volume 17 issue 12 pages 7761-7766

Dynamic Optical Tuning of Interlayer Interactions in the Transition Metal Dichalcogenides.

Clara Nyby 2
Friederike Ernst 3, 4
Yao Zhou 1
John Tolsma 5
Yao Li 3
Meng Ju Sher 6, 7
I Cheng Tung 8
Hua Zhou 8
Qi Zhang 8
Kyle L Seyler 9
GENEVIEVE CLARK 9
Yu Lin 6, 10
Diling Zhu 11
James M. Glownia 11
Sanghoon Song 11
Silke Nelson 11
Apurva Mehta 11
YIFEI YU 12
Anupum Pant 13
Burak Aslan 3
Archana Raja 3, 4
Yinsheng Guo 14
Anthony Dichiara 8
Wendy Mao 4, 6, 10
Linyou Cao 12
Jifeng Sun 15
DAVID J. SINGH 15
Tony F. Heinz 3, 4, 6
Xiaodong Xu 9
Allan H. MacDonald 5
Evan Reed 1, 4
Haidan Wen 8
A.M. Lindenberg 1, 4, 6
Publication typeJournal Article
Publication date2017-11-09
scimago Q1
wos Q1
SJR2.967
CiteScore14.9
Impact factor9.1
ISSN15306984, 15306992
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
Modulation of weak interlayer interactions between quasi-two-dimensional atomic planes in the transition metal dichalcogenides (TMDCs) provides avenues for tuning their functional properties. Here we show that above-gap optical excitation in the TMDCs leads to an unexpected large-amplitude, ultrafast compressive force between the two-dimensional layers, as probed by in situ measurements of the atomic layer spacing at femtosecond time resolution. We show that this compressive response arises from a dynamic modulation of the interlayer van der Waals interaction and that this represents the dominant light-induced stress at low excitation densities. A simple analytic model predicts the magnitude and carrier density dependence of the measured strains. This work establishes a new method for dynamic, nonequilibrium tuning of correlation-driven dispersive interactions and of the optomechanical functionality of TMDC quasi-two-dimensional materials.
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Mannebach E. M. et al. Dynamic Optical Tuning of Interlayer Interactions in the Transition Metal Dichalcogenides. // Nano Letters. 2017. Vol. 17. No. 12. pp. 7761-7766.
GOST all authors (up to 50) Copy
Mannebach E. M., Nyby C., Ernst F., Zhou Y., Tolsma J., Li Y., Sher M. J., Tung I. C., Zhou H., Zhang Q., Seyler K. L., CLARK G., Lin Yu., Zhu D., Glownia J. M., Kozina M. E., Song S., Nelson S., Mehta A., YU Y., Pant A., Aslan B., Raja A., Guo Y., Dichiara A., Mao W., Cao L., Tongay S., Sun J., SINGH D. J., Heinz T. F., Xu X., MacDonald A. H., Reed E., Wen H., Lindenberg A. Dynamic Optical Tuning of Interlayer Interactions in the Transition Metal Dichalcogenides. // Nano Letters. 2017. Vol. 17. No. 12. pp. 7761-7766.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1021/acs.nanolett.7b03955
UR - https://doi.org/10.1021/acs.nanolett.7b03955
TI - Dynamic Optical Tuning of Interlayer Interactions in the Transition Metal Dichalcogenides.
T2 - Nano Letters
AU - Mannebach, Ehren M
AU - Nyby, Clara
AU - Ernst, Friederike
AU - Zhou, Yao
AU - Tolsma, John
AU - Li, Yao
AU - Sher, Meng Ju
AU - Tung, I Cheng
AU - Zhou, Hua
AU - Zhang, Qi
AU - Seyler, Kyle L
AU - CLARK, GENEVIEVE
AU - Lin, Yu
AU - Zhu, Diling
AU - Glownia, James M.
AU - Kozina, Michael E.
AU - Song, Sanghoon
AU - Nelson, Silke
AU - Mehta, Apurva
AU - YU, YIFEI
AU - Pant, Anupum
AU - Aslan, Burak
AU - Raja, Archana
AU - Guo, Yinsheng
AU - Dichiara, Anthony
AU - Mao, Wendy
AU - Cao, Linyou
AU - Tongay, Sefaattin
AU - Sun, Jifeng
AU - SINGH, DAVID J.
AU - Heinz, Tony F.
AU - Xu, Xiaodong
AU - MacDonald, Allan H.
AU - Reed, Evan
AU - Wen, Haidan
AU - Lindenberg, A.M.
PY - 2017
DA - 2017/11/09
PB - American Chemical Society (ACS)
SP - 7761-7766
IS - 12
VL - 17
PMID - 29119791
SN - 1530-6984
SN - 1530-6992
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2017_Mannebach,
author = {Ehren M Mannebach and Clara Nyby and Friederike Ernst and Yao Zhou and John Tolsma and Yao Li and Meng Ju Sher and I Cheng Tung and Hua Zhou and Qi Zhang and Kyle L Seyler and GENEVIEVE CLARK and Yu Lin and Diling Zhu and James M. Glownia and Michael E. Kozina and Sanghoon Song and Silke Nelson and Apurva Mehta and YIFEI YU and Anupum Pant and Burak Aslan and Archana Raja and Yinsheng Guo and Anthony Dichiara and Wendy Mao and Linyou Cao and Sefaattin Tongay and Jifeng Sun and DAVID J. SINGH and Tony F. Heinz and Xiaodong Xu and Allan H. MacDonald and Evan Reed and Haidan Wen and A.M. Lindenberg},
title = {Dynamic Optical Tuning of Interlayer Interactions in the Transition Metal Dichalcogenides.},
journal = {Nano Letters},
year = {2017},
volume = {17},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/acs.nanolett.7b03955},
number = {12},
pages = {7761--7766},
doi = {10.1021/acs.nanolett.7b03955}
}
MLA
Cite this
MLA Copy
Mannebach, Ehren M., et al. “Dynamic Optical Tuning of Interlayer Interactions in the Transition Metal Dichalcogenides..” Nano Letters, vol. 17, no. 12, Nov. 2017, pp. 7761-7766. https://doi.org/10.1021/acs.nanolett.7b03955.