Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer
Jianmin Luo
1, 2
,
Yayuan Liu
2
,
Wei Liu
2
,
Guangmin Zhou
2
,
Jie Zhao
2
,
Chenxi Zu
2
,
Ouwei Sheng
1
,
Wenkui Zhang
1
,
Hyun-Wook Lee
2
,
Yi Cui
2, 3
Publication type: Journal Article
Publication date: 2017-04-12
scimago Q1
wos Q1
SJR: 2.967
CiteScore: 14.9
Impact factor: 9.1
ISSN: 15306984, 15306992
PubMed ID:
28388080
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
An all solid-state lithium-ion battery with high energy density and high safety is a promising solution for a next-generation energy storage system. High interface resistance of the electrodes and poor ion conductivity of solid-state electrolytes are two main challenges for solid-state batteries, which require operation at elevated temperatures of 60-90 °C. Herein, we report the facile synthesis of Al3+/Nb5+ codoped cubic Li7La3Zr2O12 (LLZO) nanoparticles and LLZO nanoparticle-decorated porous carbon foam (LLZO@C) by the one-step Pechini sol-gel method. The LLZO nanoparticle-filled poly(ethylene oxide) electrolyte shows improved conductivity compared with filler-free samples. The sulfur composite cathode based on LLZO@C can deliver an attractive specific capacity of >900 mAh g-1 at the human body temperature 37 °C and a high capacity of 1210 and 1556 mAh g-1 at 50 and 70 °C, respectively. In addition, the solid-state Li-S batteries exhibit high Coulombic efficiency and show remarkably stable cycling performance.
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Total citations:
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GOST
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Luo J. et al. Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer // Nano Letters. 2017. Vol. 17. No. 5. pp. 2967-2972.
GOST all authors (up to 50)
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Luo J., Liu Y., Liu W., Zhou G., Zhao J., Zu C., Sheng O., Zhang W., Lee H., Cui Y. Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer // Nano Letters. 2017. Vol. 17. No. 5. pp. 2967-2972.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.nanolett.7b00221
UR - https://doi.org/10.1021/acs.nanolett.7b00221
TI - Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer
T2 - Nano Letters
AU - Luo, Jianmin
AU - Liu, Yayuan
AU - Liu, Wei
AU - Zhou, Guangmin
AU - Zhao, Jie
AU - Zu, Chenxi
AU - Sheng, Ouwei
AU - Zhang, Wenkui
AU - Lee, Hyun-Wook
AU - Cui, Yi
PY - 2017
DA - 2017/04/12
PB - American Chemical Society (ACS)
SP - 2967-2972
IS - 5
VL - 17
PMID - 28388080
SN - 1530-6984
SN - 1530-6992
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2017_Luo,
author = {Jianmin Luo and Yayuan Liu and Wei Liu and Guangmin Zhou and Jie Zhao and Chenxi Zu and Ouwei Sheng and Wenkui Zhang and Hyun-Wook Lee and Yi Cui},
title = {Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer},
journal = {Nano Letters},
year = {2017},
volume = {17},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/acs.nanolett.7b00221},
number = {5},
pages = {2967--2972},
doi = {10.1021/acs.nanolett.7b00221}
}
Cite this
MLA
Copy
Luo, Jianmin, et al. “Solid-State Lithium–Sulfur Batteries Operated at 37 °C with Composites of Nanostructured Li7La3Zr2O12/Carbon Foam and Polymer.” Nano Letters, vol. 17, no. 5, Apr. 2017, pp. 2967-2972. https://doi.org/10.1021/acs.nanolett.7b00221.