Nano Letters, volume 17, issue 5, pages 3182-3187

A Flexible Solid Composite Electrolyte with Vertically Aligned and Connected Ion-Conducting Nanoparticles for Lithium Batteries

H Zhai ¹

Pengyu Xu ¹

Mingqiang Ning ^{1, 2}

Qian Cheng ¹

Jyotirmoy Mandal ¹

Yuan Yang ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

Program of Materials Science and Engineering, Department of Applied Physics and Applied Mathematics, Columbia University, New York, New York 10025, United States |

School of Materials Science & Engineering, Beijing Institute of Technology, Beijing, 100081, China |

Publication type: Journal Article

Publication date: 2017-04-24

American Chemical Society (ACS)

Journal: Nano Letters

Quartile SCImago

Quartile WOS

Impact factor: 10.8

ISSN: 15306984, 15306992

DOI: 10.1021/acs.nanolett.7b00715

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General Chemistry

Condensed Matter Physics

General Materials Science

Mechanical Engineering

Bioengineering

Abstract

Replacing flammable organic liquid electrolytes with solid Li-ion conductors is a promising approach to realize safe rechargeable batteries with high energy density. Composite solid electrolytes, which are comprised of a polymer matrix with ceramic Li-ion conductors dispersed inside, are attractive, since they combine the flexibility of polymer electrolytes and high ionic conductivities of ceramic electrolytes. However, the high conductivity of ceramic fillers is largely compromised by the low conductivity of the matrix, especially when nanoparticles (NPs) are used. Therefore, optimizations of the geometry of ceramic fillers are critical to further enhance the conductivity of composite electrolytes. Here we report the vertically aligned and connected Li1+xAlxTi2-x(PO4)3 (LATP) NPs in the poly(ethylene oxide) (PEO) matrix to maximize the ionic conduction, while maintaining the flexibility of the composite. This vertically aligned structure can be fabricated by an ice-templating-based method, and its conductivity reaches 0.52 × 10-4 S/cm, which is 3.6 times that of the composite electrolyte with randomly dispersed LATP NPs. The composite electrolyte also shows enhanced thermal and electrochemical stability compared to the pure PEO electrolyte. This method opens a new approach to optimize ion conduction in composite solid electrolytes for next-generation rechargeable batteries.

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Citations by journals

	5 10 15 20 25
Energy Storage Materials	Energy Storage Materials, 22, 5.38% Energy Storage Materials 22 publications, 5.38%
ACS applied materials & interfaces	ACS applied materials & interfaces, 20, 4.89% ACS applied materials & interfaces 20 publications, 4.89%
Chemical Engineering Journal	Chemical Engineering Journal, 17, 4.16% Chemical Engineering Journal 17 publications, 4.16%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 12, 2.93% Journal of Materials Chemistry A 12 publications, 2.93%
Advanced Energy Materials	Advanced Energy Materials, 11, 2.69% Advanced Energy Materials 11 publications, 2.69%
Journal of Power Sources	Journal of Power Sources, 10, 2.44% Journal of Power Sources 10 publications, 2.44%
Advanced Materials	Advanced Materials, 10, 2.44% Advanced Materials 10 publications, 2.44%
ACS Applied Energy Materials	ACS Applied Energy Materials, 10, 2.44% ACS Applied Energy Materials 10 publications, 2.44%
Advanced Functional Materials	Advanced Functional Materials, 9, 2.2% Advanced Functional Materials 9 publications, 2.2%
Advanced Science	Advanced Science, 9, 2.2% Advanced Science 9 publications, 2.2%
Journal of Energy Chemistry	Journal of Energy Chemistry, 7, 1.71% Journal of Energy Chemistry 7 publications, 1.71%
Nano Energy	Nano Energy, 7, 1.71% Nano Energy 7 publications, 1.71%
Journal of Energy Storage	Journal of Energy Storage, 7, 1.71% Journal of Energy Storage 7 publications, 1.71%
Electrochimica Acta	Electrochimica Acta, 7, 1.71% Electrochimica Acta 7 publications, 1.71%
Small	Small, 7, 1.71% Small 7 publications, 1.71%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 6, 1.47% Journal of the Electrochemical Society 6 publications, 1.47%
Solid State Ionics	Solid State Ionics, 6, 1.47% Solid State Ionics 6 publications, 1.47%
Energy and Environmental Science	Energy and Environmental Science, 6, 1.47% Energy and Environmental Science 6 publications, 1.47%
Nano Research	Nano Research, 5, 1.22% Nano Research 5 publications, 1.22%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 5, 1.22% Journal of Colloid and Interface Science 5 publications, 1.22%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 5, 1.22% Journal of Alloys and Compounds 5 publications, 1.22%
Nano-Micro Letters	Nano-Micro Letters, 4, 0.98% Nano-Micro Letters 4 publications, 0.98%
Angewandte Chemie	Angewandte Chemie, 4, 0.98% Angewandte Chemie 4 publications, 0.98%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 4, 0.98% Angewandte Chemie - International Edition 4 publications, 0.98%
ACS Energy Letters	ACS Energy Letters, 4, 0.98% ACS Energy Letters 4 publications, 0.98%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 4, 0.98% Journal of Physical Chemistry C 4 publications, 0.98%
Energy & Fuels	Energy & Fuels, 4, 0.98% Energy & Fuels 4 publications, 0.98%
Chemical Society Reviews	Chemical Society Reviews, 4, 0.98% Chemical Society Reviews 4 publications, 0.98%
Materials Chemistry Frontiers	Materials Chemistry Frontiers, 4, 0.98% Materials Chemistry Frontiers 4 publications, 0.98%
	5 10 15 20 25

Citations by publishers

	20 40 60 80 100 120 140
Elsevier	Elsevier, 138, 33.74% Elsevier 138 publications, 33.74%
Wiley	Wiley, 87, 21.27% Wiley 87 publications, 21.27%
American Chemical Society (ACS)	American Chemical Society (ACS), 66, 16.14% American Chemical Society (ACS) 66 publications, 16.14%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 45, 11% Royal Society of Chemistry (RSC) 45 publications, 11%
Springer Nature	Springer Nature, 26, 6.36% Springer Nature 26 publications, 6.36%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 8, 1.96% Multidisciplinary Digital Publishing Institute (MDPI) 8 publications, 1.96%
The Electrochemical Society	The Electrochemical Society, 6, 1.47% The Electrochemical Society 6 publications, 1.47%
Frontiers Media S.A.	Frontiers Media S.A., 5, 1.22% Frontiers Media S.A. 5 publications, 1.22%
IOP Publishing	IOP Publishing, 3, 0.73% IOP Publishing 3 publications, 0.73%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 2, 0.49% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 2 publications, 0.49%
Tsinghua University Press	Tsinghua University Press, 2, 0.49% Tsinghua University Press 2 publications, 0.49%
World Scientific	World Scientific, 1, 0.24% World Scientific 1 publication, 0.24%
Chemical Industry Press	Chemical Industry Press, 1, 0.24% Chemical Industry Press 1 publication, 0.24%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.24% Korean Society of Industrial Engineering Chemistry 1 publication, 0.24%
KeAi Communications Co.	KeAi Communications Co., 1, 0.24% KeAi Communications Co. 1 publication, 0.24%
Chinese Ceramic Society	Chinese Ceramic Society, 1, 0.24% Chinese Ceramic Society 1 publication, 0.24%
Taylor & Francis	Taylor & Francis, 1, 0.24% Taylor & Francis 1 publication, 0.24%
Oxford University Press	Oxford University Press, 1, 0.24% Oxford University Press 1 publication, 0.24%
Chinese Physical Society	Chinese Physical Society, 1, 0.24% Chinese Physical Society 1 publication, 0.24%
Hindawi Limited	Hindawi Limited, 1, 0.24% Hindawi Limited 1 publication, 0.24%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 1, 0.24% Proceedings of the National Academy of Sciences (PNAS) 1 publication, 0.24%
Research Square Platform LLC	Research Square Platform LLC, 1, 0.24% Research Square Platform LLC 1 publication, 0.24%
	20 40 60 80 100 120 140

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Zhai H. et al. A Flexible Solid Composite Electrolyte with Vertically Aligned and Connected Ion-Conducting Nanoparticles for Lithium Batteries // Nano Letters. 2017. Vol. 17. No. 5. pp. 3182-3187.

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Zhai H., Xu P., Ning M., Cheng Q., Mandal J., Yang Y. A Flexible Solid Composite Electrolyte with Vertically Aligned and Connected Ion-Conducting Nanoparticles for Lithium Batteries // Nano Letters. 2017. Vol. 17. No. 5. pp. 3182-3187.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acs.nanolett.7b00715

UR - https://doi.org/10.1021/acs.nanolett.7b00715

TI - A Flexible Solid Composite Electrolyte with Vertically Aligned and Connected Ion-Conducting Nanoparticles for Lithium Batteries

T2 - Nano Letters

AU - Xu, Pengyu

AU - Ning, Mingqiang

AU - Zhai, H

AU - Cheng, Qian

AU - Mandal, Jyotirmoy

AU - Yang, Yuan

PY - 2017

DA - 2017/04/24 00:00:00

PB - American Chemical Society (ACS)

SP - 3182-3187

IS - 5

VL - 17

SN - 1530-6984

SN - 1530-6992

ER -

BibTex |

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BibTex Copy

@article{2017_Zhai,

author = {Pengyu Xu and Mingqiang Ning and H Zhai and Qian Cheng and Jyotirmoy Mandal and Yuan Yang},

title = {A Flexible Solid Composite Electrolyte with Vertically Aligned and Connected Ion-Conducting Nanoparticles for Lithium Batteries},

journal = {Nano Letters},

year = {2017},

volume = {17},

publisher = {American Chemical Society (ACS)},

month = {apr},

url = {https://doi.org/10.1021/acs.nanolett.7b00715},

number = {5},

pages = {3182--3187},

doi = {10.1021/acs.nanolett.7b00715}

}

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MLA Copy

Zhai, H., et al. “A Flexible Solid Composite Electrolyte with Vertically Aligned and Connected Ion-Conducting Nanoparticles for Lithium Batteries.” Nano Letters, vol. 17, no. 5, Apr. 2017, pp. 3182-3187. https://doi.org/10.1021/acs.nanolett.7b00715.

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Publisher

American Chemical Society (ACS)

Journal

Nano Letters

Quartile SCImago

Quartile WOS

Impact factor

10.8

ISSN

15306984 (Print)
15306992 (Electronic)