In Situ Formation of Polycyclic Aromatic Hydrocarbons as an Artificial Hybrid Layer for Lithium Metal Anodes
Shaozhong Chang
1
,
Xin Jin
1
,
Qiya He
2
,
Tiefeng Liu
3
,
Jiabin Fang
1
,
Z. Shen
1
,
Zhengcao Li
1
,
Shuo Zhang
1
,
Mouad Dahbi
4
,
Jones Alami
4
,
Khalil Amine
3
,
Ai-dong Li
1
,
Huigang Zhang
1, 2, 5
,
Jun Lu
3
1
Publication type: Journal Article
Publication date: 2021-12-14
scimago Q1
wos Q1
SJR: 2.967
CiteScore: 14.9
Impact factor: 9.1
ISSN: 15306984, 15306992
PubMed ID:
34905368
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
Nonuniform Li deposition causes dendrites and low Coulombic efficiency (CE), seriously hindering the practical applications of Li metal. Herein, we developed an artificial solid-state interphase (SEI) with planar polycyclic aromatic hydrocarbons (PAHs) on the surface of Li metal anodes by a facile in situ formation technology. The resultant dihydroxyviolanthron (DHV) layers serve as the protective layer to stabilize the SEI. In addition, the oxygen-containing functional groups in the soft and conformal SEI film can regulate the diffusion and transport of Li ions to homogenize the deposition of Li metal. The artificial SEI significantly improves the CEs and shows superior cyclability of over 1000 h at 4 mAh cm-2. The LiFePO4/Li cell (2.8 mAh cm-2) enables a long cyclability for 300 cycles and high CEs of 99.8%. This work offers a new strategy to inhibit Li dendrite growth and enlightens the design on stable SEI for metal anodes.
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54
Total citations:
54
Citations from 2024:
23
(42.59%)
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GOST
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Chang S. et al. In Situ Formation of Polycyclic Aromatic Hydrocarbons as an Artificial Hybrid Layer for Lithium Metal Anodes // Nano Letters. 2021. Vol. 22. No. 1. pp. 263-270.
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Chang S., Jin X., He Q., Liu T., Fang J., Shen Z., Li Z., Zhang S., Dahbi M., Alami J., Amine K., Li A., Zhang H., Lu J. In Situ Formation of Polycyclic Aromatic Hydrocarbons as an Artificial Hybrid Layer for Lithium Metal Anodes // Nano Letters. 2021. Vol. 22. No. 1. pp. 263-270.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.nanolett.1c03624
UR - https://doi.org/10.1021/acs.nanolett.1c03624
TI - In Situ Formation of Polycyclic Aromatic Hydrocarbons as an Artificial Hybrid Layer for Lithium Metal Anodes
T2 - Nano Letters
AU - Chang, Shaozhong
AU - Jin, Xin
AU - He, Qiya
AU - Liu, Tiefeng
AU - Fang, Jiabin
AU - Shen, Z.
AU - Li, Zhengcao
AU - Zhang, Shuo
AU - Dahbi, Mouad
AU - Alami, Jones
AU - Amine, Khalil
AU - Li, Ai-dong
AU - Zhang, Huigang
AU - Lu, Jun
PY - 2021
DA - 2021/12/14
PB - American Chemical Society (ACS)
SP - 263-270
IS - 1
VL - 22
PMID - 34905368
SN - 1530-6984
SN - 1530-6992
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2021_Chang,
author = {Shaozhong Chang and Xin Jin and Qiya He and Tiefeng Liu and Jiabin Fang and Z. Shen and Zhengcao Li and Shuo Zhang and Mouad Dahbi and Jones Alami and Khalil Amine and Ai-dong Li and Huigang Zhang and Jun Lu},
title = {In Situ Formation of Polycyclic Aromatic Hydrocarbons as an Artificial Hybrid Layer for Lithium Metal Anodes},
journal = {Nano Letters},
year = {2021},
volume = {22},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/acs.nanolett.1c03624},
number = {1},
pages = {263--270},
doi = {10.1021/acs.nanolett.1c03624}
}
Cite this
MLA
Copy
Chang, Shaozhong, et al. “In Situ Formation of Polycyclic Aromatic Hydrocarbons as an Artificial Hybrid Layer for Lithium Metal Anodes.” Nano Letters, vol. 22, no. 1, Dec. 2021, pp. 263-270. https://doi.org/10.1021/acs.nanolett.1c03624.
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