Submillisecond Spin Relaxation in CsPb(Cl,Br)3 Perovskite Nanocrystals in a Glass Matrix
2
Publication type: Journal Article
Publication date: 2022-05-27
scimago Q1
wos Q1
SJR: 2.967
CiteScore: 14.9
Impact factor: 9.1
ISSN: 15306984, 15306992
PubMed ID:
35621509
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
Lead halide perovskite nanocrystals in a glass matrix are a promising platform for optoelectronic applications due to their excellent optical properties combined with outstanding stability against the environment. We reveal the potential of this system for spintronics by studying the electron spin properties of CsPb(Cl,Br)3 nanocrystals in a fluorophosphate glass matrix. Using optical spin orientation and spin depolarization with a radio frequency field, we measure longitudinal spin relaxation time, T1, reaching several hundreds of microseconds at low temperatures. This time T1 corresponds to a spin state with a small g factor, which we attribute to a weakly exchange-coupled electron-hole pair with antiparallel spins.
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19
Total citations:
19
Citations from 2024:
13
(68.42%)
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GOST
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Belykh V. et al. Submillisecond Spin Relaxation in CsPb(Cl,Br)3 Perovskite Nanocrystals in a Glass Matrix // Nano Letters. 2022. Vol. 22. No. 11. pp. 4583-4588.
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Belykh V., Skorikov M. L., Kulebyakina E. V., Kolobkova E. V., Kuznetsova M. S., Glazov M. M., Yakovlev D. G. Submillisecond Spin Relaxation in CsPb(Cl,Br)3 Perovskite Nanocrystals in a Glass Matrix // Nano Letters. 2022. Vol. 22. No. 11. pp. 4583-4588.
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RIS
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TY - JOUR
DO - 10.1021/acs.nanolett.2c01673
UR - https://doi.org/10.1021/acs.nanolett.2c01673
TI - Submillisecond Spin Relaxation in CsPb(Cl,Br)3 Perovskite Nanocrystals in a Glass Matrix
T2 - Nano Letters
AU - Belykh, V. V.
AU - Skorikov, Mikhail L
AU - Kulebyakina, Evgeniya V
AU - Kolobkova, Elena V.
AU - Kuznetsova, Maria S
AU - Glazov, Mikhail M.
AU - Yakovlev, D G
PY - 2022
DA - 2022/05/27
PB - American Chemical Society (ACS)
SP - 4583-4588
IS - 11
VL - 22
PMID - 35621509
SN - 1530-6984
SN - 1530-6992
ER -
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BibTex (up to 50 authors)
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@article{2022_Belykh,
author = {V. V. Belykh and Mikhail L Skorikov and Evgeniya V Kulebyakina and Elena V. Kolobkova and Maria S Kuznetsova and Mikhail M. Glazov and D G Yakovlev},
title = {Submillisecond Spin Relaxation in CsPb(Cl,Br)3 Perovskite Nanocrystals in a Glass Matrix},
journal = {Nano Letters},
year = {2022},
volume = {22},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/acs.nanolett.2c01673},
number = {11},
pages = {4583--4588},
doi = {10.1021/acs.nanolett.2c01673}
}
Cite this
MLA
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Belykh, V. V., et al. “Submillisecond Spin Relaxation in CsPb(Cl,Br)3 Perovskite Nanocrystals in a Glass Matrix.” Nano Letters, vol. 22, no. 11, May. 2022, pp. 4583-4588. https://doi.org/10.1021/acs.nanolett.2c01673.