Nano Letters, volume 17, issue 5, pages 2967-2972

Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li₇La₃Zr₂O₁₂/Carbon Foam and Polymer

Jianmin Luo ^{1, 2}

Yayuan Liu ²

Wei Liu ²

Guangmin Zhou ²

Jie Zhao ²

Chenxi Zu ²

Ouwei Sheng ¹

Wenkui Zhang ¹

Hyun-Wook Lee ²

Yi Cui ^{2, 3}

Hide authors affiliations Show authors affiliations: 3 affiliations

College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China |

Department of Materials Science and Engineering, Stanford University, Stanford, California 94305, United States |

Stanford Institute for Materials and Energy Science, SLAC National Accelerator Laboratory, Menlo Park, California 94025, United States |

Publication type: Journal Article

Publication date: 2017-04-12

American Chemical Society (ACS)

Journal: Nano Letters

Quartile SCImago

Quartile WOS

Impact factor: 10.8

ISSN: 15306984, 15306992

DOI: 10.1021/acs.nanolett.7b00221

Copy DOI

General Chemistry

Condensed Matter Physics

General Materials Science

Mechanical Engineering

Bioengineering

Abstract

An all solid-state lithium-ion battery with high energy density and high safety is a promising solution for a next-generation energy storage system. High interface resistance of the electrodes and poor ion conductivity of solid-state electrolytes are two main challenges for solid-state batteries, which require operation at elevated temperatures of 60-90 °C. Herein, we report the facile synthesis of Al3+/Nb5+ codoped cubic Li7La3Zr2O12 (LLZO) nanoparticles and LLZO nanoparticle-decorated porous carbon foam (LLZO@C) by the one-step Pechini sol-gel method. The LLZO nanoparticle-filled poly(ethylene oxide) electrolyte shows improved conductivity compared with filler-free samples. The sulfur composite cathode based on LLZO@C can deliver an attractive specific capacity of >900 mAh g-1 at the human body temperature 37 °C and a high capacity of 1210 and 1556 mAh g-1 at 50 and 70 °C, respectively. In addition, the solid-state Li-S batteries exhibit high Coulombic efficiency and show remarkably stable cycling performance.

By date By citations

Top-30

Citations by journals

	5 10 15 20 25
Energy Storage Materials	Energy Storage Materials, 23, 5.76% Energy Storage Materials 23 publications, 5.76%
Advanced Energy Materials	Advanced Energy Materials, 20, 5.01% Advanced Energy Materials 20 publications, 5.01%
ACS applied materials & interfaces	ACS applied materials & interfaces, 18, 4.51% ACS applied materials & interfaces 18 publications, 4.51%
Journal of Power Sources	Journal of Power Sources, 15, 3.76% Journal of Power Sources 15 publications, 3.76%
Small	Small, 13, 3.26% Small 13 publications, 3.26%
Chemical Engineering Journal	Chemical Engineering Journal, 12, 3.01% Chemical Engineering Journal 12 publications, 3.01%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 12, 3.01% Journal of Materials Chemistry A 12 publications, 3.01%
Nano Letters	Nano Letters, 11, 2.76% Nano Letters 11 publications, 2.76%
Journal of Energy Chemistry	Journal of Energy Chemistry, 11, 2.76% Journal of Energy Chemistry 11 publications, 2.76%
Advanced Functional Materials	Advanced Functional Materials, 11, 2.76% Advanced Functional Materials 11 publications, 2.76%
Energy and Environmental Science	Energy and Environmental Science, 10, 2.51% Energy and Environmental Science 10 publications, 2.51%
Advanced Materials	Advanced Materials, 9, 2.26% Advanced Materials 9 publications, 2.26%
Nano Energy	Nano Energy, 8, 2.01% Nano Energy 8 publications, 2.01%
ACS Applied Energy Materials	ACS Applied Energy Materials, 8, 2.01% ACS Applied Energy Materials 8 publications, 2.01%
Ionics	Ionics, 5, 1.25% Ionics 5 publications, 1.25%
Electrochimica Acta	Electrochimica Acta, 5, 1.25% Electrochimica Acta 5 publications, 1.25%
Chemical Reviews	Chemical Reviews, 5, 1.25% Chemical Reviews 5 publications, 1.25%
Nano-Micro Letters	Nano-Micro Letters, 4, 1% Nano-Micro Letters 4 publications, 1%
Electrochemical Energy Reviews	Electrochemical Energy Reviews, 4, 1% Electrochemical Energy Reviews 4 publications, 1%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 4, 1% Journal of Alloys and Compounds 4 publications, 1%
Advanced Science	Advanced Science, 4, 1% Advanced Science 4 publications, 1%
Chemistry - A European Journal	Chemistry - A European Journal, 4, 1% Chemistry - A European Journal 4 publications, 1%
Batteries & Supercaps	Batteries & Supercaps, 4, 1% Batteries & Supercaps 4 publications, 1%
Energy & Fuels	Energy & Fuels, 4, 1% Energy & Fuels 4 publications, 1%
Journal of Energy Storage	Journal of Energy Storage, 4, 1% Journal of Energy Storage 4 publications, 1%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 3, 0.75% Journal of the Electrochemical Society 3 publications, 0.75%
Nanomaterials	Nanomaterials, 3, 0.75% Nanomaterials 3 publications, 0.75%
Journal of Materials Science	Journal of Materials Science, 3, 0.75% Journal of Materials Science 3 publications, 0.75%
Rare Metals	Rare Metals, 3, 0.75% Rare Metals 3 publications, 0.75%
	5 10 15 20 25

Citations by publishers

	20 40 60 80 100 120 140
Elsevier	Elsevier, 127, 31.83% Elsevier 127 publications, 31.83%
Wiley	Wiley, 95, 23.81% Wiley 95 publications, 23.81%
American Chemical Society (ACS)	American Chemical Society (ACS), 60, 15.04% American Chemical Society (ACS) 60 publications, 15.04%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 40, 10.03% Royal Society of Chemistry (RSC) 40 publications, 10.03%
Springer Nature	Springer Nature, 30, 7.52% Springer Nature 30 publications, 7.52%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 7, 1.75% Multidisciplinary Digital Publishing Institute (MDPI) 7 publications, 1.75%
Frontiers Media S.A.	Frontiers Media S.A., 4, 1% Frontiers Media S.A. 4 publications, 1%
The Electrochemical Society	The Electrochemical Society, 3, 0.75% The Electrochemical Society 3 publications, 0.75%
Tsinghua University Press	Tsinghua University Press, 2, 0.5% Tsinghua University Press 2 publications, 0.5%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 2, 0.5% Nonferrous Metals Society of China 2 publications, 0.5%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 2, 0.5% Proceedings of the National Academy of Sciences (PNAS) 2 publications, 0.5%
Bentham Science	Bentham Science, 1, 0.25% Bentham Science 1 publication, 0.25%
Higher Education Press	Higher Education Press, 1, 0.25% Higher Education Press 1 publication, 0.25%
World Scientific	World Scientific, 1, 0.25% World Scientific 1 publication, 0.25%
Ceramic Society of Japan	Ceramic Society of Japan, 1, 0.25% Ceramic Society of Japan 1 publication, 0.25%
Chinese Academy of Sciences	Chinese Academy of Sciences, 1, 0.25% Chinese Academy of Sciences 1 publication, 0.25%
IOP Publishing	IOP Publishing, 1, 0.25% IOP Publishing 1 publication, 0.25%
ASME	ASME, 1, 0.25% ASME 1 publication, 0.25%
Taylor & Francis	Taylor & Francis, 1, 0.25% Taylor & Francis 1 publication, 0.25%
The Korean Electrochemical Society	The Korean Electrochemical Society, 1, 0.25% The Korean Electrochemical Society 1 publication, 0.25%
Hans Publishers	Hans Publishers, 1, 0.25% Hans Publishers 1 publication, 0.25%
Canadian Science Publishing	Canadian Science Publishing, 1, 0.25% Canadian Science Publishing 1 publication, 0.25%
OAE Publishing Inc.	OAE Publishing Inc., 1, 0.25% OAE Publishing Inc. 1 publication, 0.25%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.25% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.25%
	20 40 60 80 100 120 140

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Luo J. et al. Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer // Nano Letters. 2017. Vol. 17. No. 5. pp. 2967-2972.

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Luo J., Liu Y., Liu W., Zhou G., Zhao J., Zu C., Sheng O., Zhang W., Lee H., Cui Y. Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer // Nano Letters. 2017. Vol. 17. No. 5. pp. 2967-2972.

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TY - JOUR

DO - 10.1021/acs.nanolett.7b00221

UR - https://doi.org/10.1021/acs.nanolett.7b00221

TI - Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer

T2 - Nano Letters

AU - Zu, Chenxi

AU - Luo, Jianmin

AU - Liu, Wei

AU - Liu, Yayuan

AU - Zhou, Guangmin

AU - Zhao, Jie

AU - Cui, Yi

AU - Sheng, Ouwei

AU - Zhang, Wenkui

AU - Lee, Hyun-Wook

PY - 2017

DA - 2017/04/12 00:00:00

PB - American Chemical Society (ACS)

SP - 2967-2972

IS - 5

VL - 17

SN - 1530-6984

SN - 1530-6992

ER -

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BibTex Copy

@article{2017_Luo,

author = {Chenxi Zu and Jianmin Luo and Wei Liu and Yayuan Liu and Guangmin Zhou and Jie Zhao and Yi Cui and Ouwei Sheng and Wenkui Zhang and Hyun-Wook Lee},

title = {Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer},

journal = {Nano Letters},

year = {2017},

volume = {17},

publisher = {American Chemical Society (ACS)},

month = {apr},

url = {https://doi.org/10.1021/acs.nanolett.7b00221},

number = {5},

pages = {2967--2972},

doi = {10.1021/acs.nanolett.7b00221}

}

MLA

Cite this

MLA Copy

Luo, Jianmin, et al. “Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer.” Nano Letters, vol. 17, no. 5, Apr. 2017, pp. 2967-2972. https://doi.org/10.1021/acs.nanolett.7b00221.

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Publisher

American Chemical Society (ACS)

Journal

Nano Letters

Quartile SCImago

Quartile WOS

Impact factor

10.8

ISSN

15306984 (Print)
15306992 (Electronic)