Nano Letters, volume 18, issue 5, pages 3104-3112
Mg2B2O5 Nanowire Enabled Multifunctional Solid-State Electrolytes with High Ionic Conductivity, Excellent Mechanical Properties, and Flame-Retardant Performance
Publication type: Journal Article
Publication date: 2018-04-25
Journal:
Nano Letters
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 10.8
ISSN: 15306984, 15306992
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
High ionic conductivity, satisfactory mechanical properties, and wide electrochemical windows are crucial factors for composite electrolytes employed in solid-state lithium-ion batteries (SSLIBs). Based on these considerations, we fabricate Mg2B2O5 nanowire enabled poly(ethylene oxide) (PEO)-based solid-state electrolytes (SSEs). Notably, these SSEs have enhanced ionic conductivity and a large electrochemical window. The elevated ionic conductivity is attributed to the improved motion of PEO chains and the increased Li migrating pathway on the interface between Mg2B2O5 and PEO-LiTFSI. Moreover, the interaction between Mg2B2O5 and -SO2- in TFSI- anions could also benefit the improvement of conductivity. In addition, the SSEs containing Mg2B2O5 nanowires exhibit improved the mechanical properties and flame-retardant performance, which are all superior to the pristine PEO-LiTFSI electrolyte. When these multifunctional SSEs are paired with LiFePO4 cathodes and lithium metal anodes, the SSLIBs show better rate performance and higher cyclic capacity of 150, 106, and 50 mAh g-1 under 0.2 C at 50, 40, and 30 °C. This strategy of employing Mg2B2O5 nanowires provides the design guidelines of assembling multifunctional SSLIBs with high ionic conductivity, excellent mechanical properties, and flame-retardant performance at the same time.
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Citations by publishers
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Elsevier
106 publications, 39.55%
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Wiley
53 publications, 19.78%
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2 publications, 0.75%
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2 publications, 0.75%
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1 publication, 0.37%
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1 publication, 0.37%
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1 publication, 0.37%
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Pleiades Publishing
1 publication, 0.37%
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Trans Tech Publications
1 publication, 0.37%
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Proceedings of the National Academy of Sciences (PNAS)
1 publication, 0.37%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 0.37%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Sheng O. et al. Mg2B2O5 Nanowire Enabled Multifunctional Solid-State Electrolytes with High Ionic Conductivity, Excellent Mechanical Properties, and Flame-Retardant Performance // Nano Letters. 2018. Vol. 18. No. 5. pp. 3104-3112.
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Sheng O., Jin C., Luo J., Yuan H., Huang H., Gan Y., Zhang J., Xia Y., Chu L., Zhang W. Mg2B2O5 Nanowire Enabled Multifunctional Solid-State Electrolytes with High Ionic Conductivity, Excellent Mechanical Properties, and Flame-Retardant Performance // Nano Letters. 2018. Vol. 18. No. 5. pp. 3104-3112.
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TY - JOUR
DO - 10.1021/acs.nanolett.8b00659
UR - https://doi.org/10.1021/acs.nanolett.8b00659
TI - Mg2B2O5 Nanowire Enabled Multifunctional Solid-State Electrolytes with High Ionic Conductivity, Excellent Mechanical Properties, and Flame-Retardant Performance
T2 - Nano Letters
AU - Sheng, Ouwei
AU - Jin, Chengbin
AU - Luo, Jianmin
AU - Yuan, Huadong
AU - Gan, Yongping
AU - Xia, Yang
AU - Chu, Liang
AU - Zhang, Wenkui
AU - Huang, Hui
AU - Zhang, Jun
PY - 2018
DA - 2018/04/25 00:00:00
PB - American Chemical Society (ACS)
SP - 3104-3112
IS - 5
VL - 18
SN - 1530-6984
SN - 1530-6992
ER -
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@article{2018_Sheng,
author = {Ouwei Sheng and Chengbin Jin and Jianmin Luo and Huadong Yuan and Yongping Gan and Yang Xia and Liang Chu and Wenkui Zhang and Hui Huang and Jun Zhang},
title = {Mg2B2O5 Nanowire Enabled Multifunctional Solid-State Electrolytes with High Ionic Conductivity, Excellent Mechanical Properties, and Flame-Retardant Performance},
journal = {Nano Letters},
year = {2018},
volume = {18},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/acs.nanolett.8b00659},
number = {5},
pages = {3104--3112},
doi = {10.1021/acs.nanolett.8b00659}
}
Cite this
MLA
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Sheng, Ouwei, et al. “Mg2B2O5 Nanowire Enabled Multifunctional Solid-State Electrolytes with High Ionic Conductivity, Excellent Mechanical Properties, and Flame-Retardant Performance.” Nano Letters, vol. 18, no. 5, Apr. 2018, pp. 3104-3112. https://doi.org/10.1021/acs.nanolett.8b00659.