Nano Letters, volume 18, issue 6, pages 3829-3838

Vertically Aligned and Continuous Nanoscale Ceramic–Polymer Interfaces in Composite Solid Polymer Electrolytes for Enhanced Ionic Conductivity

Xiaokun Zhang ^{1, 2}

Jin Xie ¹

Feifei Shi ¹

Yi Cui ¹

Yayuan Liu ¹

Wei Liu ¹

Allen Pei ¹

Yongji Gong ¹

Hongxia Wang ¹

Kai Liu ¹

Yong Xiang ²

Yi Cui ^{1, 3}

Hide authors affiliations Show authors affiliations: 3 affiliations

Department of Materials Science and Engineering, Stanford University, Stanford, California 94305, United States |

School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu, Sichuan 611731, People’s Republic of China |

Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, United States |

Publication type: Journal Article

Publication date: 2018-05-04

American Chemical Society (ACS)

Journal: Nano Letters

Quartile SCImago

Quartile WOS

Impact factor: 10.8

ISSN: 15306984, 15306992

DOI: 10.1021/acs.nanolett.8b01111

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General Chemistry

Condensed Matter Physics

General Materials Science

Mechanical Engineering

Bioengineering

Abstract

Among all solid electrolytes, composite solid polymer electrolytes, comprised of polymer matrix and ceramic fillers, garner great interest due to the enhancement of ionic conductivity and mechanical properties derived from ceramic-polymer interactions. Here, we report a composite electrolyte with densely packed, vertically aligned, and continuous nanoscale ceramic-polymer interfaces, using surface-modified anodized aluminum oxide as the ceramic scaffold and poly(ethylene oxide) as the polymer matrix. The fast Li+ transport along the ceramic-polymer interfaces was proven experimentally for the first time, and an interfacial ionic conductivity higher than 10-3 S/cm at 0 °C was predicted. The presented composite solid electrolyte achieved an ionic conductivity as high as 5.82 × 10-4 S/cm at the electrode level. The vertically aligned interfacial structure in the composite electrolytes enables the viable application of the composite solid electrolyte with superior ionic conductivity and high hardness, allowing Li-Li cells to be cycled at a small polarization without Li dendrite penetration.

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Citations by journals

	5 10 15 20 25
ACS applied materials & interfaces	ACS applied materials & interfaces, 21, 7.53% ACS applied materials & interfaces 21 publications, 7.53%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 15, 5.38% Journal of Materials Chemistry A 15 publications, 5.38%
Journal of Power Sources	Journal of Power Sources, 13, 4.66% Journal of Power Sources 13 publications, 4.66%
Chemical Engineering Journal	Chemical Engineering Journal, 13, 4.66% Chemical Engineering Journal 13 publications, 4.66%
Energy Storage Materials	Energy Storage Materials, 13, 4.66% Energy Storage Materials 13 publications, 4.66%
Small	Small, 10, 3.58% Small 10 publications, 3.58%
Advanced Functional Materials	Advanced Functional Materials, 10, 3.58% Advanced Functional Materials 10 publications, 3.58%
Journal of Energy Chemistry	Journal of Energy Chemistry, 8, 2.87% Journal of Energy Chemistry 8 publications, 2.87%
Advanced Science	Advanced Science, 6, 2.15% Advanced Science 6 publications, 2.15%
Advanced Energy Materials	Advanced Energy Materials, 6, 2.15% Advanced Energy Materials 6 publications, 2.15%
Journal of Membrane Science	Journal of Membrane Science, 6, 2.15% Journal of Membrane Science 6 publications, 2.15%
Nano Energy	Nano Energy, 6, 2.15% Nano Energy 6 publications, 2.15%
Nano Letters	Nano Letters, 6, 2.15% Nano Letters 6 publications, 2.15%
ACS Applied Energy Materials	ACS Applied Energy Materials, 5, 1.79% ACS Applied Energy Materials 5 publications, 1.79%
Journal of Energy Storage	Journal of Energy Storage, 4, 1.43% Journal of Energy Storage 4 publications, 1.43%
Advanced Materials	Advanced Materials, 4, 1.43% Advanced Materials 4 publications, 1.43%
Materials Chemistry Frontiers	Materials Chemistry Frontiers, 4, 1.43% Materials Chemistry Frontiers 4 publications, 1.43%
Journal of Polymer Research	Journal of Polymer Research, 3, 1.08% Journal of Polymer Research 3 publications, 1.08%
Rare Metals	Rare Metals, 3, 1.08% Rare Metals 3 publications, 1.08%
Nano-Micro Letters	Nano-Micro Letters, 3, 1.08% Nano-Micro Letters 3 publications, 1.08%
Materials Today Energy	Materials Today Energy, 3, 1.08% Materials Today Energy 3 publications, 1.08%
Applied Surface Science	Applied Surface Science, 3, 1.08% Applied Surface Science 3 publications, 1.08%
Energy & Environmental Materials	Energy & Environmental Materials, 3, 1.08% Energy & Environmental Materials 3 publications, 1.08%
Energy & Fuels	Energy & Fuels, 3, 1.08% Energy & Fuels 3 publications, 1.08%
ACS Sustainable Chemistry and Engineering	ACS Sustainable Chemistry and Engineering, 3, 1.08% ACS Sustainable Chemistry and Engineering 3 publications, 1.08%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 3, 1.08% Journal of Physical Chemistry C 3 publications, 1.08%
Journal of Materials Science	Journal of Materials Science, 2, 0.72% Journal of Materials Science 2 publications, 0.72%
Materials	Materials, 2, 0.72% Materials 2 publications, 0.72%
Science China Materials	Science China Materials, 2, 0.72% Science China Materials 2 publications, 0.72%
	5 10 15 20 25

Citations by publishers

	10 20 30 40 50 60 70 80 90 100
Elsevier	Elsevier, 99, 35.48% Elsevier 99 publications, 35.48%
Wiley	Wiley, 56, 20.07% Wiley 56 publications, 20.07%
American Chemical Society (ACS)	American Chemical Society (ACS), 49, 17.56% American Chemical Society (ACS) 49 publications, 17.56%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 25, 8.96% Royal Society of Chemistry (RSC) 25 publications, 8.96%
Springer Nature	Springer Nature, 18, 6.45% Springer Nature 18 publications, 6.45%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 7, 2.51% Multidisciplinary Digital Publishing Institute (MDPI) 7 publications, 2.51%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 5, 1.79% American Institute of Physics (AIP) 5 publications, 1.79%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 3, 1.08% Nonferrous Metals Society of China 3 publications, 1.08%
Tsinghua University Press	Tsinghua University Press, 2, 0.72% Tsinghua University Press 2 publications, 0.72%
Taylor & Francis	Taylor & Francis, 2, 0.72% Taylor & Francis 2 publications, 0.72%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.36% American Association for the Advancement of Science (AAAS) 1 publication, 0.36%
The Electrochemical Society	The Electrochemical Society, 1, 0.36% The Electrochemical Society 1 publication, 0.36%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.36% Frontiers Media S.A. 1 publication, 0.36%
Chemical Industry Press	Chemical Industry Press, 1, 0.36% Chemical Industry Press 1 publication, 0.36%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.36% Taiwan Institute of Chemical Engineers 1 publication, 0.36%
IOP Publishing	IOP Publishing, 1, 0.36% IOP Publishing 1 publication, 0.36%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.36% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.36%
	10 20 30 40 50 60 70 80 90 100

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Zhang X. et al. Vertically Aligned and Continuous Nanoscale Ceramic–Polymer Interfaces in Composite Solid Polymer Electrolytes for Enhanced Ionic Conductivity // Nano Letters. 2018. Vol. 18. No. 6. pp. 3829-3838.

GOST all authors (up to 50) Copy

Zhang X., Xie J., Shi F., Cui Y., Liu Y., Liu W., Pei A., Gong Y., Wang H., Liu K., Xiang Y., Cui Y. Vertically Aligned and Continuous Nanoscale Ceramic–Polymer Interfaces in Composite Solid Polymer Electrolytes for Enhanced Ionic Conductivity // Nano Letters. 2018. Vol. 18. No. 6. pp. 3829-3838.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/acs.nanolett.8b01111

UR - https://doi.org/10.1021/acs.nanolett.8b01111

TI - Vertically Aligned and Continuous Nanoscale Ceramic–Polymer Interfaces in Composite Solid Polymer Electrolytes for Enhanced Ionic Conductivity

T2 - Nano Letters

AU - Shi, Feifei

AU - Liu, Yayuan

AU - Gong, Yongji

AU - Zhang, Xiaokun

AU - Xie, Jin

AU - Cui, Yi

AU - Liu, Wei

AU - Pei, Allen

AU - Wang, Hongxia

AU - Liu, Kai

AU - Xiang, Yong

AU - Cui, Yi

PY - 2018

DA - 2018/05/04 00:00:00

PB - American Chemical Society (ACS)

SP - 3829-3838

IS - 6

VL - 18

SN - 1530-6984

SN - 1530-6992

ER -

BibTex |

Cite this

BibTex Copy

@article{2018_Zhang,

author = {Feifei Shi and Yayuan Liu and Yongji Gong and Xiaokun Zhang and Jin Xie and Yi Cui and Wei Liu and Allen Pei and Hongxia Wang and Kai Liu and Yong Xiang and Yi Cui},

title = {Vertically Aligned and Continuous Nanoscale Ceramic–Polymer Interfaces in Composite Solid Polymer Electrolytes for Enhanced Ionic Conductivity},

journal = {Nano Letters},

year = {2018},

volume = {18},

publisher = {American Chemical Society (ACS)},

month = {may},

url = {https://doi.org/10.1021/acs.nanolett.8b01111},

number = {6},

pages = {3829--3838},

doi = {10.1021/acs.nanolett.8b01111}

}

MLA

Cite this

MLA Copy

Zhang, Xiaokun, et al. “Vertically Aligned and Continuous Nanoscale Ceramic–Polymer Interfaces in Composite Solid Polymer Electrolytes for Enhanced Ionic Conductivity.” Nano Letters, vol. 18, no. 6, May. 2018, pp. 3829-3838. https://doi.org/10.1021/acs.nanolett.8b01111.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Nano Letters

Quartile SCImago

Quartile WOS

Impact factor

10.8

ISSN

15306984 (Print)
15306992 (Electronic)