 51. No. 19. pp. 7828-7835.
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TY - JOUR
DO - 10.1021/acs.macromol.8b01073
UR - https://doi.org/10.1021/acs.macromol.8b01073
TI - Side Chain Effects on the Optoelectronic Properties and Self-Assembly Behaviors of Terthiophene–Thieno[3,4-c]pyrrole-4,6-dione Based Conjugated Polymers
T2 - Macromolecules
AU - Chen, Chien-An
AU - Yang, Po-Chih
AU - Wang, Shih-Chieh
AU - Tung, Shih Ping
AU - Su, Wei-Fang
PY - 2018
DA - 2018/09/26
PB - American Chemical Society (ACS)
SP - 7828-7835
IS - 19
VL - 51
SN - 0024-9297
SN - 1520-5835
ER -
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BibTex (up to 50 authors)
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@article{2018_Chen,
author = {Chien-An Chen and Po-Chih Yang and Shih-Chieh Wang and Shih Ping Tung and Wei-Fang Su},
title = {Side Chain Effects on the Optoelectronic Properties and Self-Assembly Behaviors of Terthiophene–Thieno[3,4-c]pyrrole-4,6-dione Based Conjugated Polymers},
journal = {Macromolecules},
year = {2018},
volume = {51},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/acs.macromol.8b01073},
number = {19},
pages = {7828--7835},
doi = {10.1021/acs.macromol.8b01073}
}
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Chen, Chien-An, et al. “Side Chain Effects on the Optoelectronic Properties and Self-Assembly Behaviors of Terthiophene–Thieno[3,4-c]pyrrole-4,6-dione Based Conjugated Polymers.” Macromolecules, vol. 51, no. 19, Sep. 2018, pp. 7828-7835. https://doi.org/10.1021/acs.macromol.8b01073.
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